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Author |
Van Grieken, R.; Vleugels, G.; Sweevers, E.; Dewolfs, R. |
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Title |
Effects of air pollution on historic buildings and monuments (1986-1990): scientific basis for conservation: analytical study of the weathering of building stones under field-exposure conditions |
Type |
A3 Journal article |
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Year |
1994 |
Publication |
European cultural heritage newsletter on research |
Abbreviated Journal |
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Volume |
8 |
Issue |
2 |
Pages |
2-7 |
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Keywords |
A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:55573 |
Serial |
7844 |
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Author |
Torfs, K.; Van Grieken, R. |
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Title |
Effects of marine spray and air pollution on monuments in the Mediterranean coastal environment |
Type |
H3 Book chapter |
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Year |
1996 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
170-174
T2 - Cultural research in Europe 1996 / Ha |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:14680 |
Serial |
7848 |
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Author |
De Vis, K.; Jembrih-Simbürger, D.; Schalm, O.; Schreiner, M.; Caen, J. |
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Title |
Einfluss verschiedener Silbersalze auf die Farbintensität von Silbergelb : analytische Untersuchungen |
Type |
A2 Journal article |
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Year |
2002 |
Publication |
Zeitschrift für Kunsttechnologie und Konservierung |
Abbreviated Journal |
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Volume |
16 |
Issue |
1 |
Pages |
147-157 |
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Keywords |
A2 Journal article; Art; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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ISSN |
0931-7198 |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:107748 |
Serial |
7855 |
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Author |
Lou, W.-K. |
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Title |
The electrical properties of low low dimensional topological insulators |
Type |
Doctoral thesis |
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Year |
2012 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
186 p. |
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Keywords |
Doctoral thesis; Condensed Matter Theory (CMT) |
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no |
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Call Number |
UA @ admin @ c:irua:158894 |
Serial |
7858 |
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Author |
Bia, P.; Caratelli, D.; Mescia, L.; Gielis, J. |
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Title |
Electromagnetic characterization of supershaped lens antennas for high-frequency applications |
Type |
H1 Book chapter |
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Year |
2013 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
1679-1682
T2 - Proceedings of the 43rd European Mi |
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Keywords |
H1 Book chapter; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Wos |
000330768700424 |
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ISBN |
978-2-87487-031-6 |
Additional Links |
UA library record; WoS full record; WoS citing articles |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:110954 |
Serial |
7865 |
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Permanent link to this record |
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Author |
Xhoffer, C.; Jacob, W.; Van Grieken, R.; Broekaert, J.A.C.; Buseck, P. |
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Title |
Electron energy-loss spectroscopy and its application to individual particle analysis |
Type |
P3 Proceeding |
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Year |
1992 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:2862 |
Serial |
7868 |
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Permanent link to this record |
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Author |
Storms, H.; Van Dyck, P.; Van Grieken, R.; Maenhaut, W. |
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Title |
Electron microprobe observations of recrystallization affecting PIXE-analysis of marine aerosol deposits |
Type |
A1 Journal article |
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Year |
1985 |
Publication |
Journal of trace and microprobe techniques |
Abbreviated Journal |
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Volume |
2 |
Issue |
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Pages |
103-117 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Edition |
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ISSN |
0733-4680; 1532-2270 |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:116718 |
Serial |
7871 |
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Permanent link to this record |
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Author |
Leysen, L.A.; De Waele, J.K.; Roekens, E.J.; Van Grieken, R.E. |
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Title |
Electron probe micro-analysis and laser microprobe mass analysis of material, leached from a limestone cathedral |
Type |
A1 Journal article |
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Year |
1987 |
Publication |
Scanning microscopy |
Abbreviated Journal |
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Volume |
1 |
Issue |
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Pages |
1617-1630 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Series Volume |
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Edition |
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ISSN |
0891-7035 |
ISBN |
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UA library record |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:116794 |
Serial |
7872 |
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Permanent link to this record |
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Author |
Hoornaert, S.; Treiger, B.; Van Grieken, R.; Valkovic, V. |
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Title |
Electron probe X-ray microanalysis for the assessment of homogeneity of candidate reference materials at the nanogram level |
Type |
H3 Book chapter |
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Year |
1996 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
29-49b
T2 - Reference materials for microanalytica |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
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UA library record |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:14681 |
Serial |
7874 |
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Permanent link to this record |
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Author |
Rahemi, V. |
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Title |
Electrosensing applications by using titania as a support for bio(inspired) molecules |
Type |
Doctoral thesis |
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Year |
2018 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
133 p. |
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Keywords |
Doctoral thesis; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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UA library record |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:152884 |
Serial |
7877 |
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Permanent link to this record |
