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Author |
Alejo, D.; Morales, M.C.; de la Torre, J.B.; Grau, R.; Bencs, L.; Van Grieken, R.; van Espen, P.; Sosa, D.; Nuñez, V. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Seasonal trends of atmospheric nitrogen dioxide and sulfur dioxide over North Santa Clara, Cuba |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Environmental monitoring and assessment |
Abbreviated Journal |
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Volume |
185 |
Issue |
7 |
Pages |
6023-6033 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Atmospheric nitrogen dioxide (NO2) and sulfur dioxide (SO2) levels were monitored simultaneously by means of Radiello passive samplers at six sites of Santa Clara city, Cuba, in the cold and the warm seasons in 2010. The dissolved ionic forms of NO2 and SO2 as nitrate and sulfite plus sulfate, respectively, were determined by means of ion chromatography. Analysis of NO2 as nitrite was also performed by UVVis spectrophotometry. For NO2, significant t tests show good agreement between the results of IC and UVVis methods. The NO2 and SO2 concentrations peaked in the cold season, while their minimum levels were experienced in the warm season. The pollutant levels do not exceed the maximum allowable limit of the Cuban Standard 39:1999, i.e., 40 μg/m3 and 50 μg/m3 for NO2 and SO2, respectively. The lowest pollutant concentrations obtained in the warm season can be attributed to an increase in their removal via precipitation (scavenging) while to the decreased traffic density and industrial emission during the summer holidays (e.g., July and August). |
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Wos |
000319753600053 |
Publication Date |
2012-12-03 |
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1420-2026; 1573-2967 |
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UA @ admin @ c:irua:107293 |
Serial |
8501 |
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Author |
Reniers, G.L.L.; Sörensen, K.; Vrancken, K. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Editorial introduction |
Type |
H1 Book chapter |
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Year |
2013 |
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Pages |
1-6
T2 - Management principles of sustainable indu |
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Keywords |
H1 Book chapter; Engineering Management (ENM); Sustainable Energy, Air and Water Technology (DuEL) |
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9783527649488 |
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UA @ admin @ c:irua:107601 |
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7833 |
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Author |
Reniers, G.L.L.; Sörensen, K.; Vrancken, K. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Conclusions and recommendations |
Type |
H1 Book chapter |
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Year |
2013 |
Publication |
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Pages |
265-268
T2 - Management principles of sustainable |
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H1 Book chapter; Engineering Management (ENM); Sustainable Energy, Air and Water Technology (DuEL) |
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9783527649488 |
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Call Number |
UA @ admin @ c:irua:107610 |
Serial |
7723 |
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Author |
De Vis, K.; Jembrih-Simbürger, D.; Schalm, O.; Schreiner, M.; Caen, J. |
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Title |
Einfluss verschiedener Silbersalze auf die Farbintensität von Silbergelb : analytische Untersuchungen |
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A2 Journal article |
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Year |
2002 |
Publication |
Zeitschrift für Kunsttechnologie und Konservierung |
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Volume |
16 |
Issue |
1 |
Pages |
147-157 |
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Keywords |
A2 Journal article; Art; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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ISSN |
0931-7198 |
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Call Number |
UA @ admin @ c:irua:107748 |
Serial |
7855 |
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Author |
Jabłoński, M.B.; Stefaniak, E.A.; Darchuk, L.; Turzańska, K.; Gorzelak, M.; Kuduk, R.; Dorriné, W.; Van Grieken, R. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Microchemical investigation of bone derived from mice treated with strontium in different chemical forms using scanning electron microscopy and micro-Raman spectroscopy |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Microchemical journal |
Abbreviated Journal |
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Volume |
108 |
Issue |
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Pages |
168-173 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
We used SEM/EDX and micro-Raman spectroscopy to investigate the chemical changes (both on the level of elementary and molecular composition) of mice bones when strontium is incorporated in their microstructure after being administered in the form of two salts: chloride and ranelate. Strontium accumulated mainly in vicinity of bone edges, both cortical and close to bone marrow. The distribution of other elements comprising bone samples (Ca, P, Mg, K etc.) was also determined by energy-dispersive X-ray analysis (EDX). The area adjacent to a cortical bone edge with accumulated strontium has presented modified Raman spectral profiles. Besides most of the Raman bands typical for both mineral (hydroxyapatite with carbonate substitution type B) and organic phases of a bone, we observed a Raman band at 811 cm− 1. It was detected regularly in the sample with high strontium concentration. |
