Records |
Author |
Zhang, Q.; De Clippeleir, H.; Su, C.; Al-Omari, A.; Wett, B.; Vlaeminck, S.E.; Murthy, S. |
Title |
Deammonification for digester supernatant pretreated with thermal hydrolysis : overcoming inhibition through process optimization |
Type |
A1 Journal article |
Year |
2016 |
Publication |
Applied microbiology and biotechnology |
Abbreviated Journal |
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Volume |
100 |
Issue |
12 |
Pages |
5595-5606 |
Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
Abstract |
The thermal hydrolysis process (THP) has been proven to be an excellent pretreatment step for an anaerobic digester (AD), increasing biogas yield and decreasing sludge disposal. The goal of this work was to optimize deammonification for efficient nitrogen removal despite the inhibition effects caused by the organics present in the THP-AD sludge filtrate (digestate). Two sequencing batch reactors were studied treating conventional digestate and THP-AD digestate, respectively. Improved process control based on higher dissolved oxygen set-point (1 mg O-2/L) and longer aeration times could achieve successful treatment of THP-AD digestate. This increased set-point could overcome the inhibition effect on aerobic ammonium-oxidizing bacteria (AerAOB), potentially caused by particulate and colloidal organics. Moreover, based on the mass balance, anoxic ammonium-oxidizing bacteria (AnAOB) contribution to the total nitrogen removal decreased from 97 +/- A 1 % for conventional to 72 +/- A 5 % for THP-AD digestate treatment, but remained stable by selective AnAOB retention using a vibrating screen. Overall, similar total nitrogen removal rates of 520 +/- A 28 mg N/L/day at a loading rate of 600 mg N/L/day were achieved in the THP-AD reactor compared to the conventional digestate treatment operating at low dissolved oxygen (DO) (0.38 +/- A 0.10 mg O-2/L). |
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000376456700033 |
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2016-02-19 |
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0175-7598; 1432-0614 |
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no |
Call Number |
UA @ admin @ c:irua:134166 |
Serial |
7755 |
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Author |
Zhang, Q.; De Clippeleir, H.; DeBarbadillo, C.; Su, C.; Al-Omari, A.; Wett, B.; Chandran, K.; Vlaeminck, S.E.; Murthy, S. |
Title |
Inhibition mechanisms affecting deammonification of dewatering filtrate from thermally hydrolyzed digested solid |
Type |
P3 Proceeding |
Year |
2016 |
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Pages |
9 p.
T2 - WEFTEC.16, 24 - 28 September 2016, New O |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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UA @ admin @ c:irua:151123 |
Serial |
8102 |
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Author |
Zhang, Q.; De Clippeleir, H.; Shaw, A.; DeBarbadillo, C.; Su, C.; Al-Omari, A.; Wett, B.; Chandran, K.; Vlaeminck, S.E.; Murthy, S. |
Title |
Mechanistic understanding of microbial activity inhibition : case study on sidestream deammonification for digester supernatant pretreated by thermal hydrolysis |
Type |
P3 Proceeding |
Year |
2016 |
Publication |
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Pages |
5 p.
T2 - WEF/IWA Nutrient Removal and Recovery Co |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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UA @ admin @ c:irua:151133 |
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8214 |
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Zhang, Q.; Higgins, M.J.; Vlaeminck, S.E.; DeBarbadillo, C.; Suzuki, R.; Kharkar, S.M.; Al-Omari, A.; Wett, B.; Chandran, K.; Murthy, S.; De Clippeleir, H. |
Title |
Minimizing recalcitrant organics and maximizing nitrogen removal linked to advanced biosolids processing at Blue Plains WWTP |
Type |
P3 Proceeding |
Year |
2017 |
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12 p.
T2 - IWA 2017 Conference on Sustainable Wast |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
Call Number |
UA @ admin @ c:irua:151107 |
Serial |
8252 |
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Author |
Zhang, Q.; De Clippeleir, H.; Al-Omari, A.; Wett, B.; Vlaeminck, S.E.; Murthy, S. |
Title |
Sidestream deammonification on thermal hydrolysis process digestate : strategies to overcome nitritation inhibition |
Type |
P3 Proceeding |
Year |
2015 |
Publication |
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11 p.
T2 - IWA Nutrient Removal and Recovery 2015: |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
Call Number |
UA @ admin @ c:irua:151147 |
Serial |
8522 |
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Author |
Zhang, Q.; Vlaeminck, S.E.; DeBarbadillo, C.; Suzuki, R.; Kharkar, S.M.; Al-Omari, A.; Wett, B.; Chandran, K.; Murthy, S.; De Clippeleir, H. |
Title |
Startup strategies of deammonification reactors treating reject water from thermally hydrolyzed solids |
Type |
P3 Proceeding |
Year |
2017 |
Publication |
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Pages |
5 p.
