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Author | Smits, J.; Van Grieken, R. | ||||
Title | Chelating 2,2′-diaminodiethylamine cellulose filters and X-ray fluorescence for preconcentration and trace analysis of natural waters | Type | A1 Journal article | ||
Year | 1981 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 9 | Issue | 2 | Pages | 81-92 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | The 2,2′-diaminodiethylamine (DEN) functional group can be expected to have ideal properties for the chelation of transition metals and their collection from aqueous solutions, independent of the alkali and alkaline earth ions concentration. Introducing DEN into cellulose filters allows straightforward preconcentration of trace cations by a simple filtration step, and the DEN-filter constitutes a suitable target for X-ray fluorescence (XRF) analysis. The linearity between the XRF-response on the loaded DEN-filter and the trace cation concentration in the solution appears excellent, up to a total filter capacity of ca. 3 μeq.cm−2. The detection limits are around 0.5 μg. l−1 in most practical cases. Accuracy and precision are around 10%. The applicability of the proposed procedure is illustrated on a comparative basis by XRF-analysis of drinking water and surface water, after preconcentration by DEN-filtration and by alternative procedures. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | A1981LF48000001 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116571 | Serial | 7638 | ||
Permanent link to this record | |||||
Author | Chakravorty, R.; Van Grieken, R. | ||||
Title | Co-precipitation with iron hydroxide and X-ray fluorescence analysis of trace metals in water | Type | A1 Journal article | ||
Year | 1982 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 11 | Issue | 1 | Pages | 67-80 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Preconcentration of transition trace ions by coprecipitation on iron-hydroxide has been combined with energy-dispersive X-ray fluorescence for environmental water analysis. The optimized preconcentration procedure implies adding 2 mg of iron to a 200 ml water sample, adding dilute NaOH up to pH 9, filtering off on a Nuclepore membrane after a 1 h equilibration time, and analyzing. Quantitative recoveries could then be obtained for Ni, Cu, Zn and Pb, e.g. at the 10 μg/l level in waters of varying salinity while Mn was partially collected. (In fact, for a given problem the iron carrier amount can be adjusted to obtain a satisfactory compromise between high recovery and low detection limit). The precision is 7-8% at the 10 μg/l level, and the detection limits are in the 0.5-1 μg/l range. Various environmental water samples are analysed by way of illustration. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | A1982NG99200007 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116573 | Serial | 7676 | ||
Permanent link to this record | |||||
Author | Niessner, R.; Klockow, D.; Bruynseels, F.; Van Grieken, R. | ||||
Title | Investigation of heterogeneous reactions of PAH's on particle surfaces using laser microprobe mass analysis | Type | A1 Journal article | ||
Year | 1985 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 22 | Issue | 3/4 | Pages | 281-295 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Artificially generated NaCl particles were coated with PAH's by using a condensation technique. These particles were exposed to reactive gases like ozone, bromine and nitrogen dioxide. The original as well as the exposed particles were investigated by fluorimetric analysis and by LAMMA (Laser Microprobe Mass Analysis) in the desorption mode, which allows the evaporation and characterization of surfaces of single particles. The results are interpreted in terms of possible heterogeneous atmospheric reactions. The reactivity of the considered PAH's towards nitrogen dioxide was found to be negligible. The structure of the reaction products formed with ozone was partially elucidated. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | A1985AZE2300009 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116576 | Serial | 8124 | ||
Permanent link to this record | |||||
Author | Wouters, L.; Artaxo, P.; Van Grieken, R. | ||||
Title | Laser microprobe mass analysis of individual Antarctic aerosol particles | Type | A1 Journal article | ||
Year | 1990 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 38 | Issue | 3 | Pages | 427-438 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Individual Antarctic aerosol particles in the 0.54 μm aerodynamic diameter range were analyzed using laser microprobe mass analysis (LAMMA). As they were sampled near the ocean, the great majority consists of seasalt, transformed to various degrees in the atmosphere. Major alterations include the association of an excess sulfate and methane sulfonate with these particles. Sulfate-rich particles containing little or no chloride were found mostly in the smallest size fraction (0.51 μm), where they account for some 5% of all particles: they are most likely highly transformed seasalt. Aluminosilicates, on the other hand, only appear among the coarser particles: they represent 2% of the particulates in the 24 μm range. The remainder of the aerosol consists of organic, Fe-rich, K-rich and Zn-rich particles. The latter groups have very low abundances: always less than 1% of the population of the impactor stage(s) onto which they were collected. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | A1990CN56100011 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116580 | Serial | 8160 | ||
Permanent link to this record | |||||
Author | Eyckmans, K.; Zhang, J.; de Hoog, J.; Joos, P.; Van Grieken, R. | ||||
Title | Leaching of nutrients and trace metals from aerosol samples: a comparison between a re-circulation and an ultrasound system | Type | A1 Journal article | ||
Year | 2001 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 80 | Issue | 3 | Pages | 227-243 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000172385700006 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:36087 | Serial | 8167 | ||
Permanent link to this record | |||||
Author | Goossenaerts, C.; Van Grieken, R.; Jacob, W.; Witters, H.; Vanderborght, O. | ||||