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Wos |
000316427100027 |
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2012-10-25 |
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0026-265x; 0026-265x |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:107882 |
Serial |
8246 |
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Author |
Bencs, L.; Horemans, B.; Van Grieken, R.; et al. |
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Title |
Atmospheric deposition fluxes to the Belgian marine waters originating from ship emissions : SHIPFLUX : final report |
Type |
Minutes and reports |
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Year |
2012 |
Publication |
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Abbreviated Journal |
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Keywords |
Minutes and reports; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:107883 |
Serial |
7524 |
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Author |
Mmari, A.G.; Potgieter-Vermaak, S.S.; Bencs, L.; McCrindle, R.I.; Van Grieken, R. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Elemental and ionic components of atmospheric aerosols and associated gaseous pollutants in and near Dar es Salaam, Tanzania |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Atmospheric environment : an international journal |
Abbreviated Journal |
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Volume |
77 |
Issue |
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Pages |
51-61 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Elemental and water-soluble ionic compounds (WSICs) of atmospheric aerosols (total suspended particulate TSP) and some gaseous pollutants (SO2, NO2 and O3) from a coastal, semi-urban and rural site in and near Dar es Salaam, Tanzania were investigated during dry and wet seasons of January 2005November 2007. Na+, Ca2+, SO42−, NO3− and Cl− made up the dominant fraction of WSICs during the dry season with average concentrations ranging from non-detectable (n.d.)5.4, 0.262.6, 0.7414.7, 0.41.5 and 1.13.4 μg m−3, respectively, while in the wet season, from n.d. up to 1.7, 1.2, 4.4, 2.1 and 3.0 μg m−3, respectively. The total air concentrations of the detected elements (Al, Si, S, Cl, K, Ca, Fe and Zn) showed seasonal and site-specific variation in the range of 7.526.6 with an average of 14.5 μg m−3. Most of the air concentrations of pollutants were observed to decrease with increasing distance from the coastal site, which is under urban and industrial pollutant emissions. Sulphur and nitrogen oxidation ratios during the dry season ranged from 0.08 to 0.91 and 0.013 to 0.049, respectively, while they were between 0.090.65 and 0.0020.095, respectively, in the wet season. These values indicate the photochemical oxidation of SO2 and a high extent of NO3−formation in the atmosphere. Neutralization ratios revealed the presence of acidic SO42− and NO3− aerosols. Principal component analysis identified sea spray, local combustion, vehicular traffic, biomass burning and re-suspended road dust as dominant sources of aerosols at the studied coastal and semi-urban sites. However, at the rural site, besides sea spray, crustal sources, soil dust re-suspension and long-range transport are the possible origins of suspended particulates. |
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000324848500006 |
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2013-05-01 |
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ISSN |
1352-2310 |
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Call Number |
UA @ admin @ c:irua:108096 |
Serial |
7882 |
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Author |
Vázquez, C.; Darchuk, L.; Stefaniak, E.A.; Van Grieken, R.; Palacios, O.R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Compositional correlation between pigments found in excavations and on human bones investigated with micro-raman spectrometry and scanning electron microscopy |
Type |
H2 Book chapter |
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Year |
2011 |
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Abbreviated Journal |
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Pages |
13-18
T2 - Integration of nuclear spectrometry met |
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Keywords |
H2 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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978-92-0-121310-5 |
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Call Number |
UA @ admin @ c:irua:108205 |
Serial |
7716 |
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Author |
Caratelli, D.; Gielis, J.; Tavkhelidze, I.; Ricci, P.E. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
The Dirichlet problem for the Laplace equation in supershaped annuli |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Boundary value problems |
Abbreviated Journal |
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Pages |
113-10 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Abstract |
The Dirichlet problem for the Laplace equation in normal-polar annuli is addressed by using a suitable Fourier-like technique. Attention is in particular focused on the wide class of domains whose boundaries are defined by the so-called superformula introduced by Gielis. A dedicated numerical procedure based on the computer algebra system Mathematica© is developed in order to validate the proposed methodology. In this way, highly accurate approximations of the solution, featuring properties similar to the classical ones, are obtained. |
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000325760900002&DestLinkType=CitingArticles&DestApp=ALL_WOS&UsrCustomerID=ef845e08c439e550330acc77c7 |
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2013-05-03 |
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1687-2762; 1687-2770 |