T2 - WEFTEC.17, 30 September 4 October 2017, |
Keywords |
P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Call Number |
UA @ admin @ c:irua:151113 |
Serial |
8579 |
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Author |
Zhang, Q.; Vlaeminck, S.E.; DeBarbadillo, C.; Su, C.; Al-Omari, A.; Wett, B.; Pümpel, T.; Shaw, A.; Chandran, K.; Murthy, S.; De Clippeleir, H. |
Title |
Supernatant organics from anaerobic digestion after thermal hydrolysis cause direct and/or diffusional activity loss for nitritation and anammox |
Type |
A1 Journal article |
Year |
2018 |
Publication |
Water research |
Abbreviated Journal |
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Volume |
143 |
Issue |
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Pages |
270-281 |
Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
Abstract |
Treatment of sewage sludge with a thermal hydrolysis process (THP) followed by anaerobic digestion (AD) enables to boost biogas production and minimize residual sludge volumes. However, the reject water can cause inhibition to aerobic and anoxic ammonium-oxidizing bacteria (AerAOB & AnAOB), the two key microbial groups involved in the deammonification process. Firstly, a detailed investigation elucidated the impact of different organic fractions present in THP-AD return liquor on AerAOB and AnAOB activity. For AnAOB, soluble compounds linked to THP conditions and AD performance caused the main inhibition. Direct inhibition by dissolved organics was also observed for AerAOB, but could be overcome by treating the filtrate with extended aerobic or anaerobic incubation or with activated carbon. AerAOB additionally suffered from particulate and colloidal organics limiting the diffusion of substrates. This was resolved by improving the dewatering process through an optimized flocculant polymer dose and/or addition of coagulant polymer to better capture the large colloidal fraction, especially in case of unstable AD performance. Secondly, a new inhibition model for AerAOB included diffusion-limiting compounds based on the porter-equation, and achieved the best fit with the experimental data, highlighting that AerAOB were highly sensitive to large colloids. Overall, this paper for the first time provides separate identification of organic fractions within THP-AD filtrate causing differential types of inhibition. Moreover, it highlights the combined effect of the performance of THP, AD and dewatering on the downstream autotrophic nitrogen removal kinetics. (C) 2018 Elsevier Ltd. All rights reserved. |
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000443664000027 |
Publication Date |
2018-06-18 |
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ISSN |
0043-1354; 1879-2448 |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:152911 |
Serial |
8623 |
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Author |
De Clippeleir, H.; Vlaeminck, S.E.; Courtens, E.N.P.; Jimenez, J.; Wadhawan, T.; Zhang, Q. |
Title |
Toward energy autarky : carbon redirection coupled with shortcut nitrogen processes |
Type |
H3 Book chapter |
Year |
2015 |
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129-150
T2 - Shortcut nitrogen removal : nitrite s |
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H3 Book chapter; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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978-1-57278-313-3 |
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UA @ admin @ c:irua:130470 |
Serial |
8676 |
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Author |
Cui, W.; Lin, W.; Lu, W.; Liu, C.; Gao, Z.; Ma, H.; Zhao, W.; Van Tendeloo, G.; Zhao, W.; Zhang, Q.; Sang, X. |
Title |
Direct observation of cation diffusion driven surface reconstruction at van der Waals gaps |
Type |
A1 Journal article |
Year |
2023 |
Publication |
Nature communications |
Abbreviated Journal |
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Volume |
14 |
Issue |
1 |
Pages |
554-10 |
Keywords |
A1 Journal article; Engineering sciences. Technology; Electron microscopy for materials research (EMAT) |
Abstract |
Weak interlayer van der Waals (vdW) bonding has significant impact on the surface/interface structure, electronic properties, and transport properties of vdW layered materials. Unraveling the complex atomistic dynamics and structural evolution at vdW surfaces is therefore critical for the design and synthesis of the next-generation vdW layered materials. Here, we show that Ge/Bi cation diffusion along the vdW gap in layered GeBi2Te4 (GBT) can be directly observed using in situ heating scanning transmission electron microscopy (STEM). The cation concentration variation during diffusion was correlated with the local Te-6 octahedron distortion based on a quantitative analysis of the atomic column intensity and position in time-elapsed STEM images. The in-plane cation diffusion leads to out-of-plane surface etching through complex structural evolutions involving the formation and propagation of a non-centrosymmetric GeTe2 triple layer surface reconstruction on fresh vdW surfaces, and GBT subsurface reconstruction from a septuple layer to a quintuple layer. Our results provide atomistic insight into the cation diffusion and surface reconstruction in vdW layered materials. Weak interlayer van der Waals (vdW) bonding has significant impact on the structure and properties of vdW layered materials. Here authors use in-situ aberration-corrected ADF-STEM for an atomistic insight into the cation diffusion in the vdW gaps and the etching of vdW surfaces at high temperatures. |
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001076227200001 |
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2023-02-02 |
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2041-1723 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
Impact Factor |
16.6 |
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Approved |
Most recent IF: 16.6; 2023 IF: 12.124 |
Call Number |
UA @ admin @ c:irua:201342 |
Serial |
9021 |
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