Records |
Author |
Callebaut, D.K.; Makarovska, Y. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
On the relationship between current and magnetic field in ring-filaments |
Type |
P1 Proceeding |
Year |
1998 |
Publication |
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Abbreviated Journal |
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Volume |
150 |
Issue |
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Pages |
111-114
T2 - IAU Colloquium 167 on New Perspective |
Keywords |
P1 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
Abstract |
There is a type of filament that forms dosed contours encircling regions of one polarity of magnetic field, while the surrounding region has the opposite polarity One distribution of ring-filaments has sizes 2R = 40,000 to 160,000 km with the maximum around 100,000 km; the other distribution (with filaments and filament channels) has bigger sizes, with a maximum around 300,000 km. At low and mid latitudes the radial component B-rs (radial for the Sun) in the region outlined by filaments varies from 50 to 100 gauss, while the longitudinal component B-phi varies from 10 to 30 gauss. The total current inside the filament is 10(10) – 10(11) A, the ratio R/a approximate to 5 to 10, the magnetic flux crossing the surface is approximate to 10(21) – 10(22) MX; th, magnetic energy is approximate to 10(29) – 10(31) erg. Polar ring-filaments at latitudes 60 degrees-80 degrees are related to the polar magnetic field reversal and the quasi-flare processes at the poles during the field reversal. Correlation between B-rs and B-phi for the polar filament bands cannot be satisfactorily explained. A theoretical model using the conservation laws is used to study the relations between the various fields, currents, etc, of shrinking polar ring-filaments and their evolution. According to this theory ring-filaments should rise higher above the photosphere when shrinking. However, observations show that the height lowers. Presumably the discrepancy is due to the lack of dissipation in the model. |
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000076565100020 |
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1-886733-70-8 |
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no |
Call Number |
UA @ admin @ c:irua:95844 |
Serial |
8333 |
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Author |
Zhang, H. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Optical diagnostics of spatiotemporal evolution characteristics of nanosecond laser-induced plasma in gases |
Type |
Doctoral thesis |
Year |
2020 |
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Pages |
117 p. |
Keywords |
Doctoral thesis; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:171436 |
Serial |
6572 |
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Author |
Barnes, D.J.; Nicholas, R.J.; Watts, M.; Peeters, F.M.; Wu, X.G.; Devreese, J.T.; Langerak, C.J.; Singleton, J.; Harris, J.J.; Foxon, C.T. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Optically detected magnetophonon resonance in GaAs-GaAlAs heterojunctions |
Type |
P3 Proceeding |
Year |
1991 |
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P3 Proceeding; Condensed Matter Theory (CMT); Theory of quantum systems and complex systems |
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Springer |
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Berlin |
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0000-00-00 |
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PHYSICS, APPLIED 47/145 Q2 # |
Call Number |
UA @ lucian @ c:irua:961 |
Serial |
2478 |
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Author |
Gonnissen, J. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Optimal statistical experiment design for detecting and locating light atoms using quantitative high resolution (scanning) transmission electron microscopy |
Type |
Doctoral thesis |
Year |
2017 |
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Doctoral thesis; Electron microscopy for materials research (EMAT) |
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Antwerpen |
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Call Number |
UA @ lucian @ c:irua:140612 |
Serial |
4444 |
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Author |
Robberecht, H.; Van Grieken, R.; Van der Sloot, H.A. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
OPtimized selenite determination in environmental waters by X-ray fluorescence |
Type |
H3 Book chapter |
Year |
1980 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
463-468
T2 - Analytical techniques in environmenta |
Keywords |
H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
Call Number |
UA @ admin @ c:irua:117482 |
Serial |
8343 |
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Author |
Michel, K.H.; Copley, J.R.D. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Orientation fluctuations, diffuse scattering and orientational order in solid C60 |
Type |
H3 Book chapter |
Year |
1996 |
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Pages |
381-384 |
Keywords |
H3 Book chapter; Condensed Matter Theory (CMT) |
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World Scientific |
Place of Publication |
Singapore |
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0000-00-00 |
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COMPUTER SCIENCE, INTERDISCIPLINARY 11/104 Q1 # PHYSICS, MATHEMATICAL 1/53 Q1 # |
Call Number |
UA @ lucian @ c:irua:16358 |
Serial |