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UA library record; WoS citing articles; WoS full record |
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UA @ admin @ c:irua:108644 |
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7812 |
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Author |
Van Wesenbeeck, K.; Hauchecorne, B.; Lenaerts, S. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Integration of a photocatalytic coating in a corona discharge unit for plasma assisted catalysis |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Journal of environmental solutions |
Abbreviated Journal |
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Volume |
2 |
Issue |
1 |
Pages |
16-24 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Abstract |
The combination of a non-thermal plasma with catalysis is considered as a sustainable indoor air purification technology to achieve complete oxidation at reduced energy cost with a longer electrode lifetime. An optimal window of operation for plasma assisted catalysis is found by varying the polarity, the applied voltage, the relative humidity of the gas phase and the configuration of the plasma reactor. The results show that, in general, negative corona discharge can obtain higher nitric oxide (NO) conversion efficiencies compared to positive corona. It is also clear that at higher applied voltages, higher conversion efficiency can be reached. The effect of relative humidity, however, is not found to be significant in the range (0 20.3 %) tested in this work. Additionally, the configuration of the plasma reactor is changed by varying the amount of pins that are attached at the collector electrode. The results show that there is an optimum at 10 pairs of pins to obtain a high conversion efficiency of NO. By applying a coating on the collector electrode of the plasma reactor, it is possible to see the influence of the coating on the performance of the plasma system, which was operating in the previously found optimal window. It stands clear that the use of a plasma assisted catalysis system has high potential as an integrated and sustainable indoor air purification technology. |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:108646 |
Serial |
5966 |
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Author |
Caratelli, D.; Gielis, J.; Ricci, P.E.; Tavkhelidze, I. |
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Title |
Some properties of “bulky” links, generated by Generalized Möbius Listing's bodies GML4n |
Type |
P3 Proceeding |
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Year |
2013 |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Call Number |
UA @ admin @ c:irua:108672 |
Serial |
8555 |
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Author |
Van Grieken, R. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Editorial : introducing Dr Markowicz as X-Ray Spectrometry's new associate editor for Europe |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
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Volume |
42 |
Issue |
4 |
Pages |
175 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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000320727900001 |
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2013-06-20 |
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0049-8246 |
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UA @ admin @ c:irua:108738 |
Serial |
7832 |
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Author |
Smits, M. |
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Title |
Photocatalytic degradation of diesel soot : from application to reaction mechanism |
Type |
Doctoral thesis |
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Year |
2013 |
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Abbreviated Journal |
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Pages |
160 p. |
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Keywords |
Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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978-90-5728-415-1 |
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no |
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UA @ admin @ c:irua:108803 |
Serial |
8380 |
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Author |
Alföldy, B.; Lööv, J.B.; Lagler, F.; Bencs, L.; Horemans, B.; Van Grieken, R.; et al. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Measurements of air pollution emission factors for marine transportation in SECA |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Atmospheric measurement techniques |
Abbreviated Journal |
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Volume |
6 |
Issue |
7 |
Pages |
1777-1791 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
The chemical composition of the plumes of seagoing ships was measured during a two week long measurement campaign in the port of Rotterdam, Hoek van Holland The Netherlands, in September 2009. Altogether, 497 ships were monitored and a statistical evaluation of emission factors (g kg−1 fuel) was provided. The concerned main atmospheric components were SO2, NO2, NOx and the aerosol particle number. In addition, the elemental and water-soluble ionic composition of the emitted particulate matter was determined. Emission factors were expressed as a function of ship type, power and crankshaft rotational speed. The average SO2 emission factor was found to be roughly half of what is allowed in sulphur emission control areas (16 vs. 30 g kg−1 fuel), and exceedances of this limit were rarely registered. A significant linear relationship was observed between the SO2 and particle number emission factors. The intercept of the regression line, 4.8 × 1015 (kg fuel)−1, gives the average number of particles formed during the burning of 1 kg zero sulphur content fuel, while the slope, 2 × 1018, provides the average number of particles formed with 1 kg sulphur burnt with the fuel. Water-soluble ionic composition analysis of the aerosol samples from the plumes showed that ~144 g of particulate sulphate was emitted from 1 kg sulphur burnt with the fuel. The mass median diameter of sulphate particles estimated from the measurements was ~42 nm. |
