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Author |
Bruynseels, F.; Storms, H.; Tavares, T.; Van Grieken, R. |
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Title |
Characterization of individual particle types in coastal air by laser microprobe mass analysis |
Type |
A1 Journal article |
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Year |
1985 |
Publication |
International journal of environmental analytical chemistry |
Abbreviated Journal |
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Volume |
23 |
Issue |
1 |
Pages |
1-14 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Laser Microprobe Mass Analysis (LAMMA) was used in a preliminary study to characterize aerosol particles from a beach and inland sites and from a heavily industrialized area. As many as six types of both positive and negative mass spectra with different inorganic and organic signals could be distinguished in the different particle size ranges. Information about the elemental composition and the speciation of S and N was obtained. With increasing distance from sea, progressive uptake of nitrate in seasalt particles was found. Complex particles, containing soot and organic ammonium sulfate, were also detected. |
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A1985AZE1800001 |
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2007-07-07 |
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0306-7319 |
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Call Number |
UA @ admin @ c:irua:116575 |
Serial |
7626 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
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Title |
Chemical characterization of airborne particulate matter above the North Sea |
Type |
P3 Proceeding |
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Year |
1985 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117500 |
Serial |
7646 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
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Title |
Chemical characterization of individual aerosol particles from remote and polluted marine air |
Type |
P3 Proceeding |
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Year |
1985 |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117497 |
Serial |
7647 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
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Title |
LAMMA and electron-microprobe analysis of atmospheric aerosols |
Type |
A1 Journal article |
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Year |
1984 |
Publication |
Journal de physique |
Abbreviated Journal |
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Volume |
45 |
Issue |
C:2 |
Pages |
785-788 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
A laser microprobe mass analyser and a highly automated electron probe X-ray microanalysis unit have been used to study the elemental composition, inorganic speciation and morphology of atmospheric aerosols collected at various remote to polluted and marine to continental locations. |
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Wos |
A1984SQ01400182 |
Publication Date |
2007-08-21 |
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Series Volume |
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Edition |
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ISSN |
0302-0738 |
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UA library record; WoS full record; WoS citing articles |
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no |
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Call Number |
UA @ admin @ c:irua:113621 |
Serial |
8148 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R.; Van der Auwera, L. |
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Title |
Characterization of North-Sea aerosols by individual particle analyses |
Type |
A1 Journal article |
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Year |
1988 |
Publication |
Atmospheric environment : an international journal |
Abbreviated Journal |
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Volume |
22 |
Issue |
11 |
Pages |
2593-2602 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
On aerosol and rain water samples, collected in the Southern Bight of the North Sea, single particle analyses were performed using both laser microprobe mass analysis and electron-probe X-ray microanalysis in combination with an automated image analysis system. In the aerosols collected from an air mass that had travelled from the Atlantic Ocean along the coast of North France, pure seasalt constituted the most abundant particle type, while aluminosilicates (mostly spherical fly-ash particles) amounted to about 20% and mixed seasalt/aluminosilicate, carbonaceous particles, CaSO4 and spherical iron oxides contributed each 510 %. In air masses that had a longer residence time over the continent, spherical iron oxides, carbonaceous particles and ammonium sulfates together made up 70 % of the total particle load. Seasalt particles were nearly all enriched in sulfate or nitrate, but they were seen to be washed out efficiently after a rain shower. In rain water, some 40 % of the particles appeared to be spherical or irregularly shaped aluminosilicates, from fly-ash and dust dispersal, but more than 50 % consisted of SiO2. The high relative abundance of these particles in rain water may be the result of Al leaching from fly-ash, or of more efficient scavenging by rain droplets. |
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A1988R523900028 |
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2003-08-06 |
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Edition |
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ISSN |
1352-2310 |
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UA library record; WoS full record; WoS citing articles |
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no |
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Call Number |
UA @ admin @ c:irua:113610 |
Serial |
7632 |
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Permanent link to this record |
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Author |
Bruynseels, F.; Van Grieken, R. |
