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| Author | Lv, H.; Meng, S.; Cui, Z.; Li, S.; Li, D.; Gao, X.; Guo, H.; Bogaerts, A.; Yi, Y. | ||||
| Title | Plasma-catalytic direct oxidation of methane to methanol over Cu-MOR: Revealing the zeolite-confined Cu2+ active sites | Type | A1 Journal Article | ||
| Year | 2024 | Publication | Chemical Engineering Journal | Abbreviated Journal | Chemical Engineering Journal |
| Volume | 496 | Issue | Pages | 154337 | |
| Keywords | A1 Journal Article; Direct oxidation Methanol production Plasma catalysis Copper-mordenite catalysts; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | Efficient methane conversion to methanol remains a significant challenge in chemical industry. This study investigates the direct oxidation of methane to methanol under mild conditions, employing a synergy of nonthermal plasma and Cu-MOR (Copper-Mordenite) catalysts. Catalytic tests demonstrate that the Cu-MOR IE-3 catalyst (i.e., prepared by three cycles of ion exchange) exhibits superior catalytic performance (with 51 % methanol selectivity and 7.9 % methane conversion). Conversely, the Cu-MOR catalysts prepared via wetness impregnation tend to over-oxidize CH4 to CO and CO2. Through systematic catalyst characterizations (XRD, TPR, UV–Vis, HRTEM, XPS), we elucidate that ion exchange mainly leads to the formation of zeolite-confined Cu2+ species, while wetness impregnation predominantly results in CuO particles. Based on the catalytic performance, catalyst characterizations and in-situ FTIR spectra, we conclude that zeolite-confined Cu2+ species serve as the active sites for plasma-catalytic direct oxidation of methane to methanol. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos  |
Publication Date | 2024-08-02 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 1385-8947 | ISBN | Additional Links | ||
| Impact Factor | 15.1 | Times cited | Open Access | ||
| Notes | PetroChina Innovation Foundation, 2018D-5007-0501 ; Fundamental Research Funds for the Central Universities, DUT21JC40 ; Fundamental Research Funds for the Central Universities; China Scholarship Council; National Natural Science Foundation of China, 22272015 ; | Approved | Most recent IF: 15.1; 2024 IF: 6.216 | ||
| Call Number | PLASMANT @ plasmant @ | Serial | 9260 | ||
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| Author | Vertongen, R.; De Felice, G.; van den Bogaard, H.; Gallucci, F.; Bogaerts, A.; Li, S. | ||||
| Title | Sorption-Enhanced Dry Reforming of Methane in a DBD Plasma Reactor for Single-Stage Carbon Capture and Utilization | Type | A1 Journal Article | ||
| Year | 2024 | Publication | ACS Sustainable Chemistry & Engineering | Abbreviated Journal | ACS Sustainable Chem. Eng. |
| Volume | 12 | Issue | 29 | Pages | 10841-10853 |
| Keywords | A1 Journal Article; plasma, dry reforming of methane, dielectric barrier discharge, sorbent, carbon capture and utilization, zeolite; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | Plasma−sorbent systems are a novel technology for single-stage carbon capture and utilization (CCU), where the plasma enables the desorption of CO2 from a sorbent and the simultaneous conversion to CO. In this study, we test the flexibility of a plasma−sorbent system in a single unit, specifically for sorption-enhanced dry reforming of methane (DRM). The experimental results indicate the selective adsorption of CO2 by the sorbent zeolite 5A in the first step, and CH4 addition during the plasma-based desorption of CO2 enables DRM to various value-added products in the second step, such as H2, CO, hydrocarbons, and the byproduct H2O. Furthermore, our work also demonstrates that zeolite has the potential to increase the conversion of CO2 and CH4, attributed to its capability to capture H2O. Aside from the notable carbon deposition, material analysis shows that the zeolite remains relatively stable under plasma exposure. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2024-07-22 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 2168-0485 | ISBN | Additional Links | ||
| Impact Factor | 8.4 | Times cited | Open Access | ||
| Notes | Fonds Wetenschappelijk Onderzoek, 110221N V404823N ; H2020 European Research Council, 810182 ; | Approved | Most recent IF: 8.4; 2024 IF: 5.951 | ||
| Call Number | PLASMANT @ plasmant @ | Serial | 9264 | ||
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| Author | Albrechts, M.; Tsonev, I.; Bogaerts, A. | ||||
| Title | Can post-plasma CH4injection improve plasma-based dry reforming of methane? A modeling study | Type | A1 Journal Article | ||
| Year | 2024 | Publication | Green Chemistry | Abbreviated Journal | Green Chem. |
| Volume | 26 | Issue | 18 | Pages | 9712-9728 |