Title | A microanalytical study of the gills of aluminium-exposed rainbow trout (Salmo gairdneri) | Type | A1 Journal article | ||
Year | 1988 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 34 | Issue | 3 | Pages | 227-237 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | |||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | A1988T017900005 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116579 | Serial | 8240 | ||
Permanent link to this record | |||||
Author | Eyckmans, K.; de Hoog, J.; van der Auwera, L.; Van Grieken, R. | ||||
Title | Speciation of aerosols by combining bulk ion chromatography and thin-window electron probe micro analysis | Type | A1 Journal article | ||
Year | 2003 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 83 | Issue | 9 | Pages | 777-786 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | |||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000184457600006 | Publication Date | 2004-05-02 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:43556 | Serial | 8571 | ||
Permanent link to this record | |||||
Author | Vanderborght, B.M.; Van Grieken, R.E. | ||||
Title | Trace metal analysis of water containing humic substances by X-ray fluorescence | Type | A1 Journal article | ||
Year | 1978 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 5 | Issue | 3 | Pages | 221-237 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Chelation by oxine followed by adsorption on activated carbon results in the efficient collection of many trace metal ions, independent of the trace metal concentration and of high alkali and alkaline earth ion abundances. Preconcentration factors around 10000 are often achieved. When this preconcentration procedure is combined with energy-dispersive X-ray fluorescence, accurate and precise analysis can be carried out, as was proven in several experiments. The technique can also be applied for the determination of divalent ions in natural waters containing up to 10 ppm of humic substances. Trivalent ions can quantitatively be collected from natural water provided suKicient activated carbon is added. Omitting the oxine chelation prior to the activated carbon adsorption step still results in collection of a sometimes important fraction of the trace metal ions from natural waters. This is related to organically bound or colloidal forms of the trace metals. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | A1978FR88000005 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:116570 | Serial | 8692 | ||
Permanent link to this record | |||||
Author | Semenov, M.Y.; Spolnik, Z.; Granina, L.; Van Grieken, R. | ||||
Title | Ultra-thin window electron probe microanalysis of suspended particles in tributaries of Lake Baikal, Siberia | Type | A1 Journal article | ||
Year | 2005 | Publication | International journal of environmental analytical chemistry | Abbreviated Journal | |
Volume | 85 | Issue | 6 | Pages | 377-386 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | |||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000229611800003 | Publication Date | 2007-07-07 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-7319 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:52360 | Serial | 8701 | ||
Permanent link to this record | |||||
Author | Van Dael, M.; Van Passel, S.; Pelkmans, L.; Guisson, R.; Reumermann, P.; Luzardo, N.M.; Witters, N.; Broeze, J. | ||||
Title | A techno-economic evaluation of a biomass energy conversion park | Type | A1 Journal article | ||
Year | 2013 | Publication | Applied Energy | Abbreviated Journal | Appl Energ |
Volume | 104 | Issue | Pages | 611-622 | |
Keywords | A1 Journal article; Engineering sciences. Technology; Engineering Management (ENM) | ||||
Abstract | Biomass as a renewable energy source has many advantages and is therefore recognized as one of the main renewable energy sources to be deployed in order to attain the target of 20% renewable energy use of final energy consumption by 2020 in Europe. In this paper the concept of a biomass Energy Conversion Park (ECP) is introduced. A biomass ECP can be defined as a synergetic, multi-dimensional biomass conversion site with a highly integrated set of conversion technologies in which a multitude of regionally available biomass (residue) sources are converted into energy and materials. A techno-economic assessment is performed on a case study in the Netherlands to illustrate the concept and to comparatively assess the highly integrated system with two mono-dimensional models. The three evaluated models consist of (1) digestion of the organic fraction of municipal solid waste, (2) co-digestion of manure and co-substrates, and (3) integration. From a socio-economic point of view it can be concluded that it is economically and energetically more interesting to invest in the integrated model than in two separate models. The integration is economically feasible and environmental benefits can be realized. For example, the integrated model allows the implementation of a co-digester. Unmanaged manure would otherwise represent a constant pollution risk. However, from an investor's standpoint one should firstly invest in the municipal solid waste digester since the net present value (NPV) of this mono-dimensional model is higher than that of the multi-dimensional model. A sensitivity analysis is performed to identify the most influencing parameters. Our results are of interest for companies involved in the conversion of biomass. The conclusions are useful for policy makers when deciding on policy instruments concerning manure processing or biogas production. (C) 2012 Elsevier Ltd. All rights reserved. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000316152700062 | Publication Date | 2012-12-25 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-2619 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 7.182 | Times cited | 45 | Open Access | |
Notes | ; We would like to thank the editor and the anonymous referees for their helpful suggestions and insightful comments that have significantly improved the paper. Furthermore, the authors gratefully acknowledge the financial support from INTERREG and the province of Limburg (Belgium). Also, we would like to thank all remaining partners of the ECP project (Eloi Schreurs, Dries Maes, Kristian Coppoolse, Han ten Berge, Bert Annevelink, Nathalie Devriendt, Erwin Cornelissen, Hannes Pieper, Pieter Vollaard, Jan Venselaar, and Hessel Abbink Spaink) for their support and contributions. Finally, we would like to express our gratitude towards the organization of the eighth International Conference on Renewable Resources and Biorefineries in Toulouse (France) for giving us the opportunity to present and thereby fine-tune our work. ; | Approved | Most recent IF: 7.182; 2013 IF: 5.261 | ||
