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Author Liu, P.; Madsen, J.; Schiotz, J.; Wagner, J.B.; Hansen, T.W. url  doi
openurl 
  Title Reversible and concerted atom diffusion on supported gold nanoparticles Type A1 Journal article
  Year (down) 2020 Publication Journal Of Physics-materials Abbreviated Journal  
  Volume 3 Issue 2 Pages 024009  
  Keywords A1 Journal article; Electron microscopy for materials research (EMAT)  
  Abstract Traditionally, direct imaging of atom diffusion is only available by scanning tunneling microscopy and field ion microscopy on geometry-constrained samples: flat surfaces for STM and needle tips for FIM. Here we show time-resolved atomic-scale HRTEM investigations of CeO2-supported Au nanoparticle surfaces to characterize the surface dynamics of atom columns on gold nanoparticles. The observed surface dynamics have been categorized into four types: layer jumping, layer gliding, re-orientation and surface reconstruction. We successfully captured atoms moving in a concerted manner with a time resolution of 0.1 s. A quantitative approach for measuring the dynamics in various gaseous surroundings at elevated temperatures is presented. An approach for measuring quantitative electron beam effects on the surface dynamics is presented by counting atom column occupation as a function of time under a range of dose rates in high vacuum.  
  Address  
  Corporate Author Thesis  
  Publisher Place of Publication Editor  
  Language Wos 000560432800009 Publication Date 2020-03-24  
  Series Editor Series Title Abbreviated Series Title  
  Series Volume Series Issue Edition  
  ISSN ISBN Additional Links UA library record; WoS full record; WoS citing articles  
  Impact Factor Times cited 2 Open Access OpenAccess  
  Notes ; ; Approved Most recent IF: NA  
  Call Number UA @ admin @ c:irua:171320 Serial 6597  
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