| Keywords | A1 Journal Article; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | Thermal plasma-driven dry reforming of methane (DRM) has gained increased attention in recent years due to its high conversion and energy conversion efficiency (ECE). Recent experimental work investigated the performance of a pure CO<sub>2</sub>plasma with post-plasma CH<sub>4</sub>injection. The rationale behind this strategy is that by utilizing a pure CO<sub>2</sub>plasma, all plasma energy can be used to dissociate CO<sub>2</sub>, while CH<sub>4</sub>reforming proceeds post-plasma in the reforming reactor with residual heat, potentially improving the energy efficiency compared to injecting both CO<sub>2</sub>and CH<sub>4</sub>into the plasma. To assess whether post-plasma CH<sub>4</sub>injection indeed improves the DRM performance, we developed a chemical kinetics model describing the post-plasma conversion process. We first validated our model by reproducing the experimental results of the pure CO<sub>2</sub>plasma with post-plasma CH<sub>4</sub>injection. Subsequently, we compared both strategies: injecting only CO<sub>2</sub>inside the plasma while injecting CH<sub>4</sub>post-plasma,<italic>vs.</italic>classical plasma-based DRM. Our modeling results indicate that below specific energy inputs (SEI) of 220 kJ mol<sup>−1</sup>, the total conversion slightly improves (<italic>ca.</italic>5%) with the first strategy. However, the ECE is slightly lower due to the low H<sub>2</sub>selectivity caused by substantial H<sub>2</sub>O formation. The highest conversion and ECE are obtained at SEI values of 240–280 kJ mol<sup>−1</sup>, where both strategies yield nearly identical results, indicating the limited potential of improving the performance of DRM by pure CO<sub>2</sub>plasma with post-plasma CH<sub>4</sub>injection. Nevertheless, the approach is still very valuable to allow higher CH<sub>4</sub>/CO<sub>2</sub>ratios without problems of coke formation within the plasma, and thus, to improve plasma stability and reach higher syngas ratios, which is more useful for further Fischer–Tropsch or methanol synthesis. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2024-08-24 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 1463-9262 | ISBN | Additional Links | ||
| Impact Factor | 9.8 | Times cited | Open Access | ||
| Notes | HORIZON EUROPE Framework Programme, 101069491 ; | Approved | Most recent IF: 9.8; 2024 IF: 9.125 | ||
| Call Number | PLASMANT @ plasmant @ | Serial | 9265 | ||
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| Author | Sun, J.; Chen, Q.; Qin, W.; Wu, H.; Liu, B.; Li, S.; Bogaerts, A. | ||||
| Title | Plasma-catalytic dry reforming of CH4: Effects of plasma-generated species on the surface chemistry | Type | A1 Journal Article | ||
| Year | 2024 | Publication | Chemical Engineering Journal | Abbreviated Journal | Chemical Engineering Journal |
| Volume | 498 | Issue | Pages | 155847 | |
| Keywords | A1 Journal Article; Dry reforming of methane Plasma catalysis Plasma-enhanced surface chemistry Path flux and sensitivity analysis Coking kinetics; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | By means of steady-state experiments and a global model, we studied the effects of plasma-generated reactive species on the surface chemistry and coking in plasma-catalytic CH4/CO2 reforming at reduced pressure (8–40 kPa). We used a hybrid ZDPlasKin-CHEMKIN model to predict the species densities over time. The detailed plasma-catalytic mechanism consists of the plasma discharge scheme, a gas-phase chemistry set and a surface mechanism. Our experimental results show that the coupling of Ni/SiO2 catalyst with plasma is more effective in CH4/CO2 activation and conversion than unpacked DBD plasma, with syngas being the main products. The highest total conversion of 16 % was achieved at 8000 V and 473 K, with corresponding CO and H2 yields of 15 % and 12 %, respectively. The reactants conversion and product selectivity are well captured by the kinetic model. Our simulation results suggest that vibrational species and radicals can accelerate the dissociative adsorption and Eley-Rideal (E-R) reactions. Path flux analysis shows that E-R reactions dominate the surface reaction pathways, which differs from thermal catalysis, indicating that the coupling of non-equilibrium plasma and catalysis can effectively shift the formation and consumption pathways of important adsorbates. For instance, our model suggests that HCOO(s) is primarily generated through the E-R reaction CO2(v) + H(s) → HCOO(s), while the hydrogenation reaction HCOO(s) + H → HCOOH(s) is the main source of HCOOH(s). Carbon deposition on the catalyst surface is primarily formed through the stepwise dehydrogenation of CH4, while the E-R reactions enhanced by plasma-generated H and O atoms dominate the consumption of carbon deposition. This work provides new insights into the effects of reactive species on the surface chemistry in plasma-catalytic CH4/CO2 reforming. |
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2024-09-17 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 1385-8947 | ISBN | Additional Links | ||
| Impact Factor | 15.1 | Times cited | Open Access | ||
| Notes | National Natural Science Foundation of China; | Approved | Most recent IF: 15.1; 2024 IF: 6.216 | ||
| Call Number | PLASMANT @ plasmant @ | Serial | 9266 | ||
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| Author | Fedirchyk, I.; Tsonev, I.; Quiroz Marnef, R.; Bogaerts, A. | ||||