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Title |
Direct detection of sulfate and nitrate layers on sampled marine aerosols by laser microprobe mass analysis |
Type |
A1 Journal article |
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Year |
1985 |
Publication |
Atmospheric environment |
Abbreviated Journal |
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Volume |
19 |
Issue |
11 |
Pages |
1969-1970 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
The direct detection of sulfate and nitrate layers on sampled marine aerosols was carried out by laser microprobe mass analysts. |
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2003-08-06 |
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ISSN |
0004-6981 |
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Call Number |
UA @ admin @ c:irua:113617 |
Serial |
7810 |
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Author |
Bruynseels, F.; Van Grieken, R. |
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Title |
Recombination reactions and geometry effects in laser microprobe mass analysis studied with 12C/13C bilayers |
Type |
A1 Journal article |
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Year |
1986 |
Publication |
International journal of mass spectrometry and ion processes |
Abbreviated Journal |
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Volume |
74 |
Issue |
2-3 |
Pages |
161-177 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Bilayers of carbon, consisting of a layer of natural carbon and a second layer highly enriched in 13C, were investigated with the LAMMA 500-® instrument. When such a bilayer is perforated by the laser beam, comparable amounts of 12C and 13C are evaporated and partly ionized so that geometry effects and recombination reactions during laser-induced ionization can straightforwardly be studied. |
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Wos |
A1986G343200003 |
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2002-07-25 |
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ISSN |
0168-1176; 1873-2801 |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:113611 |
Serial |
8461 |
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Author |
Bruynseels, F.; Van Grieken, R. |
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Title |
Recombination reactions and geometry effects in laser microprobe mass analysis studied with 12C/13C bilayers |
Type |
P3 Proceeding |
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Year |
1986 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117512 |
Serial |
8462 |
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Author |
Bruynseels, F.; Van Grieken, R. |
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Title |
Speciation and distribution of sulfur and nitrogen in individual aerosol particles measured by LAMMA |
Type |
P3 Proceeding |
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Year |
1984 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117494 |
Serial |
8568 |
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Author |
Bruynseels, F.J.; Van Grieken, R.E. |
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Title |
Laser microprobe mass spectrometric identification of sulfur species in single micrometer-size particles |
Type |
A1 Journal article |
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Year |
1984 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
56 |
Issue |
6 |
Pages |
871-873 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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A1984SP09600012 |
Publication Date |
2005-03-08 |
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ISSN |
0003-2700; 5206-882x |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:116521 |
Serial |
8163 |
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Author |
Bruynseels, F.J.; Van Grieken, R.E. |
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Title |
Molecular ion distributions in laser microprobe mass-spectrometry of calcium-oxide and calcium salts |
Type |
A1 Journal article |
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Year |
1983 |
Publication |
Spectrochimica acta: part B : atomic spectroscopy |
Abbreviated Journal |
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Volume |
38 |
Issue |
5-6 |
Pages |
853-858 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Laser Microprobe Mass Spectrometry (LAMMA) is used to examine micrometric particles of calcium oxyanion salts (CaCO3, CaSO4, CaSO4·2H2O) and calcium oxide, in both the positive and negative ion mode. The major molecular ions, appearing in the positive mass spectrum, can be divided into three series, namely CamOm-1+, (CaO)m+ and (CaO)mH+ (m = 1-4). In the case of the former two series the relative intensities of the mass peaks as a function of the fragment valence K = (1 + 2n)/m, for CamOn+, can be fitted to a Gaussian distribution curve, as was earlier demonstrated for secondary ion mass spectrometry. The high stability of the (CaO)mH+ series can be explained by the favourable fragment valence of +2 corresponding to the usual oxidation state of calcium. |
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A1983QY80000019 |
Publication Date |
2002-07-25 |
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Abbreviated Series Title |
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Edition |
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ISSN |
0584-8547; 1873-3565 |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:113626 |
Serial |
8273 |
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Author |
Buczyńska, A.J. |
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Title |
Analytical methodology for combined stable carbon isotope ratio and concentration measurement of polycyclic aromatic hydrocarbons in air particulate matter |
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Doctoral thesis |
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Year |
2014 |
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Abbreviated Journal |
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Pages |
186 p. |
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Keywords |
Doctoral thesis; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:120050 |