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Author |
Johansson, T.B.; Nelson, J.W.; Van Grieken, R.E.; Winchester, J.W. |
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Title |
Elemental analysis of aerosol-size fractions by proton-induced X-ray-emission |
Type |
A1 Journal article |
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Year |
1973 |
Publication |
Transactions of the American Nuclear Society |
Abbreviated Journal |
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Volume |
17 |
Issue |
Nov |
Pages |
103-103 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Wos |
A1973R161300114 |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0003-018x |
ISBN |
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Additional Links |
UA library record; WoS full record |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:113643 |
Serial |
7880 |
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Permanent link to this record |
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Author |
Smekens, A.; Knupfer, M.; Berghmans, P.; Van Grieken, R. |
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Title |
The elemental composition and microstructure of soot emitted by different sources |
Type |
A1 Journal article |
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Year |
2000 |
Publication |
Journal of aerosol science |
Abbreviated Journal |
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Volume |
31 |
Issue |
S1 |
Pages |
917-918 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Abbreviated Series Title |
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Edition |
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ISSN |
0021-8502; 1879-1964 |
ISBN |
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Additional Links |
UA library record |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:31647 |
Serial |
7887 |
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Permanent link to this record |
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Author |
Vargas Paredes, A.A. |
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Title |
Emergent phenomena in superconductors in presence of intraband and cross-band pairing |
Type |
Doctoral thesis |
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Year |
2020 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
142 p. |
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Keywords |
Doctoral thesis; Condensed Matter Theory (CMT) |
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Abstract |
In this thesis we investigate the emergence of new phenomena in multigap superconductors and multicomponent Ginzburg-Landau theories in the presence of intraband and cross-band pairing. The first part contains a review of emergent phenomena in superconductors with only intraband pairing, in particular the mechanism behind gap resonances which are accompanied by Higgs and Leggett modes. Then we study the gap resonances induced by two-dimensional quantum confinement and describe its spatial profile using the Bogoliubov-de Gennes equations. In the second part we describe the conditions where the cross-band pair formation is feasible. Using the formalism of Green functions we obtain the equations governing the interplay between intraband and cross-band pairing. Also, we derived the Ginzburg-Landau equations considering both intraband and cross-band pairing. Finally, we describe the crossover between the intraband-dominated and crossband-dominated regimes. These two are delimited by a tendency towards a gapless state. When a magnetic field is applied close to the gapless state, we found new arrangements of vortices like square lattices, stripes, labyrinths or of vortex clusters. The experimental signatures and consequences of crosspairing are discussed for MgB2 and Ba0.6K0.4Fe2As2. |
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UA library record |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:165865 |
Serial |
7899 |
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Permanent link to this record |
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Author |
Seuntjens, D.; Carvajal Arroyo, J.M.; Molina, J.; Boon, N.; Vlaeminck, S.E. |
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Title |
Enabling partial nitritation/anammox on pre-treated sewage with IFAS : aeration and floc SRT control strategies limit nitrate production |
Type |
P3 Proceeding |
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Year |
2017 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
3 p.
T2 - 5th IWA Benelux Young Water Professional |
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Keywords |
P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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Additional Links |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:151116 |
Serial |
7901 |
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Permanent link to this record |
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Author |
Muia, L.M.; Van Grieken, R. |
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Title |
Energy-dispersive X-ray fluorescence analysis of geological materials in borax beads using Tertian's binary coefficient approach combined with internal standard addition |
Type |
A1 Journal article |
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Year |
1991 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
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Volume |
20 |
Issue |
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Pages |
179-183 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Series Volume |
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Edition |
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ISSN |
0049-8246 |
ISBN |
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Additional Links |
UA library record |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:662 |
Serial |
7903 |
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Permanent link to this record |
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Author |
Van Grieken, R.; Robberecht, H.; Shani, J.; Van Dyck, P.; Vos, L. |
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Title |
Energy-dispersive X-ray fluorescence for direct trace analysis of biomedical and environmental samples |
Type |
H3 Book chapter |
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Year |
1982 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
159-178
T2 - X-ray fluorescence (XRF and PIXE) in |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117485 |
Serial |
7904 |
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Permanent link to this record |
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Author |
Vanderborght, B.; Van Grieken, R. |
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Title |
Energy-dispersive X-ray fluorescence for trace metals analysis of water |
Type |
H3 Book chapter |
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Year |
1975 |
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Volume |
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Pages |
1-9
T2 - Nuclear techniques in environmental resea |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117461 |
Serial |
7905 |
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Author |
Seuntjens, D.; Bundervoet, B.L.M.; Mollen, H.; De Mulder, C.; Wypkema, E.; Verliefde, A.; Nopens, I.; Colsen, J.G.M.; Vlaeminck, S.E. |
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Title |
Energy efficient treatment of A-stage effluent : pilot-scale experiences with short-cut nitrogen removal |
Type |
P3 Proceeding |
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Year |
2015 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
10 p.