| Title | Plasma-assisted NH3 cracking in warm plasma reactors for green H2 production | Type | A1 Journal Article | ||
| Year | 2024 | Publication | Chemical Engineering Journal | Abbreviated Journal | Chemical Engineering Journal |
| Volume | 499 | Issue | Pages | 155946 | |
| Keywords | A1 Journal Article; Plasma-assisted NH3 cracking Plasma reactors Warm plasma H2 production from NH3; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | renewable energy. Plasma technology is promising for this purpose, as it can crack NH3 without the need for a catalyst and is highly compatible with renewable electricity, reducing the environmental footprint of the cracking process. This work investigates the NH3 cracking performance of four different warm plasma reactors with different configurations and operating in a wide range of conditions. We show that the NH3 conversion in warm plasma reactors is primarily determined by the specific energy input, with the main difference observed in the energy cost (EC) of cracking. The lowest EC obtained is 146 kJ/mol but at a conversion of only 8 %. A more reasonable conversion of around 50 % yields an EC of around 200 kJ/mol in two of the reactors investigated. Plasma reactors operating at higher feed flow rates are more efficient and yield a higher H2 production rate. Our data indicate that NH3 cracking in these warm plasma reactors occurs mainly via thermal chemistry, with nonthermal plasma chemistry playing a less prominent role. NH3 decomposes not only inside the plasma core but also in a hot volume around it, which reduces the EC. Our study shows that warm plasmas are significantly more efficient for NH3 cracking than cold plasmas, even when the latter are combined with catalysts. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2024-09-19 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 1385-8947 | ISBN | Additional Links | ||
| Impact Factor | 15.1 | Times cited | Open Access | ||
| Notes | Belgian Federal Government; European Commission Marie Sklodowska-Curie Actions; | Approved | Most recent IF: 15.1; 2024 IF: 6.216 | ||
| Call Number | PLASMANT @ plasmant @ | Serial | 9267 | ||
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| Author | Zani, V.; Renero-Lecuna, C.; Jimenez de Aberasturi, D.; di Silvio, D.; Kavak, S.; Bals, S.; Signorini, R.; Liz-Marzán, L.M. | ||||
| Title | Core–Shell Colloidal Nanocomposites for Local Temperature Monitoring during Photothermal Heating | Type | A1 Journal Article | ||
| Year | 2024 | Publication | The Journal of Physical Chemistry C | Abbreviated Journal | J. Phys. Chem. C |
| Volume | Issue | Pages | |||
| Keywords | A1 Journal Article; Electron Microscopy for Materials Science (EMAT) ; | ||||
| Abstract | Determining temperature changes at the heating site to accurately control thermal treatments has been a major goal in the field of nanothermometry. In this study, we address the need to effectively monitor local temperature during the application of photothermal therapies, which is essential to prevent uncontrolled heating induced by nanoparticle sensitizers used in such treatments. For this purpose, we developed a synthetic protocol to produce a nanocomposite probe that allows local photothermal heating and simultaneous in situ optical nanothermometry, within the biological transparency windows. The nanocomposite material comprises gold nanorods for light-to-heat conversion and neodymium (Nd3+)-based nanoparticles for local temperature monitoring. An inert spacer made of mesoporous silica provides a core-shell structure and ensures uniform separation between both functionalities to prevent photoluminescence quenching. By using an 808 nm laser as the source for both heating and photoluminescence excitation, we demonstrate a direct correlation between local temperature and near infrared Nd3+ emission intensities, thereby providing precise local temperature monitoring. Different levels of local heating were studied by varying the incident laser power, resulting in a maximum temperature increase of 47 °C detected with the nanothermometers. Albeit presented here as a proof of concept, this concept can be translated to the design of materials for photothermal therapy. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2024-10-03 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 1932-7447 | ISBN | Additional Links | ||
| Impact Factor | 3.7 | Times cited | Open Access | ||
| Notes | L.L.L.-M. acknowledges financial support by the Spanish Agencia Estatal de Investigación and FEDER (PID2023-151281OB-I00), S.K. acknowledges the Flemish Fund for Scientific Research (FWO Vlaanderen) through a PhD research grant (Project numbers: 1181122N & 1181124N) and the European Research Council (CoG 815128, REALNANO). | Approved | Most recent IF: 3.7; 2024 IF: 4.536 | ||
| Call Number | EMAT @ emat @ | Serial | 9328 | ||
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| Author | Taylor, P.R.; Martin, J.M.L.; François, J.P.; Gijbels, R. | ||||
| Title | An ab initio study of the C3+ cation using multireference methods | Type | A1 Journal article | ||