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000322546800014 |
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2013-07-24 |
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1867-1381; 1867-8548 |
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Call Number |
UA @ admin @ c:irua:109265 |
Serial |
8211 |
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Author |
Potgieter-Vermaak, S.; Van Grieken, R.; Potgieter, J.H. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Integrated analytical techniques for analysing individual environmental particles |
Type |
H2 Book chapter |
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Year |
2012 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
123-141
T2 - Spectroscopic properties of inorganic |
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Keywords |
H2 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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ISBN |
978-1-84973-395-3 |
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no |
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Call Number |
UA @ admin @ c:irua:109314 |
Serial |
8108 |
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Author |
Margui, E.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
State-of-the-art X-ray fluorescence instrumentation for chemical analysis |
Type |
A3 Journal article |
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Year |
2013 |
Publication |
Petro Industry News |
Abbreviated Journal |
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Volume |
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Issue |
June/July |
Pages |
16-18 |
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Keywords |
A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Nowadays, X-ray fluorescence spectrometry (XRF) is a well-established analytical technique for qualitative and quantitative elemental analysis (sometimes from Be to U) of a wide variety of samples. In particular, the truly multi-element character, acceptable speed and economy, ease of automation and the possibility to directly analyse solid samples are the most important features among the many that have made it a very mature analytical tool for routine quality controls in many industries, as well as for analytical support for the research laboratory.e recent technological advances, including the design of low-power micro-focus tubes and the novel X-ray optics and detectors have made it possible to extend XRF to the determination of low-Z elements and to obtain 2D or 3D information on a micrometre-scale. Furthermore, the recent development and commercialisation of benchtop and portable instrumentation, that offer extreme simplicity of operation in a low-cost design, have promoted even more the approach of XRF for many analytical problems.is article highlights this state-of-the art technique with regards to currently available XRF instrumentation on the market as well as recent applications in environmental and industrial fields. |
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ISSN |
1472-0590 |
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no |
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Call Number |
UA @ admin @ c:irua:109342 |
Serial |
8581 |
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Author |
Blust, R.J.P.; Dardenne, F.; De Wael, K.; Nagels, L.; Van Camp, G. |
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Title |
Electrochemical aptasensors with a gelatin B matrix : EP13175128 |
Type |
Patent |
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Year |
2013 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Patent; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
An aptamer-based electrochemical sensor, wherein said aptamer is covalently bonded to or chemisorbed on an electrode, said aptamer forming a robust complex with a target molecule and is encapsulated by a gelatin B matrix; a method of manufacturing an aptamer-based electrochemical sensor for determining a concentration of a target molecule comprising the steps of: selecting an aptamer to form a robust complex with a target molecule using the SELEX procedure; synthesizing said aptamer; adsorbing said aptamer on or covalently coupling said aptamer with an electrode; and providing a gelatin B matrix for said aptamer on said electrode thereby realising said aptamer-based potentiometric or amperometric sensor; and the use of the aptamer-based electrochemical sensor produced according to the above method for the electrochemical determination of a concentration of 15 the target molecule. |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:109364 |
Serial |
5587 |
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Permanent link to this record |
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Author |
Palacios, O.M.; van Meel, K.; Van Grieken, R.; Marcó P., L.-M.; Vázquez, C. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Characterization of black volcanites from the Limay river basin, Patagonia, Argentina, using energy dispersive X-ray fluorescence spectrometry : an aid to infer human group mobility |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Journal of radioanalytical and nuclear chemistry |
Abbreviated Journal |
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Volume |
298 |
Issue |
2 |
Pages |
1245-1255 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