Serial |
7456 |
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Author |
Buczyńska, A.J.; Krata, A.; Stranger, M.; Godoi, A.F.L.; Kontozova-Deutsch, V.; Bencs, L.; Naveau, I.; Roekens, E.; Van Grieken, R. |
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Title |
Atmospheric BTEX-concentrations in an area with intensive street traffic |
Type |
A1 Journal article |
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Year |
2009 |
Publication |
Atmospheric environment : an international journal |
Abbreviated Journal |
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Volume |
43 |
Issue |
2 |
Pages |
311-318 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
The major threat to clean air in developed and industrializing countries is now posed by traffic emissions. The effects of traffic road modifications on the air quality are, however, rarely reported in the literature. The aim of this study was to determine the influence of the modernization and renovation of a traffic artery in the region of Mortsel (Antwerp, Belgium) on the concentration of volatile organic compounds such as: benzene, toluene, ethylbenzene and m-, p-, o-xylenes (BTEX). The original goal of the reconstruction works was to reduce the traffic lanes of one of the busiest streets in Antwerp, in order to discourage the road traffic and in consequence also to improve the air quality in this region. The average concentrations of BTEX before these works in 2003 were: 1.6, 7.0, 0.9, 2.3, and 0.9 ìg/m3, for benzene, toluene, ethylbenzene, m + p xylenes, and o-xylene, respectively. However, after the completion of the works, in 2005, they were slightly higher: 2.5, 9.5, 1.6, 3.4, and 1.3 ìg/m3, respectively. The scatter plots of benzene against toluene, ethylbenzene and xylenes in 2003 and 2005 showed very good correlations. This fact indicated that all of the measured compounds originated from the same source, namely the road traffic. Moreover, the data obtained from an air-monitoring station at less than 6 km distance from the sampling site (operated by the Flemish Environment Agency, and located in Borgerhout, Antwerp), confirmed the lack of influence of background concentrations of BTEX. The obtained results led to the conclusion that the reduction of the number of traffic lanes had apparently increased the traffic jams and also increased the emission from cars. Therefore, these modernization works had even a negative impact on the local concentration of traffic-related pollutants as BTEX. |
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000262956500011 |
Publication Date |
2008-10-18 |
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Edition |
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ISSN |
1352-2310 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:72925 |
Serial |
7518 |
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Author |
Bulut, P.; Beceren, B.; Yildirim, S.; Sevik, C.; Gurel, T. |
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Title |
Promising room temperature thermoelectric conversion efficiency of zinc-blende AgI from first principles |
Type |
A1 Journal article |
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Year |
2021 |
Publication |
Journal Of Physics-Condensed Matter |
Abbreviated Journal |
J Phys-Condens Mat |
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Volume |
33 |
Issue |
1 |
Pages |
015501 |
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Keywords |
A1 Journal article; Condensed Matter Theory (CMT) |
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Abstract |
The theoretical investigation on structural, vibrational, and electronic properties of zinc-blende (ZB) AgI were carried out employing first principles density functional theory calculations. Thermoelectric properties then were predicted through semi-classical Boltzmann transport equations within the constant relaxation time approximation. Equilibrium lattice parameter, bulk modulus, elastic constants, and vibrational properties were calculated by using generalized gradient approximation. Calculated properties are in good agreement with available experimental values. Electronic and thermoelectric properties were investigated both with and without considering spin-orbit coupling (SOC) effect which is found to have a strong influence on p-type Seebeck coefficient as well as the power factor of the ZB-AgI. By inclusion of SOC, a reduction of the band-gap and p-type Seebeck coefficients as well as the power factor was found which is the indication of that spin-orbit interaction cannot be ignored for p-type thermoelectric properties of the ZB-AgI. By using deformation potential theory for electronic relaxation time and experimentally predicted lattice thermal conductivity, we obtained aZTvalue 1.69 (0.89) at 400 K for n-type (p-type) carrier concentration of 1.5 x 10(18)(4.6 x10(19)) cm(-3)that makes ZB-AgI as a promising room temperature thermoelectric material. |
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Place of Publication |
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Editor |
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Language |
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Wos |
000577217600001 |
Publication Date |
2020-09-14 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
0953-8984 |
ISBN |
|
Additional Links |
UA library record; WoS full record |
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Impact Factor |
2.649 |
Times cited |
|
Open Access |
Not_Open_Access |
|
|
Notes |
|
Approved |
Most recent IF: 2.649 |
|
|
Call Number |
UA @ admin @ c:irua:193762 |
Serial |
8425 |
|
Permanent link to this record |
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Author |
Buydens, L.; van Espen, P.; Rutan, S. |
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Title |
CAC-2010 : Twelfth international conference on chemometrics in analytical chemistry |
Type |
Editorial |
|
Year |
2011 |
Publication |
Analytica chimica acta |
Abbreviated Journal |
|
|
|
Volume |
705 |
Issue |
1/2 |
Pages |
1 |
|
|
Keywords |
Editorial; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000295993900001 |
Publication Date |