| Year | 1991 | Publication | The journal of chemical physics | Abbreviated Journal | J Chem Phys |
| Volume | 95 | Issue | Pages | 6530-6534 | |
| Keywords | A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
| Abstract | |||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | New York, N.Y. | Editor | ||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0021-9606 | ISBN | Additional Links | UA library record | |
| Impact Factor | 2.952 | Times cited | Open Access | ||
| Notes | Approved | no | |||
| Call Number | UA @ lucian @ c:irua:720 | Serial | 39 | ||
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| Author | Vandelannoote, R.; Blommaert, W.; Gijbels, R.; van Grieken, R. | ||||
| Title | Analysis of geothermal waters by spark source mass spectrometry | Type | A3 Journal article | ||
| Year | 1981 | Publication | Fresenius' Zeitschrift für analytische Chemie | Abbreviated Journal | |
| Volume | 309 | Issue | 4 | Pages | 291-294 |
| Keywords | A3 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT); AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Although the analysis of thermal water by spark-source mass spectrometry (SSMS) is rather timeconsuming, it allows the detection of about 20 elements of geochemical interest down to the ppb-level. A physical preconcentration is proposed in order to collect elements having quite different chemical properties, e.g. alkalis, transition elements, and elements occurring in anionic form. The relative sensitivity factors appear to be rather independent of the salt content of the graphite electrodes. Contrary to neutron activation analysis, SSMS has a quite uniform elemental sensitivity, and allows to determine elements for which neutron activation is not suitable, e.g. Sn and Pb. The precision of SSMS is however by a factor of about 2 worse than that obtained for neutron activation. | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | München | Editor | ||
| Language | Wos |
Publication Date | 2004-11-15 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0016-1152;1618-2650; | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | 8 | Open Access | ||
| Notes | Approved | no | |||
| Call Number | UA @ lucian @ c:irua:116638 | Serial | 100 | ||
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| Author | Van 't dack, L.; Blommaert, W.; Vandelannoote, R.; Gijbels, R.; van Grieken, R. | ||||
| Title | Equilibrium constants for trace elements in natural waters | Type | A1 Journal article | ||
| Year | 1983 | Publication | Reviews in analytical chemistry | Abbreviated Journal | |
| Volume | 7 | Issue | Pages | 297-401 | |
| Keywords | A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT); AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
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| Publisher | Place of Publication | Tel Aviv | Editor | ||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0048-752x | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ lucian @ c:irua:111446 | Serial | 1078 | ||
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| Author | Van Tendeloo, G. | ||||
| Title | Fullerenen: een nieuwe vorm van koolstof | Type | A3 Journal article | ||
| Year | 1995 | Publication | Echo 3: essays voor chemie-onderwijs | Abbreviated Journal | |
| Volume | Issue | Pages | 79-85 | ||
| Keywords | A3 Journal article; Electron microscopy for materials research (EMAT) | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | ISBN | Additional Links | UA library record | ||
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | MATERIALS SCIENCE, MULTIDISCIPLINARY 96/271 Q2 # | |||
| Call Number | UA @ lucian @ c:irua:13310 | Serial | 1296 | ||
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| Author | Bogaerts, A.; Gijbels, R. | ||||
| Title | Modeling of glow discharges: what can we learn from it? | Type | A3 Journal article | ||
| Year | 1997 | Publication | Analytical chemistry A-pages | Abbreviated Journal | |
| Volume | 69 | Issue | Pages | 719-727 | |
| Keywords | A3 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | ISBN | Additional Links | UA library record | ||
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | UA @ lucian @ c:irua:19611 | Serial | 2126 | ||
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| Author | Herrebout, D.; Bogaerts, A.; Gijbels, R. | ||||
| Title | Modelleren van plasmas gebruikt voor de afzetting van dunne lagen | Type | A2 Journal article | ||
| Year | 2004 | Publication | Chemie magazine | Abbreviated Journal | |
| Volume | Issue | 2 | Pages | 34-38 | |
| Keywords | A2 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0379-7651 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | UA @ lucian @ c:irua:82302 | Serial | 2149 | ||
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| Author | Adriaensen, L.; Vangaever, F.; Gijbels, R. | ||||
| Title | Organische TOF-S-SIMS: gebruik van opgedampt Ag en Au voor de verhoging van secundaire ionenintensiteiten | Type | A2 Journal article | ||
| Year | 2004 | Publication | Chemie magazine | Abbreviated Journal | |