The investigation of hunter-gatherers archaeological sites in the Limay river basin, Patagonia, Argentina, raised questions concerning the lithic technology. The chemical characterization of artifacts, rocks and possible sources of provenances could help to elucidate the hunter-gatherer mobility. In three archaeological sitesRincón Chico 2 (RCh2/87; 14C 710 ± 60 BP), Cueva Traful I (CTI; 14C 9430 ± 230 BP) and Casa de Piedra de Ortega (CPO; 14C 2840 ± 80 BP), tools and debitage or discarded flakes made in black volcanic rock have been found. Nearby an extensive rock outcrop of black volcanite, Paso Limay quarry (CPL), with similar characteristics was located. Samples coming from these four sites were analyzed by energy dispersive X-ray fluorescence spectrometry. This characterization allowed the geochemical classification of the lithic material and to correlate the samples with the suspected source after a previous statistical analysis. The majority of the samples were classified as dacites and rhyolites. Only samples coming from CPO site, the closest place to CPL were made exclusively with the quarry rocks. A set of five samples from RCh2/87 and two samples from CTI appear to have same chemical composition as CPL in spite of this site is placed in the opposite bank of the Limay river suggesting that hunter-gatherers could accede to the quarry, eventually. Finally, only a set of five samples coming from RCh2/87 and CTI do not group with the quarry. This fact evidences the existence of secondary sources of supply. The information of this research allowed inferring ancient human mobility patterns in the region. |
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Wos |
000325624300061 |
Publication Date |
2013-07-25 |
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ISSN |
0236-5731; 1588-2780 |
ISBN |
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UA library record; WoS full record |
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no |
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Call Number |
UA @ admin @ c:irua:109743 |
Serial |
7619 |
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Permanent link to this record |
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Author |
Zwozdziak, A.; Sowka, I.; Krupińska, B.; Zwozdziak, J.; Nych, A. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Infiltration or indoor sources as determinants of the elemental composition of particulate matter inside a school in Wroclaw, Poland? |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Building and environment |
Abbreviated Journal |
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Volume |
66 |
Issue |
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Pages |
173-180 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Children's exposure to air pollution requires a focus on air quality in places where they spend most time, e.g. in schools. Therefore, understanding how indoor elemental concentrations relate the outdoor ones is necessary to create healthy indoor school environment. The aims of this study were to examine the elemental composition of particulate matter (PM1, PM2.5, PM10) in the school and also to investigate to what degree indoor elemental concentrations are affected by outdoor air or generated inside the school. The measurements were performed inside and outside the public school building in the centre of the city. It was observed that concentrations of most elements were higher at school than outside. The dominant elements in PM1 both indoors and outdoors were S, Cl, K, and Zn. PM2.5 and PM10 fractions inside the school were clearly enriched in elements of mineral origin, additionally S, Zn, K and Cl were also present in high concentrations both indoors and outdoors. Results suggested that a significant contribution to indoor Zn, Pb and S concentrations in the PM2.5 fraction was from penetration of outdoor air. 88%, 80% and 90% of the observed total variations in indoor concentrations of Zn, Pb, and S were explained by the linear relationship between indoor and outdoor concentrations. The lack of correlation between indoor and outdoor concentrations obtained for Si, Ca, Ti, Sr indicated that these metals were more likely to originate from indoor sources. (C) 2013 Elsevier Ltd. All rights reserved. |
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Wos |
000321423500017 |
Publication Date |
2013-05-09 |
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Edition |
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ISSN |
0360-1323 |
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no |
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Call Number |
UA @ admin @ c:irua:109788 |
Serial |
8087 |
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Author |
Verreydt, G.; Annable, M.D.; Kaskassian, S.; van Keer, I.; Bronders, J.; Diels, L.; Vanderauwera, P. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Field demonstration and evaluation of the passive flux meter on a CAH groundwater plume |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Environmental Science and Pollution Research |
Abbreviated Journal |
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Volume |
20 |
Issue |
7 |
Pages |
4621-4634 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL); Biochemical Wastewater Valorization & Engineering (BioWaVE) |
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Abstract |