Call Number | UA @ admin @ c:irua:127552 | Serial | 6145 | ||
Permanent link to this record | |||||
Author | Vasilakou, K.; Nimmegeers, P.; Thomassen, G.; Billen, P.; Van Passel, S. | ||||
Title | Assessing the future of second-generation bioethanol by 2030 : a techno-economic assessment integrating technology learning curves | Type | A1 Journal article | ||
Year | 2023 | Publication | Applied energy | Abbreviated Journal | |
Volume | 344 | Issue | Pages | 121263-15 | |
Keywords | A1 Journal article; Economics; Engineering sciences. Technology; Engineering Management (ENM); Intelligence in PRocesses, Advanced Catalysts and Solvents (iPRACS) | ||||
Abstract | Lignocellulosic biomass is the most abundant source of renewable biomass and is seen as a high-potential replacement for petroleum-based resources. The conversion technologies to advanced biofuels are still at a low maturity level, thus allowing for future cost reductions through technological learning. This fact is barely considered in state-of-the-art techno-economic assessments and a structured approach to account for technological learning in techno-economic assessments is needed. In this study, a framework for techno-economic assessments of advanced biofuels, integrating learning curves, is proposed. As a validation of this framework, the economic feasibility of the valorization of corn stover for the production of second-generation bioethanol in Belgium is studied. Process flowsheet simulations in Aspen Plus are developed, with an emphasis on the comparison of four different pretreatment technologies and two plant capacities at 156 dry kt biomass/y and 667 dry kt/y. The dilute acid pretreatment model of the large-scale biorefinery required the lowest minimum learning rate to reach an economically feasible biorefinery by 2030, being 3.9%, almost half as the one calculated for the smaller scale plant. This learning rate seems to be achievable based on learning rates commonly estimated in literature. We conclude that there is a potential for advanced ethanol production in Belgium under the current state of technology for large-scale biorefineries, which require additional biomass imports, when accounting for future cost reductions through learning | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 001007488700001 | Publication Date | 2023-05-22 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-2619 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 11.2 | Times cited | Open Access | ||
Notes | Approved | Most recent IF: 11.2; 2023 IF: 7.182 | |||
Call Number | UA @ admin @ c:irua:196509 | Serial | 9186 | ||
Permanent link to this record | |||||
Author | Snoeckx, R.; Bogaerts, A. | ||||
Title | Plasma technology – a novel solution for CO2conversion? | Type | A1 Journal article | ||
Year | 2017 | Publication | Chemical Society reviews | Abbreviated Journal | Chem Soc Rev |
Volume | 46 | Issue | 19 | Pages | 5805-5863 |
Keywords | A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
Abstract | CO2 conversion into value-added chemicals and fuels is considered as one of the great challenges of the 21st century. Due to the limitations of the traditional thermal approaches, several novel technologies are being developed. One promising approach in this field, which has received little attention to date, is plasma technology. Its advantages include mild operating conditions, easy upscaling, and gas activation by energetic electrons instead of heat. This allows thermodynamically difficult reactions, such as CO2 splitting and the dry reformation of methane, to occur with reasonable energy cost. In this review, after exploring the traditional thermal approaches, we have provided a brief overview of the fierce competition between various novel approaches in a quest to find the most effective and efficient CO2 conversion technology. This is needed to critically assess whether plasma technology can be successful in an already crowded arena. The following questions need to be answered in this regard: are there key advantages to using plasma technology over other novel approaches, and if so, what is the flip side to the use of this technology? Can plasma technology be successful on its own, or can synergies be achieved by combining it with other technologies? To answer these specific questions and to evaluate the potentials and limitations of plasma technology in general, this review presents the current state-of-the-art and a critical assessment of plasma-based CO2 conversion, as well as the future challenges for its practical implementation. |
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000412141600006 | Publication Date | 2017-08-21 | |
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Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0306-0012 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 38.618 | Times cited | 168 | Open Access | OpenAccess |
Notes | We would like to thank W. Wang (University of Antwerp) for providing the data on the thermal equilibrium conversions. Furthermore, we acknowledge financial support from the IAP/7 (Inter-university Attraction Pole) programme ‘PSI-Physical Chemistry of Plasma-Surface Interactions’ by the Belgian Federal Office for Science Policy (BELSPO), the Methusalem financing of the University of Antwerp, the Fund for Scientific Research Flanders (FWO; Grant no. G.0383.16N, G.0254.14N and G.0217.14N), the TOP research project of the Research Fund of the University of Antwerp (grant ID. 32249). | Approved | Most recent IF: 38.618 | ||
Call Number | PLASMANT @ plasmant @c:irua:145921 | Serial | 4709 | ||
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Author | Smondyrev, M.A.; Peeters, F.M.; Vansant, P.; Devreese, J.T. | ||||
Title | Exact equations for large bipolarons in the strong-coupling limit | Type | A1 Journal article | ||
Year | 1994 | Publication | Journal of physics: A: mathematical and general | Abbreviated Journal | |