| Volume | Issue | Pages | 10-12 | ||
| Keywords | A2 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
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| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Gent | Editor | ||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0379-7651 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | UA @ lucian @ c:irua:51979 | Serial | 2511 | ||
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| Author | Nikolaev, A.V.; Prassides, K.; Michel, K.H. | ||||
| Title | Phase transitions in AC60 (A=Rb, Cs) fullerides | Type | A3 Journal article | ||
| Year | 1997 | Publication | Recent advances in the chemistry and physics of fullerenes and related materials | Abbreviated Journal | |
| Volume | 5 | Issue | Pages | 450-460 | |
| Keywords | A3 Journal article; Condensed Matter Theory (CMT) | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | ISBN | Additional Links | UA library record | ||
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | UA @ lucian @ c:irua:21182 | Serial | 2596 | ||
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| Author | Blommaert, W.; Vandelannoote, R.; Van 't dack, L.; Gijbels, R.; van Grieken, R. | ||||
| Title | Relative evaluation of neutron activation, X-ray fluorescence and spark source mass spectrometry for multi-element analysis of geothermal waters | Type | A3 Journal article | ||
| Year | 1980 | Publication | Journal of radioanalytical chemistry | Abbreviated Journal | |
| Volume | 57 | Issue | Pages | 382-400 | |
| Keywords | A3 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT); AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 0000-00-00 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0134-0719 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | ||||
| Call Number | UA @ lucian @ c:irua:111432 | Serial | 2859 | ||
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| Author | Bogaerts, A.; Snoeckx, R.; Trenchev, G.; Wang, W. | ||||
| Title | Modeling for a Better Understanding of Plasma-Based CO2 Conversion | Type | H1 Book Chapter | ||
| Year | 2018 | Publication | Plasma Chemistry and Gas Conversion | Abbreviated Journal | |
| Volume | Issue | Pages | |||
| Keywords | H1 Book Chapter; Plasma, laser ablation and surface modeling Antwerp (PLASMANT) ; | ||||
| Abstract | This chapter discusses modeling efforts for plasma-based CO2 conversion, which are needed to obtain better insight in the underlying mechanisms, in order to improve this application. We will discuss two types of (complementary) modeling efforts that are most relevant, that is, (i) modeling of the detailed plasma chemistry by zero-dimensional (0D) chemical kinetic models and (ii) modeling of reactor design, by 2D or 3D fluid dynamics models. By showing some characteristic calculation results of both models, for CO2 splitting and in combination with a H-source, and for packed bed DBD and gliding arc plasma, we can illustrate the type of information they can provide. | ||||
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| Publisher | IntechOpen | Place of Publication | Rijeka | Editor | Britun, N.; Silva, T. |
| Language | Wos |
Publication Date | 2018-12-19 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | ISBN | Additional Links | UA library record | ||
| Impact Factor | Times cited | Open Access | Not_Open_Access | ||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | PLASMANT @ plasmant @ Bogaerts18c:irua:155915 | Serial | 5142 | ||
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| Author | Poma, G.; McGrath, T.J.; Christia, C.; Govindan, M.; Covaci, A. | ||||
| Title | Emerging halogenated flame retardants in the indoor environment | Type | A1 Journal article | ||
| Year | 2020 | Publication | Comprehensive analytical chemistry | Abbreviated Journal | |
| Volume | 88 | Issue | Pages | 107-140 | |
| Keywords | A1 Journal article; Pharmacology. Therapy; Electron microscopy for materials research (EMAT); Toxicological Centre | ||||
| Abstract | Indoor environments are considered an important contributor to external human exposure to halogenated flame retardants (HFRs) due to the large amounts of chemicals currently incorporated in indoor equipment and the time humans spend every day in indoor environments. In this chapter, the presence and use of novel brominated flame retardants (NBFRs), dechlorane plus (DPs), chlorinated organophosphorus flame retardants (Cl-PFRs) and chlorinated paraffins (CPs) in indoor dust, air and consumer products collected from different indoor microenvironments (homes, public indoor spaces, and vehicles) are discussed. While data on the concentrations of HFRs in indoor dust and air are widely available, figures are still scarce for consumer products, such as textiles and foams, furnishings, flooring, electric and electronic products and building materials. This knowledge gaps still represents the biggest obstacle in linking eventual sources of contamination to the presence and chemical patterns in indoor dust and air. | ||||