2011-08-14 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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|
Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
0003-2670; 1873-4324 |
ISBN |
|
Additional Links |
UA library record; WoS full record |
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Impact Factor |
|
Times cited |
|
Open Access |
|
|
|
Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:93573 |
Serial |
7570 |
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Permanent link to this record |
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Author |
Buyle, M.; Audenaert, A.; Brusselaers, J.; Van Passel, S. |
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|
Title |
Rebound effects following technological advancement? The case of a global shock in ferrochrome supply |
Type |
A1 Journal article |
|
Year |
2023 |
Publication |
Journal of cleaner production |
Abbreviated Journal |
|
|
|
Volume |
391 |
Issue |
|
Pages |
136264-11 |
|
|
Keywords |
A1 Journal article; Economics; Engineering sciences. Technology; Energy and Materials in Infrastructure and Buildings; Engineering Management (ENM) |
|
|
Abstract |
Novel recycling technologies aim at increasing material efficiency by turning former waste products into valuable reclaimed resources. A key question is whether such technologies really reduce primary resource consumption or instead stimulate aggregated market demand. In this study the consequences of a positive shock in ferrochrome supply to the global stainless steel value chain is assessed quantitatively. This new source might be unlocked by technology under development for the recovery of chromium from carbon and stainless steel slags. The aim of this study is to quantitatively assess the income and substitution effects of reclaimed ferrochrome along a part of the stainless steel value chain. The impact of the supply shock is analysed by means of a vector autoregression (VAR), a dynamic model where lagged values of all included variables estimate current state of the system. Additionally, the VAR model is extended to a structural vector autoregression (SVAR) to account for contemporary effects as well. Both the VAR and SVAR model indicate that additional ferrochrome supply leads to an increase in aggregated supply of stainless steel, in combination with a substitution effect between ferrochrome and nickel. The extended SVAR model additionally highlights that contemporaneous effects do play an important role as well to capture the direct rebound effect in the ferrochrome market when working with quarterly data. In other words, an additional supply of reclaimed ferrochrome triggers a complex combination of interactions and consequences, yet it does not necessarily lead to a lower overall material consumption. The main contributions of this paper are the assessment of direct rebound effects of supplying reclaimed metals along the value chain and the demonstration that quantifying the effects of circular strategies is feasible. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000930165300001 |
Publication Date |
2023-01-30 |
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Series Editor |
|
Series Title |
|
Abbreviated Series Title |
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|
|
Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
0959-6526 |
ISBN |
|
Additional Links |
UA library record; WoS full record |
|
|
Impact Factor |
11.1 |
Times cited |
|
Open Access |
OpenAccess |
|
|
Notes |
|
Approved |
Most recent IF: 11.1; 2023 IF: 5.715 |
|
|
Call Number |
UA @ admin @ c:irua:193569 |
Serial |
7365 |
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Permanent link to this record |
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Author |
Buyle, M.; Maes, B.; Van Passel, S.; Boonen, K.; Vercalsteren, A.; Audenaert, A. |
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|
Title |
Ex-ante LCA of emerging carbon steel slag treatment technologies : fast forwarding lab observations to industrial-scale production |
Type |
A1 Journal article |
|
Year |
2021 |
Publication |
Journal Of Cleaner Production |
Abbreviated Journal |
J Clean Prod |
|
|
Volume |
313 |
Issue |
|
Pages |
127921 |
|
|
Keywords |
A1 Journal article; Engineering sciences. Technology; Energy and Materials in Infrastructure and Buildings (EMIB) |
|
|
Abstract |
The valuable properties of carbon steel slag are currently underexploited. To date, research mainly focusses on valorising a single property of the slag. In this study an ex-ante life cycle assessment (LCA) was applied to evaluate the environmental profile of a novel technological pathway aimed at the extraction of chromium from carbon steel slag in combination with high quality valorisation of the residual matrix material. A comparison with current practice was made, not only by calculating the environmental impact of the lab scale observations, but more importantly by estimating the impact on an industrial scale. Practical guidance on ex-ante LCA is limited, so this study contributes by incorporating simulations on thermodynamic behaviour, complemented with empirical calculation rules and including information derived from similar technologies to perform the upscaling. These principles of ex-ante LCA were applied to the lab results of two consecutive research iterations. Substantial improvements of the environmental profile were observed: ex-ante results turned out to be a factor 20 lower compared to the results from the lab observations after the first iteration and had decreased by a factor 2 compared to the small pilot scale of the second iteration. All upscaled results are better than those from the worst case reference scenario (landfill). Based on the experience gained after this iterative research cycle, a practical recommendation is that at a low technology readiness level using more simple calculation rules in combination with a flowsheet based on elementary design principles for processes at an industrial scale is a more efficient way of modelling compared to a fully-fledged process design from the start. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000693416000002 |
Publication Date |