Volume | 27 | Issue | Pages | 7925-7936 | |
Keywords | A1 Journal article; Condensed Matter Theory (CMT); Theory of quantum systems and complex systems | ||||
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Publisher | Place of Publication | London | Editor | ||
Language | Wos | A1994PW35300035 | Publication Date | 0000-00-00 | |
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ISSN ![]() |
0305-4470 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | 17 | Open Access | ||
Notes | Approved | no | |||
Call Number | UA @ lucian @ c:irua:9276 | Serial | 1106 | ||
Permanent link to this record | |||||
Author | Hellemans, K.; Vincke, A.; Cagno, S.; Herremans, D.; De Clercq, W.; Janssens, K. | ||||
Title | Composition and state of alteration of 18th-century glass finds found at the Cistercian nunnery of Clairefontaine, Belgium | Type | A1 Journal article | ||
Year | 2014 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 47 | Issue | Pages | 121-133 | |
Keywords | A1 Journal article; Philosophy; History; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | A hundred 18th-century glass fragments were recovered at the Clairefontaine monastery in the Belgian province of Luxembourg. They were analysed by a combination of SEM-EDX and LA-ICP-MS in order to determine their major composition as well as their trace element signature. Multivariate statistical methods such as hierarchical clustering and principal component analysis were used to divide the glass fragments into four main groups: potassium-rich glass, sodium-rich glass, potassium/lime-rich glass and high-lime-low-alkali glass. Within every group, not only a similarity in composition is observed, but also in colour, morphology and deterioration patterns. Potash glass fragments are the most abundant and show extensive deterioration; two classes of potash glass were identified: one similar to certain Central European glass compositions, while the other one, characterised by large variations in potash: lime ratio, may be attributed to local (regional) glass production. (C) 2014 Elsevier Ltd. All rights reserved. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000339037300012 | Publication Date | 2014-04-24 | |
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Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 12 | Open Access | |
Notes | ; Archaeological fieldwork at Clairefontaine was directed by Prof. Dr. J. De Meulemeester (dagger) and financed by the Walloon Government. Post-excavation research is carried out within the framework of the PhD-project (FNR Luxembourg BFR06-80): “The material culture of Clairefontaine abbey”. This investigation was supported by the Interuniversity Attraction Poles Programme (Belgian Science Policy – IUAP VI/16) and by the HERCULES foundation. This work was partly supported by the Research Council of Norway through its Centres of Excellence funding scheme, project number 223268/F50. ; | Approved | Most recent IF: 2.602; 2014 IF: 2.196 | ||
Call Number | UA @ admin @ c:irua:118711 | Serial | 5536 | ||
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Author | Cagno, S.; Cosyns, P.; Izmer, A.; Vanhaecke, F.; Nys, K.; Janssens, K. | ||||
Title | Deeply colored and black-appearing Roman glass : a continued research | Type | A1 Journal article | ||
Year | 2014 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 42 | Issue | Pages | 128-139 | |
Keywords | A1 Journal article; Philosophy; History; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | In the context of archaeological and historical assessment of Roman black-appearing glass, the chemical and physical characterization of a large collection of samples originating from various areas of the Roman Empire has been gathered over the past years to (i) verify whether a minor segment of the overall Roman glass production can help in determining possible diachronic changes in Roman imperial glass production (1st century AD – 5th century AD) and (ii) reveal regional compositional differences. In this paper, the latest results on the chemical composition of an additional 44 black-appearing Roman glass samples are presented, together with general conclusions based upon the entire compositional dataset of over 400 analyzed black glass samples. The results show that the Roman black glass is obtained through several glass compositions with a specific chronological, geographical and typological distribution. (C) 2013 Elsevier Ltd. All rights reserved. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000332133100011 | Publication Date | 2013-11-13 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 18 | Open Access | |
Notes | ; This research was supported by the Interuniversity Attraction Poles Programme – Belgian Science Policy (IUAP VI/16) and the Hercules fund, Brussels (grant A11/ 0387). The text also presents results of GOA “XANES meets ELNES” (Research Fund University of Antwerp, Belgium), FWO (Brussels, Belgium) projects no. G.0704.08 and G.01769.09, and VUB project OZR-BOF 1247. This work was partly supported by the Research Council of Norway through its Centres of Excellence funding scheme, project number 223268/F50. ; | Approved | Most recent IF: 2.602; 2014 IF: 2.196 | ||
Call Number | UA @ admin @ c:irua:115865 | Serial | 5567 | ||
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Author | Cagno, S.; Favaretto, L.; Mendera, M.; Izmer, A.; Vanhaecke, F.; Janssens, K. | ||||
Title | Evidence of early medieval soda ash glass in the archaeological site of San Genesio (Tuscany) | Type | A1 Journal article | ||
Year | 2012 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 39 | Issue | 5 | Pages | 1540-1552 |