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| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2019-11-22 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 978-0-444-64339-1 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | OpenAccess | ||
| Notes | Approved | Most recent IF: NA | |||
| Call Number | UA @ admin @ c:irua:168776 | Serial | 6505 | ||
| Permanent link to this record | |||||
| Author | Reggers, C.; Van Grieken, R. | ||||
| Title | 2,2′-Diaminodiethylamine cellulose powder for trace metal preconcentrations from water | Type | A3 Journal article | ||
| Year | 1984 | Publication | Fresenius' Zeitschrift für analytische Chemie | Abbreviated Journal | |
| Volume | 317 | Issue | 5 | Pages | 520-526 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Cellulose powder with 2,2′-diaminodiethylamine (DEN) functional groups exhibits efficient complexation of transition metal cations. Collection yields above 85 % are obtained up to a chelation capacity of 1.5 meq per gram. Since a good collection is obtained for a pH up from 5, no pH adjustments have to be made for natural water samples. The cellulose-DEN powder is insensitive to abundant substances like alkali and alkaline earth ions, and humic matter. Some cations can be eluted efficiently in a small volume of HNO3. Blank concentration levels from the cellulose-DEN powder are reported. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2004-11-17 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0016-1152 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116640 | Serial | 7383 | ||
| Permanent link to this record | |||||
| Author | Mmari, A.G.; Potgieter-Vermaak, S.S.; Uiso, C.B.S.; Makundi, I.N.; Potgieter, J.H.; Van Grieken, R. | ||||
| Title | Corrosive marine atmosphere investigations in Tanzania: exposure sites and preliminary results | Type | A3 Journal article | ||
| Year | 2007 | Publication | Newsletter of the International Global Atmospheric Chemistry Project | Abbreviated Journal | |
| Volume | Issue | 36 | Pages | 13-18 | |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | |||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | |||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | ISBN | Additional Links | UA library record | ||
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:65012 | Serial | 7739 | ||
| Permanent link to this record | |||||
| Author | Puglisi, A.; Bassini, S.; Reimhult, E. | ||||
| Title | Cyclodextrin-appended superparamagnetic iron oxide nanoparticles as cholesterol-mopping agents | Type | A1 Journal article | ||
| Year | 2021 | Publication | Frontiers In Chemistry | Abbreviated Journal | Front Chem |
| Volume | 9 | Issue | Pages | 795598 | |
| Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Antwerp Electrochemical and Analytical Sciences Lab (A-Sense Lab) | ||||
| Abstract | Cholesterol plays a crucial role in major cardiovascular and neurodegenerative diseases, including Alzheimer’s disease and rare genetic disorders showing altered cholesterol metabolism. Cyclodextrins (CDs) have shown promising therapeutic efficacy based on their capacity to sequester and mobilise cholesterol. However, the administration of monomeric CDs suffers from several drawbacks due to their lack of specificity and poor pharmacokinetics. We present core-shell superparamagnetic iron oxide nanoparticles (SPIONs) functionalised with CDs appended to poly (2-methyl-2-oxazoline) polymers grafted in a dense brush to the iron oxide core. The CD-decorated nanoparticles (CySPIONs) are designed so that the macrocycle is specifically cleaved off the nanoparticle’s shell at a slightly acidic pH. In the intended use, free monomeric CDs will then mobilise cholesterol out of the lysosome to the cytosol and beyond through the formation of an inclusion complex. Hence, its suitability as a therapeutic platform to remove cholesterol in the lysosomal compartment. Synthesis and full characterization of the polymer as well as of the core-shell SPION are presented. Cholesterol-binding activity is shown through an enzymatic assay. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2021-11-18 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 2296-2646 | ISBN | Additional Links | UA library record | |
| Impact Factor | 3.994 | Times cited | Open Access | Not_Open_Access | |
| Notes | Approved | Most recent IF: 3.994 | |||
| Call Number | UA @ admin @ c:irua:192273 | Serial | 7749 | ||
| Permanent link to this record | |||||
| Author | Van Grieken, R.; Van 't dack, L.; Costa Dantas, C.; Moura de Amorim, W.; Maenhaut, W. | ||||
| Title | Elemental constituents of atmospheric aerosols in Recife, North-East Brazil | Type | A3 Journal article | ||
| Year | 1982 | Publication | Environmental pollution: series B : chemical and physical | Abbreviated Journal | |