This study comprises the first application of the Passive Flux Meter (PFM) for the measurement of chlorinated aliphatic hydrocarbon (CAH) mass fluxes and Darcy water fluxes in groundwater at a European field site. The PFM was originally developed and applied to measurements near source zones. The focus of the PFM is extended from near source to plume zones. For this purpose, 48 PFMs of 1.4 m length were constructed and installed in eight different monitoring wells in the source and plume zone of a CAH-contaminated field site located in France. The PFMs were retrieved, sampled, and analyzed after 3 to 11 weeks of exposure time, depending on the expected contaminant flux. PFM evaluation criteria include analytical, technical, and practical aspects as well as conditions and applicability. PFM flux data were compared with so-called traditional soil and groundwater concentration data obtained using active sampling methods. The PFMs deliver reasonable results for source as well as plume zones. The limiting factor in the PFM applicability is the exposure time together with the groundwater flux. Measured groundwater velocities at the field site range from 2 to 41 cm/day. Measured contaminant flux data raise up to 13 g/m(2)/day for perchloroethylene in the plume zone. Calculated PFM flux averaged concentration data and traditional concentration data were of similar magnitude for most wells. However, both datasets need to be compared with reservation because of the different sampling nature and time. Two important issues are the PFM tracer loss during installation/extraction and the deviation of the groundwater flow field when passing the monitoring well and PFM. The demonstration of the PFM at a CAH-contaminated field site in Europe confirmed the efficiency of the flux measurement technique for source as well as plume zones. The PFM can be applied without concerns in monitoring wells with European standards. The acquired flux data are of great value for the purpose of site characterization and mass discharge modeling, and can be used in combination with traditional soil and groundwater sampling methods. |
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000321126700030 |
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2013-01-02 |
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ISSN |
0944-1344; 1614-7499 |
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no |
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Call Number |
UA @ admin @ c:irua:109817 |
Serial |
7965 |
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Permanent link to this record |
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Author |
Aerts, A.; Janssens, K.; Adams, F. |
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Title |
Chemical analysis of the powder deposit on Chinese jade objects |
Type |
H3 Book chapter |
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Year |
1995 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
12-13 |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Additional Links ![sorted by Additional Links field, ascending order (up)](img/sort_asc.gif) |
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no |
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Call Number |
UA @ admin @ c:irua:10986 |
Serial |
5510 |
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Author |
Roland, M.; Serrano-Ortiz, P.; Kowalski, A.S.; Van Grieken, R.; Janssens, I.A.; et al. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Atmospheric turbulence triggers pronounced diel pattern in karst carbonate geochemistry |
Type |
A1 Journal article |
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Year |
2013 |
Publication |
Biogeosciences |
Abbreviated Journal |
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Volume |
10 |
Issue |
7 |
Pages |
5009-5017 |
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Keywords |
A1 Journal article; Plant and Ecosystems (PLECO) – Ecology in a time of change; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
CO2 exchange between terrestrial ecosystems and the atmosphere is key to understanding the feedbacks between climate change and the land surface. In regions with carbonaceous parent material, CO2 exchange patterns occur that cannot be explained by biological processes, such as disproportionate outgassing during the daytime or night-time CO2 uptake during periods when all vegetation is senescent. Neither of these phenomena can be attributed to carbonate weathering reactions, since their CO2 exchange rates are too small. Soil ventilation induced by high atmospheric turbulence is found to explain atypical CO2 exchange between carbonaceous systems and the atmosphere. However, by strongly altering subsurface CO2 concentrations, ventilation can be expected to influence carbonate weathering rates. By imposing ventilation-driven CO2 outgassing in a carbonate weathering model, we show here that carbonate geochemistry is accelerated and does play a surprisingly large role in the observed CO2 exchange pattern of a semi-arid ecosystem. We found that by rapidly depleting soil CO2 during the daytime, ventilation disturbs soil carbonate equilibria and therefore strongly magnifies daytime carbonate precipitation and associated CO2 production. At night, ventilation ceases and the depleted CO2 concentrations increase steadily. Dissolution of carbonate is now enhanced, which consumes CO2 and largely compensates for the enhanced daytime carbonate precipitation. This is why only a relatively small effect on global carbonate weathering rates is to be expected. On the short term, however, ventilation has a drastic effect on synoptic carbonate weathering rates, resulting in a pronounced diel pattern that exacerbates the non-biological behavior of soil-atmosphere CO2 exchanges in dry regions with carbonate soils. |
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Wos |
000322242700039 |
Publication Date |
2013-07-24 |
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1726-4170; 1726-4189 |
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Additional Links ![sorted by Additional Links field, ascending order (up)](img/sort_asc.gif) |
UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:109862 |
Serial |
7533 |
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Author |
Nuyts, G.; Cagno, S.; Hellemans, K.; Veronesi, G.; Cotte, M.; Janssens, K. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Study of the early stages of Mn intrusion in corroded glass by means of combined SR FTIR/\muXRF imaging and XANES spectroscopy |
Type |
P1 Proceeding |
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Year |