Keywords | A1 Journal article; Philosophy; History; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | The early medieval period marks an important turning point in the history of glassmaking, since it comprises the transition period between the mineral-based silica-soda-lime glass of the Roman tradition and the plant ash-based glass. With the aim of expanding the knowledge on the glass recipes and technologies of this period, 37 glass samples were analyzed, originating from the archaeological excavations of San Genesio (Tuscany) and dated from the fourth to the eleventh century. The major and minor element concentrations were measured with SEM-EDX, while the trace elements were quantified with LA-ICP-MS. The results were compared with published compositions of glass samples of similar age in order to highlight differences and similarities. The results offer a very interesting view on the glass circulation in the religious/residential/manufacturing center of San Genesio in the early medieval period. Most of the glass has a typical late-Roman composition, but some glass fragments are identified as soda ash glass. These are among the earliest medieval ash-fluxed glasses ever found in the Italian peninsula. (C) 2011 Elsevier Ltd. All rights reserved. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000301620900034 | Publication Date | 2012-01-02 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 24 | Open Access | |
Notes | ; This research was supported by the Interuniversity Attraction Poles Programme – Belgian Science Policy (IUAP VI/16). The text also presents results of GOA “XANES meets ELNES” (Research Fund University of Antwerp, Belgium) and from FWO (Brussels, Belgium) projects no. G.0704.08 and G.01769.09. ; | Approved | Most recent IF: 2.602; 2012 IF: 1.889 | ||
Call Number | UA @ admin @ c:irua:98251 | Serial | 5618 | ||
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Author | Meulebroeck, W.; Cosyns, P.; Baert, K.; Wouters, H.; Cagno, S.; Janssens, K.; Terryn, H.; Nys, K.; Thienpont, H. | ||||
Title | Optical spectroscopy as a rapid and low-cost tool for the first-line analysis of glass artefacts : a step-by-step plan for Roman green glass | Type | A1 Journal article | ||
Year | 2011 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 38 | Issue | 9 | Pages | 2387-2398 |
Keywords | A1 Journal article; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Archaeometric research on glass artefacts is continuously evolving and is converging towards a multidisciplinary research domain where different types of techniques are applied depending on the questions asked and the circumstances involved. The technique described in this work is optical spectroscopy. The benefit of this technique being the possibility of building up a knowledge database for a large amount of material in a relatively short period of time and with a relatively limited budget. This is of particular interest for the investigation of extensive and/or unexplored glass collections where a first-line analysis of artefacts could facilitate the selection of material needing further and more detailed examination. This publication explores the extent to which optical spectroscopy can be used for a first-line analysis of green coloured glass artefacts from the Roman period. It is shown that the colour coordinates calculated from the measured transmission spectrum could reveal information about the fragment under study. In particular it is shown that 1) based on the position of the calculated colour values on the colour diagram (CIE1931) one could easily know whether the artefact was coloured using only iron or if copper oxides were also present. In the case of the artefact owing its colour solely to the presence of iron, the distance between the measured colour values and the colour diagrams white point can roughly indicate the iron concentration of the sample; 2) artefacts that were fabricated under similar furnace conditions can also be identified on the colour diagram; 3) samples with identical compositions and fabrication conditions but with different sample thickness, gave rise to a variation in the colour coordinates, thus allowing optical spectroscopy to help identify fragments which might belong to the same object. | ||||
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Publisher | Place of Publication | Editor | |||
Language | Wos | 000293551200037 | Publication Date | 2011-05-12 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 18 | Open Access | |
Notes | ; The authors would like to express their gratitude to the Vrije Universiteit Brussel for funding this research in the framework of HOA15, a “Horizontal Research Action” which encourages collaboration between research groups from different departments within the same University having expertise in specific research disciplines and also to the OZR-project 1247 BOF. The authors are also very grateful to the following persons for having permitted the study of their material: Rica Annaert and Sofie Vanhoutte of the “Vlaams lnstituut voor Onroerend Erfgoed (VIOE): Grobbendonk, Matagne-la-Petite, Oudenburg; Jean-Louis Antoine of the Musee Archeologique Namur: Nismes; Tom Debruyne of the ”Erfgoedcel“ Tienen: Tienen: Marc Rogge and Kurt Braeckman of the ”Provinciaal Archeologisch Museum (PAM)": Kruishoutem, Velzeke; Walter Sevenants: Rumst and Anne de Pyre-Gysel from the Musee Romain d'Avenches: Avenches. ; | Approved | Most recent IF: 2.602; 2011 IF: 1.914 | ||
Call Number | UA @ admin @ c:irua:92389 | Serial | 5756 | ||
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Author | Cagno, S.; Mendera, M.; Jeffries, T.; Janssens, K. | ||||
Title | Raw materials for medieval to post-medieval Tuscan glassmaking : new insight from LA-ICP-MS analyses | Type | A1 Journal article | ||
Year | 2010 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 37 | Issue | 12 | Pages | 3030-3036 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | LA-ICP-MS analyses were performed on a set of Tuscan (post) medieval archaeological glass finds dated to the 1316th century in order to quantitatively determine the trace element contents. The results are used for defining and distinguishing several compositional groups. The trace element data are consistent with the distinctions obtained by considering the major element data determined via quantitative SEM-EDX, but allow to obtain new insights into the nature and quality of the silica sources employed and the presumed method of ash purification. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000283903500008 | Publication Date | 2010-07-06 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 38 | Open Access | |
Notes | ; This research was supported by the Interuniversity Attraction Poles Program – Belgian Science Policy (IUAP VI/16). The text also presents results of GOA “Atom” (Research Fund University of Antwerp, Belgium) and of FWO (Brussels, Belgium) projects no. G.0177.03, G.0103.04 and G.0689.06. ; | Approved | Most recent IF: 2.602; 2010 IF: 1.710 | ||