| Volume | 4 | Issue | 2 | Pages | 143-163 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Few data are available on the inorganic atmospheric pollution in the rapidly expanding cities of South America, like Recife, on the Atlantic Coast of North-east Brazil. Therefore, the elemental composition of atmospheric aerosols was investigated for nine sites in the Recife conurbation and a fairly remote site in the area. Total aerosol samples were collected on cellulose filters for analysis by energy dispersive X-ray fluorescence and cascade impactors were used to collect the aerosols as a function of particle size for subsequent analysis by proton-induced X-ray emission. Local soil aliquots were also analysed. About eighteen elements were quantified in all cases. The average total atmospheric concentrations appeared to be well above natural levels but usually lower than, or comparable with, those of North American and European cities. Dispersal of sea spray and of local soil (often contaminated with, for example, Cu, Zn and Pb from industrial sources) contributes predominantly to the total atmospheric load in Recife. However, the particle size fraction results also indicated strong excesses in the small particle mode for S, K, V, Mn, Ni, Cu, Zn, Br and Pb, mainly in the downtown area. Again, the corresponding enrichment factors were only moderate in comparison with other published urban data. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2003-09-11 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0143-148x; 1878-0695 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:111437 | Serial | 7894 | ||
| Permanent link to this record | |||||
| Author | Van Grieken, R.; Markowicz, A.; Török, S. | ||||
| Title | Energy-dispersive X-ray spectrometry : present state and trends | Type | A3 Journal article | ||
| Year | 1986 | Publication | Fresenius' Zeitschrift für analytische Chemie | Abbreviated Journal | |
| Volume | 324 | Issue | 8 | Pages | 825-831 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Recent development, present state and expected future developments in energy-dispersive X-ray spectrometry are discussed. Attention is paid to the improvements in analytical selectivity, sensitivity, detection limit, quantitative character and applicability range, which are the result of new or better excitation sources, detectors, instrument design, automation, computer software and theoretical developments. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2004-11-15 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0016-1152 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116642 | Serial | 7907 | ||
| Permanent link to this record | |||||
| Author | Vanderborght, B.M.; Van Grieken, R.E. | ||||
| Title | Enrichment of trace metals in water by adsorption on activated carbon | Type | A1 Journal article | ||
| Year | 1977 | Publication | Analytical chemistry | Abbreviated Journal | |
| Volume | 49 | Issue | 2 | Pages | 311-316 |
| Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | |||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | |||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0003-2700; 5206-882x | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116513 | Serial | 7923 | ||
| Permanent link to this record | |||||
| Author | Van Grieken, R.; Speecke, A.; Hoste, J. | ||||
| Title | Geometry errors in 14 MeV neutron activation analysis | Type | A3 Journal article | ||
| Year | 1973 | Publication | Journal of radioanalytical chemistry | Abbreviated Journal | |
| Volume | 13 | Issue | 1 | Pages | 225-233 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | The effects of inaccurate sample sizes and sample positioning on 14 MeV neutron activation analysis results are estimated for 30, 20 and 10 mm diameter targets. It appears that axial positioning is the most critical parameter and that using a larger tritium target will yield an overall improvement of the reproducibility. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2006-10-11 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0134-0719; 2064-2857 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116453 | Serial | 7999 | ||
| Permanent link to this record | |||||
| Author | Van Schandevijl, R.; Van Grieken, R.; Hoste, J. | ||||
| Title | The half-life of 28Al | Type | A3 Journal article | ||
| Year | 1971 | Publication | Journal of radioanalytical chemistry | Abbreviated Journal | |
| Volume | 9 | Issue | 1 | Pages | 55-60 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | The half-life of28Al was redetermined on aluminium samples of different origin. Three different counting techniques were applied. The availability of highly purified samples (up to 99.9999%), the use of very fast electronic counting equipment and a complete automatisation allowed a good precision to be obtained in the final result of 2.2405 min. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2006-10-11 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0134-0719; 2064-2857 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116451 | Serial | 8016 | ||
| Permanent link to this record | |||||
| Author | Wegrzynek, D.; Jambers, W.; Van Grieken, R.; Eisma, D. | ||||
| Title | Individual particle analysis of Western Mediterranean sediment cores, Rhône suspended matter and Sahara aerosols: investigation of inputs to the sediments | Type | A1 Journal article | ||
| Year | 1997 | Publication | Marine chemistry | Abbreviated Journal | |