2013 |
Publication |
Procedia Chemistry
T2 – Youth in Conservation of Cultural Heritage Conference (YOCOCU), June 18-20, 2012, University of Antwerp, Antwerp, Belgium |
Abbreviated Journal |
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Volume |
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Issue |
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Pages |
239-247 |
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Keywords |
P1 Proceeding; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Historical glass, especially medieval glass, can undergo weathering under the influence of time and environmental conditions. The aim of this investigation was to better understand the processes involved in this natural degradation process by studying artificially altered glass samples prepared for the use of evaluation of conservation methods. Non-durable glass sensors produced by the Fraunhofer Institute (type M1.0) were used as a starting material for artificial alteration. These were immersed in acidic (pH = 0, 2, 4) and neutral solutions (1 h – 8 h). In a second stage the glass samples were immersed in a 0.5 M MnCl2 solution (24 h, 48 h and 72 h), allowing intrusion of Mn from the solution into the gel layer. The samples were characterized at different stages with reflectance FTIR spectroscopy, mu XRF mapping and mu XANES. All measurements were carried out at ESRF, beamline ID21. Reflectance FTIR spectroscopy measurements were performed in the 800 4000 cm(-1) range. Cluster analysis of the resulting maps evidenced the rapid growth of the gel layer in strong acidic conditions. The average spectra for each cluster feature show for the original glass a strong Si-O- stretching band between 900 and 1000 cm(-1), whereas the gel layer could be identified by the increasing Si-O-Si bands around 1100 and 1250 cm(-1). mu XRF maps were recorded at different stages of the experiment at energies around the Mn-K edge (6.539 keV) and with a step size of 2 by 2 m. These confirm the leaching of K+ and Ca+2 from the glass and the intrusion of Mn from the solution. Mn was found throughout the entire gel layer, but with a concentration gradient peaking at the surface. XANES point measurements were recorded at various points where Mn was present. No spatial variation was found, but linear combination fitting of the spectra with various Mn reference compounds indicated that Mn2+Mn23+O4 is the main Mn compound in the gel layer, as was hypothesised by Watkinson et al. The standard corroded glass samples studied here can be used for the evaluation of conservation treatments in follow-up experiments. (C) 2013 The Authors. Published by Elsevier B.V. Selection and peer-review under responsibility of the IA-CS (Italian Association of Conservation Scientists) and University of Antwerp |
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000321673900030 |
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2013-04-17 |
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8 |
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ISSN |
1876-6196 |
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Times cited |
4 |
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Notes |
; This research was supported by the Interuniversity Attraction Poles Programme – Belgian Science Policy (IUAP VI/16). The text also presents results of GOA XANES “meets ELNES” (Research Fund University of Antwerp, Belgium) and from FWO (Brussels, Belgium) projects no. G.0704.08 and G.01769.09. We gratefully acknowledge ESRF for granting beamtime (experiment EC873). ; |
Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:109871 |
Serial |
5851 |
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Author |
Aerts, A.; Janssens, K.; Adams, F. |
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Title |
A chemical investigation of altered jade art objects |
Type |
A3 Journal article |
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Year |
1995 |
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Orientations |
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79-80 |
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A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:10989 |
Serial |
5516 |
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Author |
Cagno, S.; de Raedt, I.; Jeffries, T.; Janssens, K. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Composition of Facon de Venise glass from early 17th century London in comparison with luxury glass of the same age |
Type |
P1 Proceeding |
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Year |
2012 |
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Proceedings of the Society of Photo-optical Instrumentation Engineers
T2 – Conference on Integrated Approaches to the Study of Historical Glass, (IASHG), APR 16-17, 2012, Brussels, BELGIUM |
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842205-842212 |
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P1 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
SEM-EDX and LA-ICP-MS analyses were performed on a set of early 17th century London glass fragments. The samples originate from two archaeological sites (Aldgate and Old Broad Street) where glass workshops were active in this period. The great majority of the samples are made of soda glass. Two distinct compositional groups are observed, each typical of one site of provenance. The samples originating from the Old Broad Street excavation feature a silica-soda-lime composition, with a moderate amount of potash. The samples from Aldgate are richer in potassium and feature higher amounts of trace elements such as Rb, Zr and Cu. The distinction between the two groups stems from different flux and silica sources used for glassmaking. A comparison with different European glass compositions of that time reveals no resemblance with genuine Venetian production, yet the composition of the Old Broad Street glass shows a close similarity to that of fragments produced 'a la facon de Venise' in Antwerp at the end of the 16th century. This coincides with historical sources attesting the arrival of glassworkers from the Low Countries in England and suggests that a transfer of technology took place near the turn of the century. |