Call Number | UA @ admin @ c:irua:85814 | Serial | 5802 | ||
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Author | Cagno, S.; Badano, M.B.; Mathis, F.; Strivay, D.; Janssens, K. | ||||
Title | Study of medieval glass fragments from Savona (Italy) and their relation with the glass produced in Altare | Type | A1 Journal article | ||
Year | 2012 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 39 | Issue | 7 | Pages | 2191-2197 |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Altare was in the medieval and post-medieval period an important glassmaking center in the Liguria region in Northern Italy. The first historical evidence of glassmaking in Altare is dated to the twelfth century. In spite of that, due to the continuity of glassmaking up to the present time and the contemporaneous intensive urbanization of the territory, no medieval glass from Altare or its immediate vicinity has been analyzed up to now. In this work, glass from archaeological excavations in the center of Savona, city with close ties with the glassmaking center, was studied. Glass fragments, dated from the tenth to the sixteenth century were selected from the collections of the Archaeological Museum in Savona and non-destructively analyzed with quantitative PIXE-PIGE. The resulting compositions, compared with known glass productions of the same time and evaluated on the basis of historical documents, offer an interesting panorama on the variety of glass circulation in Liguria. (C) 2012 Elsevier Ltd. All rights reserved. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000305849400027 | Publication Date | 2012-03-29 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | 21 | Open Access | |
Notes | ; This research was supported by the Interuniversity Attraction Poles Programme – Belgian Science Policy (IUAP VI/16). The text also presents results of GOA “XANES meets ELNES” (Research Fund University of Antwerp, Belgium) and from FWO (Brussels, Belgium) projects no. G.0704.08 and G.01769.09. The authors gratefully acknowledge Prof. Carlo Varaldo for allowing the study of the glass preserved in the Archaeological Museum of Savona. ; | Approved | Most recent IF: 2.602; 2012 IF: 1.889 | ||
Call Number | UA @ admin @ c:irua:100332 | Serial | 5849 | ||
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Author | Aerts, A.; Janssens, K.; Adams, F. | ||||
Title | Trace-level microanalysis of Roman glass from Khirbet Qumran, Israel | Type | A1 Journal article | ||
Year | 1999 | Publication | Journal of archaeological science | Abbreviated Journal | J Archaeol Sci |
Volume | 26 | Issue | Pages | 883-891 | |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | |||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000082470800005 | Publication Date | 2002-09-17 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-4403 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.602 | Times cited | Open Access | ||
Notes | Approved | Most recent IF: 2.602; 1999 IF: NA | |||
Call Number | UA @ admin @ c:irua:25299 | Serial | 5881 | ||
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Author | Fedina, L.; Lebedev, O.I.; Van Tendeloo, G.; van Landuyt, J. | ||||
Title | In-situ HREM irradiation study of point defect clustering in strained GexSi1-x/(001)Si heterostructure | Type | A1 Journal article | ||
Year | 1997 | Publication | Conference series of the Institute of Physics | Abbreviated Journal | |
Volume | 157 | Issue | Pages | 55-58 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | |||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | London | Editor | ||
Language | Wos | 000071954600008 | Publication Date | 0000-00-00 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-2346 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | 1 | Open Access | ||
Notes | Approved | Most recent IF: NA | |||
Call Number | UA @ lucian @ c:irua:21432 | Serial | 1578 | ||
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Author | Stuer, C.; van Landuyt, J.; Bender, H.; Rooyackers, R.; Badenes, G. | ||||
Title | Morphology and defects in shallow trench isolation structures | Type | A1 Journal article | ||
Year | 1999 | Publication | Conference series of the Institute of Physics | Abbreviated Journal | |
Volume | 164 | Issue | Pages | 443-446 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | |||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | London | Editor | ||
Language | Wos | 000166835300094 | Publication Date | 0000-00-00 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-2346 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | Times cited | 1 | Open Access | ||
Notes | Approved | Most recent IF: NA | |||
Call Number | UA @ lucian @ c:irua:29690 | Serial | 2206 | ||
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Author | Fedina, L.; Gutakovskii, A.; Aseev, A.; van Landuyt, J.; Vanhellemont, J. | ||||
Title | New intermediate defect configuration in Si studied by in situ HREM irradiation | Type | A1 Journal article | ||
Year | 1997 | Publication | Conference series of the Institute of Physics | Abbreviated Journal | |
Volume | 157 | Issue | Pages | 43-46 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | |||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | London | Editor | ||
Language | Wos | 000071954600006 | Publication Date | 0000-00-00 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-2346 | ISBN | Additional Links | UA library record; WoS full record; | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | Most recent IF: NA | |||
Call Number | UA @ lucian @ c:irua:21428 | Serial | 2318 | ||
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Author | Vanhellemont, J.; Bender, H.; van Landuyt, J. | ||||
Title | TEM studies of processed Si device materials | Type | A1 Journal article | ||
Year | 1997 | Publication | Conference series of the Institute of Physics | Abbreviated Journal | |