2021-06-14 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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|
|
Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
0959-6526 |
ISBN |
|
Additional Links |
UA library record; WoS full record |
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|
Impact Factor |
5.715 |
Times cited |
|
Open Access |
Not_Open_Access |
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Notes |
|
Approved |
Most recent IF: 5.715 |
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Call Number |
UA @ admin @ c:irua:179313 |
Serial |
6922 |
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Permanent link to this record |
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Author |
Buysse, C. |
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Title |
Perovskite capillaries for gas separation in sustainable energy production |
Type |
Doctoral thesis |
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Year |
2011 |
Publication |
|
Abbreviated Journal |
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Volume |
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Issue |
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Pages |
201 p. |
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Keywords |
Doctoral thesis; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Abstract |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
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Publication Date |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
|
ISBN |
|
Additional Links |
UA library record |
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|
Impact Factor |
|
Times cited |
|
Open Access |
|
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|
Notes |
|
Approved |
no |
|
|
Call Number |
UA @ admin @ c:irua:90548 |
Serial |
8373 |
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Permanent link to this record |
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Author |
Buytaert, V.; Muys, B.; Devriendt, N.; Pelkmans, L.; Kretzschmar, J.G.; Samson, R. |
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Title |
Towards integrated sustainability assessment for energetic use of biomass : a state of the art evaluation of assessment tools |
Type |
A1 Journal article |
|
Year |
2011 |
Publication |
Renewable and sustainable energy reviews |
Abbreviated Journal |
|
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|
Volume |
15 |
Issue |
8 |
Pages |
3918-3933 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Abstract |
Biomass is expected to play an increasingly significant role in the greening of energy supply. Nevertheless, concerns are rising about the sustainability of large-scale energy crop production. Impacts must be assessed carefully before deciding whether and how this industry should be developed, and what technologies, policies and investment strategies should be pursued. There is need for a comprehensive and reliable sustainability assessment tool to evaluate the environmental, social and economic performance of biomass energy production. This paper paves the way for such a tool by analysing and comparing the performance and applicability of a selection of existing tools that are potentially useful for sustainability assessment of bioenergy systems. The selected tools are: Criteria And Indicators (C&I), Life Cycle Assessment (LCA), Environmental Impact Assessment (EIA), Cost Benefit Analysis (CBA), Exergy Analysis (EA) and System Perturbation Analysis (SPA). To evaluate the tools, a framework was constructed that consists of four evaluation levels: sustainability issues, tool attributes, model structure, area of application. The tools were then evaluated using literature data and with the help of a Delphi panel of experts. Finally, a statistical analysis was performed on the resulting data matrix to detect significant differences between tools. It becomes clear that none of the selected tools is able to perform a comprehensive sustainability assessment of bioenergy systems. Every tool has its particular advantages and disadvantages, which means that trade-offs are inevitable and a balance must be found between scientific accuracy and pragmatic decision making. A good definition of the assessment objective is therefore crucial. It seems an interesting option to create a toolbox that combines procedural parts of C&I and EIA, supplemented with calculation algorithms of LCA and CBA for respectively environmental and economic sustainability indicators. Nevertheless, this would require a more comprehensive interdisciplinary approach to align the different tool characteristics and focuses. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000298764100043 |
Publication Date |
2011-08-06 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
1364-0321; 1879-0690 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
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|
Impact Factor |
|
Times cited |
|
Open Access |
|
|
|
Notes |
|
Approved |
no |
|
|
Call Number |
UA @ admin @ c:irua:96444 |
Serial |
8682 |
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Permanent link to this record |
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Author |
Byrnes, I.; Rossbach, L.M.; Brede, D.A.; Grolimund, D.; Sanchez, D.F.; Nuyts, G.; Cuba, V.; Reinoso-Maset, E.; Salbu, B.; Janssens, K.; Oughton, D.; Scheibener, S.; Teien, H.-C.; Lind, O.C. |
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Title |
Synchrotron-based X-ray fluorescence imaging elucidates uranium toxicokinetics in Daphnia magna |
Type |
A1 Journal article |
|
Year |
2023 |
Publication |
ACS nano |
Abbreviated Journal |
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|
Volume |
17 |
Issue |
6 |
Pages |
5296-5305 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Antwerp X-ray Imaging and Spectroscopy (AXIS) |
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Abstract |