2512 |
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Author |
Nikolaev, A.V.; Michel, K.H.; Copley, J.R.D. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Orientational disorder and order in C60-fullerite and in MC60-alkali metal fullerides |
Type |
H3 Book chapter |
Year |
1999 |
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Pages |
183-214 |
Keywords |
H3 Book chapter; Condensed Matter Theory (CMT) |
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Plenum Press |
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New York |
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0000-00-00 |
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Approved |
Most recent IF: NA |
Call Number |
UA @ lucian @ c:irua:28505 |
Serial |
2515 |
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Author |
Mozo, I.; Lacoste, L.; Aussenac, J.; De Cocker, P.; Vlaeminck, S.E.; Sperandio, M.; Caligaris, M.; Barillon, B.; Martin Ruel, S. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Overcoming the challenges for mainstream deammonification on municipal wastewater in warm and cold areas |
Type |
P3 Proceeding |
Year |
2016 |
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Pages |
3 p.
T2 - 13th IWA Leading-Edge Conference on Wate |
Keywords |
P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
Call Number |
UA @ admin @ c:irua:151137 |
Serial |
8351 |
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Author |
Janssens, K.; Adams, F. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Overview |
Type |
H3 Book chapter |
Year |
2000 |
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Pages |
1-16 |
Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:27577 |
Serial |
5764 |
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Author |
Mitchell, T.E.; Gronsky, R.; Van Tendeloo, G. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Oxide superconductors: electron microscopy |
Type |
H3 Book chapter |
Year |
1992 |
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Pages |
401-408 |
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H3 Book chapter; Electron microscopy for materials research (EMAT) |
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Pergamon Press |
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Oxford |
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0000-00-00 |
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no |
Call Number |
UA @ lucian @ c:irua:4435 |
Serial |
2543 |
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Author |
Zou, H.; Krekels, T.; Van Tendeloo, G.; Wagener, G.; Buchgeister, M.; Hosseini, S.M.; Kopitzki, K. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Oxygen ordering and critical temperature plateaus in ABa2Cu3O7-d (A=Er, Nd, Sm, Yb), pp |
Type |
P3 Proceeding |
Year |
1992 |
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Pages |
278-279 |
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P3 Proceeding; Electron microscopy for materials research (EMAT) |
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Beijing |
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0000-00-00 |
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no |
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UA @ lucian @ c:irua:4443 |
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2547 |
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Madani, M.; Bogaerts, A.; Gijbels, R.; Vangeneugden, D. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Parametric study by means of numerical modelling for a dielectric barrier discharge at atmospheric pressure in nitrogen |
Type |
P3 Proceeding |
Year |
2004 |
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Pages |
49-52 |
Keywords |
P3 Proceeding; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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S.l. |
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0000-00-00 |
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Most recent IF: NA |
Call Number |
UA @ lucian @ c:irua:82304 |
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2554 |
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Author |
Wegrzynek, D.; Van Grieken, R.; Eisma, D. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Particle analysis of sediments from the Gulf of Lions, suspended matter from the Rhone river, and Sahara dust |
Type |
H3 Book chapter |
Year |
1994 |
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Abbreviated Journal |
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Pages |
51-60
T2 - Particles and particle-water interactio |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
Call Number |
UA @ admin @ c:irua:9525 |
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8358 |
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Verreydt, G.; Bronders, J.; van Keer, I.; Diels, L.; Vanderauwera, P. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Passive samplers for monitoring VOCs in groundwater : prospects related to mass flux measurements |
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P3 Proceeding |
Year |
2011 |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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978-1-907161-16-2 |
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Call Number |
UA @ admin @ c:irua:110412 |
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8364 |
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Peeters, B.; Safdar, S.; Carlier, B.; Spasic, D.; Daems, D.; Lammertyn, J. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