T2 - IWA Nutrient Removal and Recovery 2015: |
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Keywords |
P3 Proceeding; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL) |
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no |
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Call Number |
UA @ admin @ c:irua:151146 |
Serial |
7909 |
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Permanent link to this record |
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Author |
Vanderborght, B.M.; Van Grieken, R.E. |
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Title |
Enrichment of trace metals in water by adsorption on activated carbon |
Type |
A1 Journal article |
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Year |
1977 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
49 |
Issue |
2 |
Pages |
311-316 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Edition |
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ISSN |
0003-2700; 5206-882x |
ISBN |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:116513 |
Serial |
7923 |
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Permanent link to this record |
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Author |
Van Grieken, R.; Bresseleers, K.; Smits, J.; Vanderborght, B.; Vanderstappen, M. |
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Title |
Enrichment procedures for water analysis by X-ray energy spectrometry |
Type |
P3 Proceeding |
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Year |
1976 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA library record |
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Notes |
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no |
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Call Number |
UA @ admin @ c:irua:113634 |
Serial |
7924 |
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Permanent link to this record |
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Author |
Alexiades, V.; Autrique, D. |
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Title |
Enthalpy model for heating, melting, and vaporization in laser ablation |
Type |
A1 Journal article |
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Year |
2010 |
Publication |
Electronic journal of differential equations |
Abbreviated Journal |
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Volume |
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Issue |
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Pages |
1-13 |
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Keywords |
A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
Laser ablation is used in a growing number of applications in various areas including medicine, archaeology, chemistry, environmental and materials sciences. In this work the heat transfer and phase change phenomena during nanosecond laser ablation of a copper (Cu) target in a helium (He) background gas at atmospheric pressure are presented. An enthalpy model is outlined, which accounts for heating, melting, and vaporization of the target. As far as we know, this is the first model that connects the thermodynamics and underlying kinetics of this challenging phase change problem in a selfconsistent way. |
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000455668500001 |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1072-6691 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:190550 |
Serial |
7925 |
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Permanent link to this record |
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Author |
Xhoffer, C.; Van Grieken, R. |
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Title |
Environmental aerosol characterization by single particle analysis techniques |
Type |
H3 Book chapter |
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Year |
1993 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
207-245
T2 - Environmental particles; 2 / Buffle, |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:6267 |
Serial |
7926 |
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Author |
Delalieux, F.; Cardell, C.; Todorov, V.; Dekov, V.; Van Grieken, R. |
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Title |
Environmental conditions controlling the chemical weathering of the Madara Horseman monument, NE Bulgaria |
Type |
A1 Journal article |
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Year |
2001 |
Publication |
Journal of cultural heritage |
Abbreviated Journal |
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Volume |
2 |
Issue |
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Pages |
43-54 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Edition |
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ISSN |
1296-2074 |
ISBN |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:32822 |
Serial |
7927 |
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Permanent link to this record |
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Author |
Camuffo, D.; Van Grieken, R.; Busse, H.-J.; Sturaro, G.; Valentino, A.; Bernardi, A.; Blades, N.; Shooter, D.; Gysels, K.; Deutsch, F.; Wieser, M.; Kim, O.; Ulrych, U. |
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Title |
Environmental monitoring in four European museums |
Type |
A1 Journal article |
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Year |
2001 |
Publication |
Atmospheric environment : an international journal |
Abbreviated Journal |
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Volume |
35 |
Issue |
S1 |
Pages |
S127-S140 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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000169404000015 |
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Edition |
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ISSN |
1352-2310 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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no |
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Call Number |
UA @ admin @ c:irua:36082 |
Serial |
7928 |