A combination of synchrotron-based elemental anal-ysis and acute toxicity tests was used to investigate the biodistribution and adverse effects in Daphnia magna exposed to uranium nanoparticle (UNP, 3-5 nm) suspensions or to uranium reference (Uref) solutions. Speciation analysis revealed similar size distributions between exposures, and toxicity tests showed com-parable acute effects (UNP LC50: 402 mu g L-1 [336-484], Uref LC50: 268 mu g L-1 [229-315]). However, the uranium body burden was 3 -to 5-fold greater in UNP-exposed daphnids, and analysis of survival as a function of body burden revealed a similar to 5-fold higher specific toxicity from the Uref exposure. High-resolution X-ray fluorescence elemental maps of intact, whole daphnids from sublethal, acute exposures of both treatments revealed high uranium accumulation onto the gills (epipodites) as well as within the hepatic ceca and the intestinal lumen. Uranium uptake into the hemolymph circulatory system was inferred from signals observed in organs such as the heart and the maxillary gland. The substantial uptake in the maxillary gland and the associated nephridium suggests that these organs play a role in uranium removal from the hemolymph and subsequent excretion. Uranium was also observed associated with the embryos and the remnants of the chorion, suggesting uptake in the offspring. The identification of target organs and tissues is of major importance to the understanding of uranium and UNP toxicity and exposure characterization that should ultimately contribute to reducing uncertainties in related environmental impact and risk assessments. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000960129800001 |
Publication Date |
2023-03-15 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
1936-0851 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
|
|
Impact Factor |
17.1 |
Times cited |
|
Open Access |
OpenAccess |
|
|
Notes |
|
Approved |
Most recent IF: 17.1; 2023 IF: 13.942 |
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|
Call Number |
UA @ admin @ c:irua:196061 |
Serial |
8631 |
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Permanent link to this record |
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Author |
Byrnes, I.; Rossbach, L.M.; Jaroszewicz, J.; Grolimund, D.; Sanchez, D.F.; Gomez-Gonzalez, M.A.; Nuyts, G.; Reinoso-Maset, E.; Janssens, K.; Salbu, B.; Brede, D.A.; Lind, O.C. |
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Title |
Synchrotron XRF and histological analyses identify damage to digestive tract of uranium NP-exposed Daphnia magna |
Type |
A1 Journal article |
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Year |
2023 |
Publication |
Environmental science and technology |
Abbreviated Journal |
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|
|
Volume |
57 |
Issue |
2 |
Pages |
1071-1079 |
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Keywords |
A1 Journal article; Antwerp X-ray Imaging and Spectroscopy (AXIS) |
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Abstract |
Micro-and nanoscopic X-ray techniques were used to investigate the relationship between uranium (U) tissue distributions and adverse effects to the digestive tract of aquatic model organism Daphnia magna following uranium nanoparticle (UNP) exposure. X-ray absorption computed tomography measure-ments of intact daphnids exposed to sublethal concentrations of UNPs or a U reference solution (URef) showed adverse morphological changes to the midgut and the hepatic ceca. Histological analyses of exposed organisms revealed a high proportion of abnormal and irregularly shaped intestinal epithelial cells. Disruption of the hepatic ceca and midgut epithelial tissues implied digestive functions and intestinal barriers were compro-mised. Synchrotron-based micro X-ray fluorescence (XRF) elemental mapping identified U co-localized with morphological changes, with substantial accumulation of U in the lumen as well as in the epithelial tissues. Utilizing high-resolution nano-XRF, 400-1000 nm sized U particulates could be identified throughout the midgut and within hepatic ceca cells, coinciding with tissue damages. The results highlight disruption of intestinal function as an important mode of action of acute U toxicity in D. magna and that midgut epithelial cells as well as the hepatic ceca are key target organs. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000910915100001 |
Publication Date |
2023-01-04 |
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Series Editor |
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Series Title |
|
Abbreviated Series Title |
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Series Volume |
|
Series Issue |
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Edition |
|
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|
ISSN |
0013-936x; 1520-5851 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
|
|
Impact Factor |
11.4 |
Times cited |
|
Open Access |
OpenAccess |
|
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Notes |
|
Approved |
Most recent IF: 11.4; 2023 IF: 6.198 |
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Call Number |
UA @ admin @ c:irua:193478 |
Serial |
7342 |
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Permanent link to this record |
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Author |
Cabal Rodríguez, A.E.; Leyva Pernia, D.; Schalm, O.; van Espen, P.J.M. |
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Title |
Possibilities of energy-resolved X-ray radiography for the investigation of paintings |
Type |
A1 Journal article |
|
Year |
2012 |
Publication |
Analytical and bioanalytical chemistry |
Abbreviated Journal |
|
|
|
Volume |
402 |
Issue |
4 |
Pages |
1471-1480 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
X-ray radiographic images of paintings often show little or no contrast. In order to increase the contrast in radiographic images we measured the X-ray spectrum of a low power X-ray tube, after passing through the painting, with a high energy-resolution SDD detector. To obtain images, the detector is collimated with a 400 mu m diameter pinhole and the painting was moved through the beam in the x and y-direction using a dwell time of a few seconds per pixel. The data obtained consists of a data cube of, typically, 200 x 200 pixels and a 512-channel X-ray spectrum for each pixel, spanning the energy range from 0 to 40 keV. Having the absorbance spectrum available for each pixel, we are able, a posteriori, to produce images by edge subtraction for any given element. In this way high contrast, element-specific, images can be obtained. Because of the high energy-resolution a much simpler edge subtraction algorithm can be applied. We also used principal-component imaging to obtain, in a more automated way, images with high contrast. Some of these images can easily be attributed to specific elements. It turns out that preprocessing of the spectral data is crucial for the success of the multivariate image processing. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000299842000008 |