PCR amplified DNAzyme-amplicons for generic solid-phase antimicrobial resistance screening |
Type |
P1 Proceeding |
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2019 |
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971-974
T2 - Transducers 2019 : Eurosensors XXXIII |
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P1 Proceeding; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
Abstract |
Fiber optic surface plasmon resonance (FO-SPR) has shown its potential for the detection of nucleic acids and more recently the technology has been combined with catalytic active strands such as DNAzymes. In this work, an innovative, generic solid-phase DNA sensor concept is presented, based on FO-SPR and PCR amplified DNAzyme activity. Improved levels of specificity and sensitivity were obtained down to picomolar concentrations. Moreover, the FO-SPR sensor concept enables AuNP amplified DNA target detection, independent of the target sequence length. The FO-SPR sensor was demonstrated for the screening of the mobile colistin resistance (MCR-2) gene, a gene important for the antimicrobial resistance in Gram-negative species such as E. Coli. |
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000539487000245 |
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no |
Call Number |
UA @ admin @ c:irua:166108 |
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8367 |
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Author |
Buysse, C. |
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Perovskite capillaries for gas separation in sustainable energy production |
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Doctoral thesis |
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2011 |
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201 p. |
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Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
Call Number |
UA @ admin @ c:irua:90548 |
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8373 |
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Brunekreef, B.; Janssen, N., A.H.; de Hartog, J., J.; Oldenwening, M.; Meliefste, K.; Hoek, G.; Lanki, T.; Timonen, K., L.; Vallius, M.; Pekkanen, J.; Van Grieken, R. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Personal, indoor, and outdoor exposures to PM2.5 and its components for groups of cardiovascular patients in Amsterdam and Helsinki |
Type |
Minutes and reports |
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2005 |
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Minutes and reports; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
Call Number |
UA @ admin @ c:irua:51816 |
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8374 |
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Author |
Van Hal, M. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Photo(electro)catalytic air purification and soot degradation with simultaneous energy recovery |
Type |
Doctoral thesis |
Year |
2021 |
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Issue |
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Pages |
XXXII, 203 p. |
Keywords |
Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
Abstract |
Today’s society is increasingly challenged by a range of urgent environmental problems. Air pollution is one of these pressing topics. This thesis will mainly focus on the degradation of volatile organic compounds (VOCs) and particulate matter (PM) – more specifically soot. A second globally urging topic is the quest for sustainable energy production. To simultaneously target both environmental problems, a photoelectrochemical (PEC) cell will be studied in this thesis, combining air purification and sustainable energy production in a single device. Photocatalysis is used at the anode of the PEC cell to drive the air purification process, while the energy contained in the degraded compounds is (partially) recovered at the cathode, either as H2 gas or electricity. The first two experimental chapters focus on the proof of concept of such an unbiased all-gas phase PEC cell targeting VOC degradation, using both TiO2- and WO3-based photocatalysts. In the two following experimental chapters the photocatalytic soot oxidation capacity of these TiO2- and WO3-based photocatalysts was studied. In the final experimental chapter the previously obtained results were combined, striving towards an efficient, sunlight-driven and soot-degrading waste gas-to-energy PEC cell. |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:184521 |
Serial |
8378 |
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Author |
Borah, R. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Photoactive nanostructures : from single plasmonic nanoparticles to self-assembled films |
Type |
Doctoral thesis |
Year |
2022 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
xxxiv, 220 p. |
Keywords |
Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
Abstract |