Volume | 157 | Issue | Pages | 393-402 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | Recent developments in the field of TEM characterisation of Si device materials are discussed and illustrated by a few case studies of material in different stages of various kinds of processing. Important challenges are the ever decreasing defect densities and device feature sizes. Defect delineation techniques using large area inspection tools yielding accurate coordinates of the defects to be studied have therefore become an essential part of the TEM analysis procedure. The possibility to transfer these defect coordinates without loss of accuracy to tools for local TEM specimen preparation is also a conditio sine qua non for a successful analysis. Insitu TEM remains important as dynamic processes can be observed and analysed under well defined experimental conditions. As case studies illustrating new developments, results are presented on defects in as-grown Ct silicon, on in-situ studies in processed silicon, on problem sites in advanced integrated circuit structures and on assessment of localised strain fields in the nm size scale. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | London | Editor | ||
Language | Wos | 000071954600079 | Publication Date | 0000-00-00 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-2346 | ISBN | Additional Links | UA library record; WoS full record; | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | Most recent IF: NA | |||
Call Number | UA @ lucian @ c:irua:21430 | Serial | 3486 | ||
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Author | Vincze, L.; Janssens, K.; Adams, F. | ||||
Title | X-ray optics for synchrotron-radiation-induced X-ray micro fluorescence at the european synchrotron-radiation facility, Grenoble | Type | A1 Journal article | ||
Year | 1993 | Publication | Institute of physics conference series | Abbreviated Journal | |
Volume | Issue | 130 | Pages | 613-616 | |
Keywords | A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) | ||||
Abstract | Different optical designs for generating synchrotron x-ray micro beams suitable for use in an X-ray fluorescence microscope using an ESRF bending magnet X-ray source are compared. Attention is devoted to the spatial and energy distribution of the photons in the micro beam and to the minimum detection limits that are achievable with each alternative optical system. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | A1993LW34000126 | Publication Date | ||
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-2346 | ISBN | Additional Links | UA library record; WoS full record | |
Impact Factor | Times cited | Open Access | |||
Notes | Approved | no | |||
Call Number | UA @ admin @ c:irua:104541 | Serial | 5917 | ||
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Author | Vanmeert, M.; Razzokov, J.; Mirza, M.U.; Weeks, S.D.; Schepers, G.; Bogaerts, A.; Rozenski, J.; Froeyen, M.; Herdewijn, P.; Pinheiro, V.B.; Lescrinier, E. | ||||
Title | Rational design of an XNA ligase through docking of unbound nucleic acids to toroidal proteins | Type | A1 Journal article | ||
Year | 2019 | Publication | Nucleic acids research | Abbreviated Journal | Nucleic Acids Res |
Volume | 47 | Issue | 13 | Pages | 7130-7142 |
Keywords | A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) | ||||
Abstract | Xenobiotic nucleic acids (XNA) are nucleic acid analogues not present in nature that can be used for the storage of genetic information. In vivo XNA applications could be developed into novel biocontainment strategies, but are currently limited by the challenge of developing XNA processing enzymes such as polymerases, ligases and nucleases. Here, we present a structure-guided modelling-based strategy for the rational design of those enzymes essential for the development of XNA molecular biology. Docking of protein domains to unbound double-stranded nucleic acids is used to generate a first approximation of the extensive interaction of nucleic acid processing enzymes with their substrate. Molecular dynamics is used to optimise that prediction allowing, for the first time, the accurate prediction of how proteins that form toroidal complexes with nucleic acids interact with their substrate. Using the Chlorella virus DNA ligase as a proof of principle, we recapitulate the ligase's substrate specificity and successfully predict how to convert it into an XNA-templated XNA ligase. | ||||
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Corporate Author | Thesis | ||||
Publisher | Place of Publication | Editor | |||
Language | Wos | 000490556600047 | Publication Date | 2019-07-26 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0305-1048 | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 10.162 | Times cited | 1 | Open Access | |
Notes | European Research Council, FP7/2007-2013 ERC-2012-ADG 20120216/320683 ; KU Leuven, OT/14/128 ; Biotechnology and Biosciences Research Council, BB/N01023X/1 BB/N010221/1 ; Authors are grateful to Prof. Dr A.M.J.J. (Alexandre) Bonvin from the University of Utrecht and the WeNMR institute for his expert contribution. We have greatly benefited from discussions and help from numerous postdocs over the years (in particular, Dr E. Groaz, Dr E. Eremeeva, Dr J. Masschelein, Dr S. Xiaoping and Dr M. Renders) as well as graduate student D. Kestemont and undergraduate student M. Abdel Fattah Ismail. We express our gratitude to L. Margamuljana for helpful discussions and excellent technical assistance on in vitro experiments. | Approved | Most recent IF: 10.162 | ||
Call Number | PLASMANT @ plasmant @c:irua:162105 | Serial | 5359 | ||
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Author | Van Tendeloo, G.; Lebedev, O.I.; Amelinckx, S. | ||||
Title | Atomic and microstructure of CMR materials | Type | A1 Journal article | ||
Year | 2000 | Publication | Journal of magnetism and magnetic materials | Abbreviated Journal | J Magn Magn Mater |
Volume | 211 | Issue | Pages | 73-83 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | |||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | Amsterdam | Editor | ||
Language | Wos | 000085772100013 | Publication Date | 2002-07-25 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0304-8853; | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.63 | Times cited | 48 | Open Access | |
Notes | Iuap 4-10 | Approved | Most recent IF: 2.63; 2000 IF: 0.996 | ||
Call Number | UA @ lucian @ c:irua:54773 | Serial | 165 | ||
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Author | Khazzan, S.; Bessais, L.; Van Tendeloo, G.; Mliki, N. | ||||
Title | Correlation between the nanocrystalline Sm(Fe,Mo)12 and its out of equilibrium phase Sm(Fe,Mo)10 | Type | A1 Journal article | ||