| Volume | 57 | Issue | Pages | 25-40 | |
| Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | |||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | |||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0304-4203; 1872-7581 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:18778 | Serial | 8079 | ||
| Permanent link to this record | |||||
| Author | Vandeputte, D.F.; Jacob, W.A.; Van Grieken, R.E. | ||||
| Title | Influence of fixation procedures on the microanalysis of lead-induced intranuclear inclusions in rat kidney | Type | A1 Journal article | ||
| Year | 1990 | Publication | The journal of histochemistry and cytochemistry | Abbreviated Journal | |
| Volume | 38 | Issue | 3 | Pages | 331-337 |
| Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Using Laser Microprobe Mass Analysis (LAMMA), we studied the chemical composition of lead-induced intranuclear inclusions in rat kidney tissue prepared by three different wet chemical fixation procedures for transmission electron microscopy. Fixation with glutaraldehyde-Na2S gave the same results as fixation with glutaraldehyde only: a high lead concentration could be detected. Therefore, for lead strongly bound to proteins, precipitation procedures are not essential. Post-fixation with osmium tetroxide drastically changed the composition of the inclusions: the lead concentration decreased substantially, while sodium, calcium, and barium were introduced. The osmium tetroxide fixative was found to be the source of the contamination. It also contained aluminum, and we suggest that other proteins (e.g., in neurofibrillary tangles) might be able to take up Al out of solution and that care must be exercised in interpreting the microanalytical results of osmium-fixed material. For the microanalysis of the lead inclusions, fixation with glutaraldehyde only provides a good compromise between preservation of the ultrastructure and maintenance of the element distribution. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2011-04-01 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0022-1554 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116831 | Serial | 8091 | ||
| Permanent link to this record | |||||
| Author | van de Vijver, F.L.; Verbueken, A.H.; Van Grieken, R.E.; de Broe, M.E.; Visser, W.J. | ||||
| Title | Laser microprobe mass analysis : a tool for evaluating histochemical staining of trace elements | Type | L1 Letter to the editor | ||
| Year | 1985 | Publication | Clinical chemistry : international journal of laboratory medicine and molecular diagnostics | Abbreviated Journal | |
| Volume | 31 | Issue | 2 | Pages | 351-352 |
| Keywords | L1 Letter to the editor; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) | ||||
| Abstract | |||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | |||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0009-9147; 1530-8561 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116715 | Serial | 8154 | ||
| Permanent link to this record | |||||
| Author | Denoyer, E.; Van Grieken, R.; Adams, F.; Ntausch, D.F.S. | ||||
| Title | Laser microprobe mass spectrometry : 1 : basic principles and performance characteristics | Type | A1 Journal article | ||
| Year | 1982 | Publication | Analytical chemistry | Abbreviated Journal | |
| Volume | 54 | Issue | 1 | Pages | 26a-33a |
| Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | |||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2012-05-29 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0003-2700; 5206-882x | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116517 | Serial | 8164 | ||
| Permanent link to this record | |||||
| Author | Vos, L.; Van Grieken, R. | ||||
| Title | Matrix effects and analysis of biological material by spark source mass spectrometry | Type | A3 Journal article | ||
| Year | 1985 | Publication | Fresenius' Zeitschrift für analytische Chemie | Abbreviated Journal | |
| Volume | 321 | Issue | 1 | Pages | 32-36 |
| Keywords | A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
| Abstract | Spark-source mass spectrometric analyses of synthetic simulated biological samples were performed to determine the importance of matrix effects. A correlation between the variation of the relative sensitivity coefficients (RSC's) and the spark plasma composition, hence plasma temperature, was found. The determined RSC's were used in the analysis of four biological standard reference materials. An accuracy of 1013% and detection limits between 0.005 and 0.5 ppm were obtained during analysis under normal conditions. | ||||
| Address | |||||
| Corporate Author | Thesis | ||||
| Publisher | Place of Publication | Editor | |||
| Language | Wos |
Publication Date | 2004-11-14 | ||
| Series Editor | Series Title | Abbreviated Series Title | |||
| Series Volume | Series Issue | Edition | |||
| ISSN | 0016-1152 | ISBN | Additional Links | UA library record | |
| Impact Factor | Times cited | Open Access | |||
| Notes | Approved | no | |||
| Call Number | UA @ admin @ c:irua:116641 | Serial | 8209 | ||
| Permanent link to this record | |||||