Publication Date |
2011-07-14 |
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Series Editor |
|
Series Title |
|
Abbreviated Series Title |
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Series Volume |
|
Series Issue |
|
Edition |
|
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|
ISSN |
1618-2642; 1618-2650 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
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Impact Factor |
|
Times cited |
|
Open Access |
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|
Notes |
|
Approved |
no |
|
|
Call Number |
UA @ admin @ c:irua:96200 |
Serial |
8394 |
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Permanent link to this record |
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Author |
Cabal, A.; Schalm, O.; Eyskens, P.; Willems, P.; Harth, A.; van Espen, P. |
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Title |
Comparison of x-ray absorption and emission techniques for the investigation of paintings |
Type |
A1 Journal article |
|
Year |
2015 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
|
|
|
Volume |
44 |
Issue |
3 |
Pages |
141-148 |
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|
Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Antwerp Cultural Heritage Sciences (ARCHES) |
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|
Abstract |
Four x-ray techniques: computed radiography, emission radiography, energy-resolved radiography and imaging x-ray fluorescence were compared using four mock-up panel paintings. The paintings have different stratigraphy and pigments and are representative for different historical periods. One of the paintings has a hidden underlying painting. The type of pigments used mainly influences the information obtained by both the emission and absorption measurements; high-Z white pigment and high-Z color pigments giving the best contrast. Each of the techniques revealed interesting aspects of the paintings, but none of them could reveal the hidden painting to a satisfactory level. Due to the statistical quality of the spectral data, x-ray fluorescence gives elemental images with high contrast. The radiographic images are better to reveal the internal structure. Imaging x-ray fluorescence and energy-resolved radiography measurements can be done simultaneously, and the combination has the highest potential for the study of complex multilayer paintings. Copyright (c) 2015 John Wiley & Sons, Ltd. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000353644500010 |
Publication Date |
2015-02-05 |
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Series Editor |
|
Series Title |
|
Abbreviated Series Title |
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|
Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
0049-8246 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
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Impact Factor |
|
Times cited |
|
Open Access |
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|
Notes |
|
Approved |
no |
|
|
Call Number |
UA @ admin @ c:irua:126016 |
Serial |
7698 |
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Permanent link to this record |
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Author |
Cadorim, L.R.; de Toledo, L.V.; Ortiz, W.A.; Berger, J.; Sardella, E. |
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Title |
Closed vortex state in three-dimensional mesoscopic superconducting films under an applied transport current |
Type |
A1 Journal article |
|
Year |
2023 |
Publication |
Physical review B |
Abbreviated Journal |
Phys Rev B |
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|
Volume |
107 |
Issue |
9 |
Pages |
094515-94518 |
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Keywords |
A1 Journal article; Condensed Matter Theory (CMT) |
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Abstract |
By using the full 3D generalized time-dependent Ginzbug-Landau equation, we study a long superconducting film of finite width and thickness under an applied transport current. We show that, for sufficiently large thickness, the vortices and the antivortices become curved before they annihilate each other. As they approach the center of the sample, their ends combine, producing a single closed vortex. We also determine the critical values of the thickness for which the closed vortex sets in for different values of the Ginzburg-Ladau parameter. Finally, we propose a model of how to detect a closed vortex experimentally. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Editor |
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Language |
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Wos |
000957055800002 |
Publication Date |
2023-03-20 |
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Series Editor |
|
Series Title |
|
Abbreviated Series Title |
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|
|
Series Volume |
|
Series Issue |
|
Edition |
|
|
|
ISSN |
2469-9969; 2469-9950 |
ISBN |
|
Additional Links |
UA library record; WoS full record; WoS citing articles |
|
|
Impact Factor |
3.7 |
Times cited |
|
Open Access |
Not_Open_Access |
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|
Notes |
|
Approved |
Most recent IF: 3.7; 2023 IF: 3.836 |
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|
Call Number |
UA @ admin @ c:irua:196079 |
Serial |
7673 |
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Permanent link to this record |
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Author |
Cadorim, L.R.; Sardella, E.; Milošević, M.V. |
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Title |