Photoactive nanoparticles and their light-driven applications have gained tremendous scientific attention towards remediation of the global environmental problems, meeting alternative energy demands, and other new technological discoveries. The research work presented in this dissertation includes a fundamental investigation of such nanoparticles to gain deeper insights that will ultimately benefit their application. In particular, the study of plasmonic metal nanoparticles and metal oxide nanoparticles for light driven applications is the major theme of this work. The investigation begins with isolated plasmonic Au and Ag nanoparticles, followed by a natural extension to nanoparticle clusters, and then further to nanoparticle films. Next, the application of such plasmonic nanoparticle films for gaseous phase sensing of volatile organic compounds is explored. Finally, the film formation of metal-oxide nanoparticles by self-assembly is investigated for the fabrication of photoactive functional interfaces. The fundamental theoretical investigation of the isolated plasmonic nanoparticles encompasses alloy and core-shell nanostructures of Au-Ag bimetallic compositions. First, the optical properties of bimetallic alloy and core-shell nanoparticles are compared for different structures such as nanospheres, nanotriangles and nanorods. Based on the optical properties, the photothermal properties of these nanostructures are also evaluated for relevant light-driven applications. Further, to bridge the gap between the theoretical and experimental optical properties of colloidal plasmonic nanoparticles, the effect of different statistical parameters pertaining to the particle size distribution is studied. Going from isolated nanoparticles to nanoparticle clusters, the changes in the optical properties of plasmonic nanoparticles when they form finite clusters is investigated. A strong effect of clustering on the absorption intensities of the nanoparticles and hence, on the photothermal properties is found. Next, for the study of plasmonic nanoparticle infinite arrays, Au and Ag nanoparticles films are experimentally obtained by the self-assembly at the air-ethylene glycol interface. Upon further validation of the computational models with the experimental optical properties of these films, the near-field and far-field optical response of the plasmonic nanoparticle arrays is investigated. An application of the self-assembled Au nanoparticle film is then demonstrated in the sensing of volatile organic compounds (VOCs). Finally, the focus is shifted from plasmonic nanoparticles to metal oxide nanoparticles for their self-assembly at the air-water interface to obtain self-assembled films. For this, the hydrophobic functionalization of four metal oxides nanoparticles namely, TiO2, ZnO, WO3 and CuO is investigated. The insights from this work is useful for the design and fabrication of functional nanoparticles and interfaces for light driven applications. |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:189155 |
Serial |
7188 |
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Author |
Smits, M. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Photocatalytic degradation of diesel soot : from application to reaction mechanism |
Type |
Doctoral thesis |
Year |
2013 |
Publication |
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Issue |
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Pages |
160 p. |
Keywords |
Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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978-90-5728-415-1 |
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UA library record |
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no |
Call Number |
UA @ admin @ c:irua:108803 |
Serial |
8380 |
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Author |
Verlinden, G.; Gijbels, R.; Geuens, I. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Photographic materials |
Type |
H3 Book chapter |
Year |
2001 |
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Issue |
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Pages |
727-752 |
Keywords |
H3 Book chapter; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Surface Spectra IM |
Place of Publication |
Chichester |
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0000-00-00 |
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Most recent IF: NA |
Call Number |
UA @ lucian @ c:irua:37256 |
Serial |
2613 |
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Author |
Remond, G.; Gijbels, R.; Levenson, L.L.; Shimizu, R. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Physics of generation and detection of signals used for microcharacterization |
Type |
ME3 Book as editor |
Year |
1994 |
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Pages |
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ME3 Book as editor; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Scanning Microscopy International |
Place of Publication |
Chicago, Ill. |
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0000-00-00 |
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no |
Call Number |
UA @ lucian @ c:irua:10258 |
Serial |
2619 |
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Author |
de Nolf, W.; Vekemans, B.; Janssens, K.; van der Snickt, G.; Falkenberg, G. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Pigment identification by scanning μ-XRF/μ-XRD |
Type |
H3 Book chapter |
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2007 |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:64595 |
Serial |
5773 |
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Author |
Idrissi, H.; Schryvers, D.; Salje, E.K.H.; Zhang, H.; Carpenter, M.A.; Moya, X. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Pinning of the martensitic microstructures by dislocations in Cu74.08Al23.13Be2.79 |
Type |
P1 Proceeding |
Year |
2009 |
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Pages |
02029,1-02029,5 |
Keywords |