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Permanent link to this record |
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Author |
Jambers, W.; Van Grieken, R.E. |
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Title |
Environmental problems |
Type |
H3 Book chapter |
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Year |
1997 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
803-819
T2 - Handbook of microscopy: applications |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:18789 |
Serial |
7929 |
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Permanent link to this record |
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Author |
Gielis, J. |
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Title |
Er bestaan geen absurde, irrationele, onregelmatige of onderling niet-onmeetbare meetkundige getallen |
Type |
A2 Journal article |
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Year |
2021 |
Publication |
Wiskunde en onderwijs |
Abbreviated Journal |
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Volume |
47 |
Issue |
188 |
Pages |
23-33 |
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Keywords |
A2 Journal article; Sustainable Energy, Air and Water Technology (DuEL) |
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ISSN |
2032-0485 |
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UA library record |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:183083 |
Serial |
7934 |
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Permanent link to this record |
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Author |
Vazquez, C.; Boeykens, S.; Palacios, O.; Caracciolo, N.; Kontozova-Deutsch, V.; Krupińska, B.; Van Grieken, R. |
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Title |
Estudio de la contaminacion del aire urbano en cuatro museos de Argentina |
Type |
H3 Book chapter |
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Year |
2013 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
271-282
T2 - Patrimonio cultural : la gestion, el |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Edition |
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ISBN |
978-987-1323-31-9 |
Additional Links |
UA library record |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:110908 |
Serial |
7936 |
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Permanent link to this record |
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Author |
Visser, W.J.; Van de Vyver, F.L.; Verbueken, A.H.; d'Haese, P.; Bekaert, A.B.; Van Grieken, R.E.; Duursma, S.A.; de Broe, M.E. |
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Title |
Evaluation of different techniques used to determine aluminium in patients with chronic renal failure |
Type |
P3 Proceeding |
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Year |
1985 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Keywords |
P3 Proceeding; Pathophysiology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
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UA library record |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:117496 |
Serial |
7938 |
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Permanent link to this record |
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Author |
Sankaran, K.; Swerts, J.; Carpenter, R.; Couet, S.; Garello, K.; Evans, R.F.L.; Rao, S.; Kim, W.; Kundu, S.; Crotti, D.; Kar, G.S.; Pourtois, G. |
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Title |
Evidence of magnetostrictive effects on STT-MRAM performance by atomistic and spin modeling |
Type |
P1 Proceeding |
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Year |
2018 |
Publication |
2018 Ieee International Electron Devices Meeting (iedm) |
Abbreviated Journal |
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Pages |
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Keywords |
P1 Proceeding; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
For the first time, we demonstrate, using an atomistic description of a 30nm diameter spin-transfer-torque magnetic random access memories (STT-MRAM), that the difference in mechanical properties of its sub-nanometer layers induces a high compressive strain in the magnetic tunnel junction (MTJ) and leads to a detrimental magnetostrictive effect. Our model explains the issues met in engineering the electrical and magnetic performances in scaled STT-MRAM devices. The resulting high compressive strain built in the stack, particularly in the MgO tunnel barrier (t-MgO), and its associated non-uniform atomic displacements, impacts on the quality of the MTJ interface and leads to strain relieve mechanisms such as surface roughness and adhesion issues. We illustrate that the strain gradient induced by the different materials and their thicknesses in the stacks has a negative impact on the tunnel magneto-resistance (TMR), on the magnetic nucleation process and on the STT-MRAM performance. |
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000459882300147 |
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Abbreviated Series Title |
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Edition |
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978-1-72811-987-8; 978-1-72811-987-8 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:158694 |
Serial |
7942 |
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Permanent link to this record |
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Author |
Cui, Z. |
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Title |
Experimental and theoretical study on SF6 degradation by packed-bed DBD plasma |
Type |
Doctoral thesis |
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Year |
2021 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Keywords |
Doctoral thesis; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