Year | 2014 | Publication | Journal of magnetism and magnetic materials | Abbreviated Journal | J Magn Magn Mater |
Volume | 363 | Issue | Pages | 125-132 | |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | Nanostructured Sm-Fe-Mo semi-hard magnetic material exhibiting enhanced magnetic properties can be produced by ball milling followed by recrystallization. Milled samples were annealed for 30 min in a vacuum at different temperatures (T-A) between 700 and 1190 degrees C. The effects of heat treatment and Mo content on structural and magnetic property changes have been investigated by means of X-ray diffraction using the Rietvekl method, transmission electron microscopy and magnetic measurements. For samples annealed at T-A > 900 degrees C the tetragonal ThMn12-type structure is identified, while for 700 < T-A < 900 degrees C a new out of equilibrium P6/mmm type structure was found as the major phase. This novel nanocrystalline phase has never been synthesized before. The correspondent stoichiometry is determined on the basis of the vacancy model. The Rietveld analysis gives a stoichiometry ratio equal to 1:10, for the out of equilibrium hexagonal phase, which is described with three crystallographic transition metal sites: 3g is fully occupied, 61 occupation is limited to hexagons surrounding the Fe dumbbell pairs 2e. We have performed a magnetic and structural study of nanocrystalline metastable P6/mrnm Sm(Fe1-xMo)(10), correlated with structural transformation towards its equilibrium derivative 14/mrnm Sm(Fe1-xMo)(12). A maximum of the coercive field H-C (H-C > 5 kOe) has been observed for the new hexagonal P6/rnmm phase suggesting that nanocrystalline Sm(Fe,Mo)(10), is a semi hard material, and is potential candidate for magnetic recording. (C) 2014 Elsevier B.V. All rights reserved. | ||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | Amsterdam | Editor | ||
Language | Wos | 000335393900021 | Publication Date | 2014-04-05 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0304-8853; | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.63 | Times cited | 6 | Open Access | |
Notes | Approved | Most recent IF: 2.63; 2014 IF: 1.970 | |||
Call Number | UA @ lucian @ c:irua:117139 | Serial | 524 | ||
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Author | Angelakeris, M.; Li, Z.A.; Hilgendorff, M.; Simeonidis, K.; Sakellari, D.; Filippousi, M.; Tian, H.; Van Tendeloo, G.; Spasova, M.; Acet, M.; Farle, M. | ||||
Title | Enhanced biomedical heat-triggered carriers via nanomagnetism tuning in ferrite-based nanoparticles | Type | A1 Journal article | ||
Year | 2015 | Publication | Journal of magnetism and magnetic materials | Abbreviated Journal | J Magn Magn Mater |
Volume | 381 | Issue | 381 | Pages | 179-187 |
Keywords | A1 Journal article; Electron microscopy for materials research (EMAT) | ||||
Abstract | Biomedical nanomagnetic carriers are getting a higher impact in therapy and diagnosis schemes while their constraints and prerequisites are more and more successfully confronted. Such particles should possess a well-defined size with minimum agglomeration and they should be synthesized in a facile and reproducible high-yield way together with a controllable response to an applied static or dynamic field tailored for the specific application. Here, we attempt to enhance the heating efficiency in magnetic particle hyperthermia treatment through the proper adjustment of the core-shell morphology in ferrite particles, by controlling exchange and dipolar magnetic interactions at the nanoscale. Thus, core-shell nanoparticles with mutual coupling of magnetically hard (CoFe2O4) and soft (MnFe2O4) components are synthesized with facile synthetic controls resulting in uniform size and shell thickness as evidenced by high resolution transmission electron microscopy imaging, excellent crystallinity and size monodispersity. Such a magnetic coupling enables the fine tuning of magnetic anisotropy and magnetic interactions without sparing the good structural, chemical and colloidal stability. Consequently, the magnetic heating efficiency of CoFe2O4. and MnFe2O4 core-shell nanoparticles is distinctively different horn that of their counterparts, even though all these nanocrystals were synthesized under similar conditions. For better understanding of the AC magnetic hyperthermia response and its correlation with magnetic-origin features we study the effect of the volume ratio of magnetic hard and soft phases in the bimagnetic core-shell nanocrystals. Eventually, such particles may be considered as novel heating carriers that under further biomedical functionalization may become adaptable multifunctional heat-triggered nanoplatforms. (C) 2014 Elsevier B.V. All rights reserved. | ||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | Amsterdam | Editor | ||
Language | Wos | 000349361100027 | Publication Date | 2014-12-29 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0304-8853; | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.63 | Times cited | 20 | Open Access | |
Notes | 312483 Esteem2; Esteem2_ta | Approved | Most recent IF: 2.63; 2015 IF: 1.970 | ||
Call Number | c:irua:125284 c:irua:125284 | Serial | 1049 | ||
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Author | Freire, J.A.K.; Matulis, A.; Peeters, F.M.; Freire, V.N.; Farias, G.A. | ||||
Title | Exciton trapping in a hybrid ferromagnetic/semiconductor magnetic antidot | Type | A1 Journal article | ||
Year | 2001 | Publication | Journal of magnetism and magnetic materials | Abbreviated Journal | J Magn Magn Mater |
Volume | 226/230 | Issue | Pages | 2038-2039 | |
Keywords | A1 Journal article; Condensed Matter Theory (CMT) | ||||
Abstract | |||||
Address | |||||
Corporate Author | Thesis | ||||
Publisher | Place of Publication | Amsterdam | Editor | ||
Language | Wos | 000170628400349 | Publication Date | 2002-07-25 | |
Series Editor | Series Title | Abbreviated Series Title | |||
Series Volume | Series Issue | Edition | |||
ISSN ![]() |
0304-8853; | ISBN | Additional Links | UA library record; WoS full record; WoS citing articles | |
Impact Factor | 2.63 | Times cited | 2 | Open Access | |
Notes | Approved | Most recent IF: 2.63; 2001 IF: 1.329 | |||
Call Number | UA @ lucian @ c:irua:37314 | Serial | 1119 | ||
Permanent link to this record |