P1 Proceeding; Electron microscopy for materials research (EMAT) |
Abstract |
A single crystal of Cu74.08Al23.13Be2.79 undergoes a martensitic phase transition at 246K and 232K under heating and cooling, respectively. Surprisingly, the martensite phase is elastically much harder than the austenite phase showing that interfaces between various crystallographic variants are strongly pinned and can not be moved by external stress while the phase boundary between the austenite and martensite regions in the sample remains mobile. This unusual behavior was revealed by Dynamical Mechanical Analysis and Resonant Ultrasound Spectroscopy. Transmission Electron Microscopy shows that the pinning is generated by dislocations, which are inherited from the austenite phase. Such dislocations can hinder the movement of stacking faults in the 18R martensite structure or twin boundaries between martensite variants. |
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Edp |
Place of Publication |
Coutaboeuf |
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000274582300033 |
Publication Date |
2009-08-31 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
Impact Factor |
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Times cited |
2 |
Open Access |
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Notes |
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Approved |
Most recent IF: NA |
Call Number |
UA @ lucian @ c:irua:81952 |
Serial |
2626 |
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Author |
Liu, X.; Van Winckel, T.; Kjellerup, B.V.; Takacs, I.; Sturm, B.; Vlaeminck, S.E.; Al-Omari, A.; Murthy, S.; De Clippeleir, H. |
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Pinpointing bioflocculation limitations for enhanced carbon management in high-rate activated sludge |
Type |
P3 Proceeding |
Year |
2017 |
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Pages |
6 p.
T2 - WEF Nutrient Symposium 2017, 12 - 14 Jun |
Keywords |
P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
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UA @ admin @ c:irua:151118 |
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8384 |
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Gao, J.; Huang, W.; Gielis, J.; Shi, P. |
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Plant morphology and function, geometric morphometrics, and modelling : decoding the mathematical secrets of plants |
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ME3 Book as editor |
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2023 |
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224 p. |
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ME3 Book as editor; Sustainable Energy, Air and Water Technology (DuEL) |
Abstract |
Delve into the diverse aspects of plant morphology, their responses to global climate change, and the spatiotemporal dynamics of forest productivity. Join us on a journey through the intricate web of plant characteristics and their impact on the environment. |
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2024-01-02 |
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978-3-0365-9422-4; 978-3-0365-9423-1 |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:201545 |
Serial |
9073 |
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Author |
Clavel, J. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Plant-mycorrhizal interactions and their role in plant invasions in mountains |
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Doctoral thesis |
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2024 |
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182 p. |
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Doctoral thesis; Plant and Ecosystems (PLECO) – Ecology in a time of change |
Abstract |
Non-native species invasions are one of the most impactful drivers of biodiversity and ecosystem services loss worldwide. One aspect of plant species invasion, which is only recently starting to be recognized as a determinant of invasion success, is the symbiosis between plant and mycorrhizal fungi. Here, I focus on anthropogenic disturbance in mountain ecosystems and its impact on plant communities and mycorrhizal fungi to answer how these communities are impacted by disturbance and whether non-native plants can benefit to establish and spread. To this end I used a combination of different approaches: 1) repeated surveys of plants and arbuscular mycorrhizal fungi along disturbed roadsides in the mountains of Norway, 2) combining a global dataset of native and non-native plants along mountain roads with a database associating plants with their mycorrhizal types, and 3) an in-situ experiment measuring non-native plant success and changes in fungal community following different types of disturbances. Through these methods, I could assess the effects of anthropogenic disturbance on mycorrhizal symbiosis and non-native plant species at multiple scales and resolutions. We found that road disturbance has a globally consistent effect on mycorrhizal types in mountain systems, as plants associated with arbuscular mycorrhizal (AM) fungi were more abundant following disturbance. Conversely, vegetation associated with either ectomycorrhizal (EcM) or ericoid mycorrhizal (ErM) fungi was less abundant in disturbed sites. In the regional study, AM fungi were most abundant and diverse in the roots of plant communities affected by road disturbance. Non-native plants were also restricted to these disturbed sites. The experimental results