Sulfur hexafluoride (SF6), as a man-made gas, is widely used in power industry, semiconductor industry and metal-processing industry. However, SF6 is a greenhouse gas and its global warming potential is 23500 times that of CO2. Besides, SF6 is very stable, with a lifetime in the atmosphere for more than one thousand years. Under natural conditions, only the ultraviolet light can make it slowly decomposed. Thus, the emission of SF6 has a great threat to the environment. In recent years, with the development of our national economy, the use of SF6 increased dramatically. And 90% of the SF6 emissions come from the power industry. In the meantime, the emission of SF6 exists a ‘hysteresis effect’, as many of the SF6-gas insulation equipment will retire in next decades, the emission of SF6 may increase sharply, and this may put great pressure on the environment. Therefore, it’s necessary to make efforts in controlling and treating the SF6 emission. Among the SF6 abatement technologies, the non-thermal plasma(NTP) represented by the dielectric barrier discharge(DBD) can effectively degrade SF6 and is suitable for large-scale industry applications. However, its energy efficiency still gets room for improvement and this kind of method has a defect that it’s hard to regulate the degradation by-products. Therefore, this paper proposed the combination of the packed bed reactor and the DBD technology to form a packed DBD discharge system for SF6 degradation, so that to further improve the energy efficiency and regulate the selectivity of by-products. By experiment and simulation research, the following innovations have been achieved: (1) Based on the packed bed DBD platform, the power parameter and gas-phase parameters of SF6 degradation were studied. It was found that the discharge process was significantly enhanced with the addition of packing particles, and the discharge energy efficiency was improved. The increase of input voltage can obviously increase the degradation rate, but reduces the energy efficiency. The increase of SF6 initial concentration and gas flow rate can improve the energy efficiency, but reduce the degradation rate. Therefore, both degradation rate and energy efficiency should be considered in deciding basic experimental conditions. (2) Active gases, such as O2, H2O and NH3, could effectively promote the degradation rate of SF6, and changed the product selectivity. In our packed bed DBD system, O2 and H2O have the optimal concentration conditions, which are 2% and 1%, respectively. The addition of O2 can promote the generation of S-O-F products, and inhibit the selectivity of SO2, while the addition of H2O had the opposite effects. In addition, the synergistic degradation of NH3 and SF6 will produce solid products, such as NH3HF, NH4HF2 and elemental S. For gaseous products, the increase of NH3 will lead to the generation of SO2 in the final degradation products and inhibit the generation of S-O-F products. (3) Different kinds of packing materials have great impacts on the degradation system in the discharge parameters, degradation rate and energy efficiency, as well as the products distribution. In the experiment, we compared the degradation results in three systems: glass beads packing, γ-Al2O3 packing and no-packing system. The packing of glass beads effectively improved the discharge voltage amplitude and discharge power, while had a limited effect on the equivalent capacitance of the dielectric. Besides, γ-Al2O3 packing had little effect on voltage amplitude, but obviously increased the equivalent capacitance of the dielectric. Furthermore, the degradation rate and energy efficiency in γ-Al2O3 system was higher than that of glass bead system. For products selectivity, γ-Al2O3 system was more desirable, where S-O-F type of product selectivity was suppressed and the SO2 selectivity increased significantly. By contrast, the glass beads system hardly affected the product selectivity. This results are presumably due to the relatively high dielectric constant of γ-Al2O3 particles and γ-Al2O3 itself may act as a reactant or a catalyst participating in the degradation reactions. (4) The size and status of the packing particles also have significant effects on the degradation process. The systems packed with 1, 2 and 4mm γ-Al2O3 particles for SF6 degradation were compared, and the 2mm system had the best performance, which may because the 2mm system had a good balance between the active contact area and the gas residence time. In addition, the packing pellets suffered from a hydration process slightly reduced the discharge parameters in the γ-Al2O3 packing system and significantly reduced the degradation rate was, which may because the H2O molecules pre-occupied the active sites on the γ-Al2O3 surface and reduced the discharge process. (5) Based on density functional theory (DFT), the degradation process of SF6 in the packed bed DBD system was studied at atomic scale. It was found that the SF6 can occur a physical adsorption at AlⅢ active sites on γ-Al2O3 surface. The activation barrier for the first degradation step of SF6 on γ-Al2O3 surface is much lower than in gas phase, which proved that the SF6 molecule is activated on the γ-Al2O3 surface. In addition, the plasma may affect the γ-Al2O3 surface to generate excess electrons or external electric fields. This two effects can change the adsorbed SF6 molecules from physical adsorption to chemisorption, together with an obvious stretching of S-F bonds, indicating that the plasma surface effects prmote the activation and decomposition of SF6 molecules. Furthermore, the stepwise degradation process of SF6 on γ-Al2O3 surface were investigated. The influence of radicals produced by plasma on the degradation process was analyzed. It was found that via Eley–Rideal (ER) reactions, high-energy radicals could effectively reduce the activation barriers and promote the surface reactions. Finally, the degradation mechanism of SF6 molecules in the packed bed plasma system was summarized, which may provide a theoretical basis for the study of harmless degradation of SF6. Keywords: SF6; Packed Bed DBD; Discharge Parameters; Products Analysis; Degradation Mechanism |
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UA @ admin @ c:irua:180819 |
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