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000311900800005 |
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2012-06-06 |
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8422 |
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978-0-8194-9104-6; 0277-786x |
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Additional Links ![sorted by Additional Links field, ascending order (up)](img/sort_asc.gif) |
UA library record; WoS full record; WoS citing articles |
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1 |
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; ; |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:110142 |
Serial |
5543 |
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Author |
Verreydt, G.; Bronders, J.; van Keer, I.; Diels, L.; Vanderauwera, P. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Passive samplers for monitoring VOCs in groundwater : prospects related to mass flux measurements |
Type |
P3 Proceeding |
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Year |
2011 |
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P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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978-1-907161-16-2 |
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no |
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Call Number |
UA @ admin @ c:irua:110412 |
Serial |
8364 |
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Author |
Herremans, D.; Cagno, S.; Vincke, A.; de Clercq, W.; Janssens, K. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Composition and state of alteration of 18th century glass from the Cistercian nunnery of Clairefontaine (Belgium) |
Type |
P1 Proceeding |
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Year |
2012 |
Publication |
Proceedings of the Society of Photo-optical Instrumentation Engineers
T2 – Conference on Integrated Approaches to the Study of Historical Glass, (IASHG), APR 16-17, 2012, Brussels, BELGIUM |
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842206-842211 |
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P1 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
An extended set of 18th century glass vessels was analyzed by means of SEM-EDX (major and minor element composition) The fragmented archaeological objects were recovered from a latrine belonging to the early 18th century building phase of the nunnery of Clairefontaine, near Arlon (B). On the basis of typology and decoration, the major part of the vessels could be dated around the middle of the 18th century. Variety in color and weathering of the glass suggest differences in glassmaking recipes and in the composition and origin of raw materials. The results of the analysis show how two main compositional groups constitute about 90% of the analyzed glass set, and these are constituted by potash glass (transparent beakers) and high lime low alkali glass (green bottles). Next to these, a few potash-lime and soda glasses are also found. The type of alteration has also a clear relation with the original glass composition. |
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000311900800006 |
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2012-06-06 |
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8422 |
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978-0-8194-9104-6; 0277-786x |
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Notes |
; ; |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:110799 |
Serial |
5537 |
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Author |
Vazquez, C.; Boeykens, S.; Palacios, O.; Caracciolo, N.; Kontozova-Deutsch, V.; Krupińska, B.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Estudio de la contaminacion del aire urbano en cuatro museos de Argentina |
Type |
H3 Book chapter |
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2013 |
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271-282
T2 - Patrimonio cultural : la gestion, el |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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978-987-1323-31-9 |
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UA @ admin @ c:irua:110908 |
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7936 |
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Author |
de Nolf, W. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Imaging of crystalline phase distributions by means of scanning and tomographic X-ray powder diffraction |
Type |
Doctoral thesis |
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2013 |
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407 p. |
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Doctoral thesis; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:110910 |
Serial |
8057 |
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Author |
Janssens, K.; Degryse, P.; Cosyns, P.; Caen, J.; Van 't dack, L. |
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Title |
Annales of the 17th Congress of the International Association for the History of Glass (Antwerp, Belgium, 2006) |
Type |
ME2 Book as editor or co-editor |
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2009 |
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704 p. |
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ME2 Book as editor or co-editor; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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978-90-5487-618-2 |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:110922 |
Serial |
5473 |
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