Vortical versus skyrmionic states in the topological phase of a twisted bilayer with d-wave superconducting pairing |
Type |
A1 Journal article |
|
Year |
2024 |
Publication |
Physical review B |
Abbreviated Journal |
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|
|
Volume |
110 |
Issue |
6 |
Pages |
064508-64511 |
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Keywords |
A1 Journal article; Condensed Matter Theory (CMT) |
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Abstract |
It was recently shown that a chiral topological phase emerges from the coupling of two twisted monolayers of superconducting Bi2Sr2CaCu2O8+delta for 2 Sr 2 CaCu 2 O 8 +delta for certain twist angles. In this work, we reveal the behavior of such twisted superconducting bilayers with d x 2 – y 2 pairing symmetry in the presence of an applied magnetic field. Specifically, we show that the emergent vortex matter can serve as a smoking gun for the detection of topological superconductivity in such bilayers. Moreover, we report two distinct skyrmionic states that characterize the chiral topological phase and provide a full account of their experimental signatures and their evolution with the twist angle. |
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https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=brocade2&SrcAuth=WosAPI&KeyUT=WOS:001290 |
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2024-08-12 |
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2469-9969; 2469-9950 |
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UA library record; WoS full record |
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Impact Factor |
3.7 |
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Approved |
Most recent IF: 3.7; 2024 IF: 3.836 |
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Call Number |
UA @ admin @ c:irua:208602 |
Serial |
9327 |
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Author |
Caen, J.; Cagno, S.; Janssens, K. |
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Title |
The stained-glass panel depicting the anointing at Bethany : art historical research, technical analysis, and treatment |
Type |
H2 Book chapter |
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2013 |
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247-257 |
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Keywords |
H2 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Antwerp Cultural Heritage Sciences (ARCHES) |
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Abstract |
In 2008, Museum M in Louvain (Flanders, Belgium) acquired a panel depicting The Anointing at Bethany that is believed once to have adorned the citys former Charterhouse. The panel required conservation treatment, which was preceded by a thorough art-historical and technical examination. It emerged that comparable panels are kept at the Metropolitan Museum of Art and the Riverside Church in New York. Chemical analyses show most of the glass in the panel to have a typical 16th century high-limelow-alkali composition. The conservation treatment was based on the evaluation of these findings and focused very strongly on enhancing the aesthetic balance for an improved reading of the panel. |
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978-90-8932-113-8 |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:114605 |
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5847 |
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Author |
Caen, J.; Legrand, S.; van der Snickt, G.; Janssens, K. |
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Title |
Macro X-ray fluorescence (MA-XRF) scanning : a new and efficient method for documenting stained-glass panels |
Type |
P3 Proceeding |
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Year |
2015 |
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P3 Proceeding; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Antwerp Cultural Heritage Sciences (ARCHES) |
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978-2-9543731-1-9 |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:126832 |
Serial |
5697 |
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Author |
Caen, J.; Schalm, O.; Janssens, K. |
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Title |
15th century stained-glass windows in the former County of Flanders : a historical and chemical study related to recent conservation campaigns |
Type |
P2 Proceeding |
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Year |
2009 |
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459-466 |
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Keywords |
P2 Proceeding; Engineering sciences. Technology; History; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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978-90-5487-618-2 |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:115477 |
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5449 |
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Caen, J.; Schalm, O.; Janssens, K. |
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Caractérisation historique et chimique des peintures en grisaille et du verre de vitrail dans l'oeuvre de J.-B. Capronnier (1814 – 1891) et J.-B. Bethune (1821 – 1894) |
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P3 Proceeding |
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2000 |
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P3 Proceeding; Art; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:112007 |
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7576 |
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Caen, J.; Schalm, O.; Pires De Matos, A.; Ruivo, A.; Ferreira, M.; Janssens, K. |
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Reproduction of 16-17th centuries enamels for stained glass after orignal compositions and recipes |
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P3 Proceeding |
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2008 |
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P3 Proceeding; Art; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:112032 |
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5814 |
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