showed that physical disturbance and nutrient addition have negative effects on EcM fungi and positive effects on fungal pathogens, and facilitate non-native plant success. Our results show that anthropogenic disturbance does have an effect on mycorrhizal fungi that in turn impacts the distribution of plant species in disturbed mountain systems. The resulting shift in mycorrhizal fungi benefiting AM fungi and AM plant species could have implications for non-native plant invasions. Indeed, we know that non-native plants predominantly form associations with AM fungi. Therefore, anthropogenic disturbance can facilitate non-native plant success through disruption of the native fungal communities, and especially so in high elevation and cold climate regions which are naturally less dominated by AM plants. I believe this highlights the importance of mycorrhizal symbiosis in understanding plant invasions and emphasizes the importance of monitoring sources of anthropogenic disturbance in mountains to prevent future establishment of non-native plants. |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:204154 |
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9219 |
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Van Wesenbeeck, K.; Hauchecorne, B.; Lenaerts, S. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Plasma assisted catalysis : an efficient and sustainable indoor air purification technology |
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P3 Proceeding |
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2012 |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:127490 |
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5981 |
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Van Wesenbeeck, K.; Hauchecorne, B.; Lenaerts, S. |
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Plasma catalysis : integration of a photocatalytic coating in a corona discharge unit |
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P3 Proceeding |
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2013 |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:127487 |
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5982 |
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Author |
Wang, J. |
Title ![sorted by Title field, ascending order (up)](img/sort_asc.gif) |
Plasma catalysis : study of CO2 reforming of CH4 in a DBD reactor |
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Doctoral thesis |
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2022 |
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XVI, 232 p. |
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Doctoral thesis; Engineering sciences. Technology; Laboratory of adsorption and catalysis (LADCA); Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
Abstract |
The plasma-based dry reforming in a dielectric barrier discharge (DBD) reactor is important to achieve sustainable goals, but many challenges remain. For example, the conversion and energy yield of DBD reactors are relatively low, and the catalysts or packing materials used in existing studies cannot improve them, possibly due to the unsuitable properties and structures of catalysts or packing materials for plasma processes. In order to study the effect of catalyst structure on plasma-based dry reforming, a controllable synthesis of the catalyst supports or templates was explored. In Chapter 2, an initially immiscible synthesis method was proposed to synthesize uniform silica spheres, which can replace the organic solvent-based Stöber method to successfully synthesize silica particles with the same size ranges as the original Stöber process without addition of organic solvents. Using the silica spheres as templates, 3D porous Cu and CuO catalysts with different pore sizes were synthesized in Chapter 3 to study the effect of catalyst pore size on the plasma-catalytic dry reforming. In most cases, the smaller the pore size, the higher the conversion of CH4 and CO2 due to the reaction of radicals and ions formed in the plasma. An exception are the samples synthesized from 1 μm silica, which show better performance due to the electric field enhancement for pore sizes close to the Debye length. Besides the pore size, the particle diameter of the catalyst or packing is also one of the important factors affecting the interaction between plasma and catalyst. In Chapter 4, SiO2 spheres (with or without supported metal) were used to study the effect of different support particle sizes on plasma-based dry reforming. We found that a uniform SiO2 packing improves the conversion of plasma-based dry reforming. The conversion of plasma-based dry reforming first increases and then decreases with increasing particle size, due to the balance between the promoting and hindering effect of the particle filling on the plasma discharge. Chapter 5 is to improve the design of the DBD reactor itself, in order to try to increase its low energy yield. Some stainless steel rings were put over the inner electrode rod of the DBD reactor. The presence of rings increases the local electric field, the displaced charges and the discharge fraction, and also makes the discharge more stable and with more uniform intensity. The placement of the rings improves the performance of the reactor at 30 W supplied power. |
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Approved |
Most recent IF: NA |
Call Number |
UA @ admin @ c:irua:194045 |
Serial |
7273 |
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