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Author |
de Maeyer-Worobiec, A.; Stefaniak, E.A.; Brooker, A.; Van Grieken, R. |
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Title |
Application of combined SEM/EDX and μ-Raman approaches for the chemical and structural characterisation of fine particulates |
Type |
P3 Proceeding |
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Year |
2007 |
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P3 Proceeding; Laboratory Experimental Medicine and Pediatrics (LEMP); AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:64633 |
Serial |
7470 |
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Author |
Akselsson, R.; Orsini, C.; Meinert, D.L.; Johansson, T.B.; Van Grieken, R.E.; Kaufmann, H.C.; Chapman, K.R.; Nelson, J.W.; Winchester, J.W. |
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Title |
Application of proton induced X-ray emission analysis to the St. Louis regional air pollution study |
Type |
P3 Proceeding |
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Year |
1976 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:113633 |
Serial |
7481 |
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Author |
Hoornaert, S.; Van Grieken, R. |
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Title |
Atmospheric aerosol particles: a review on sources, sinks and effects |
Type |
P3 Proceeding |
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Year |
2002 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:40622 |
Serial |
7514 |
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Author |
Van Grieken, R.; Torfs, K. |
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Title |
Atmospheric aerosols and deposition near historic buildings: chemistry, sources, interrelationships and relevance |
Type |
P3 Proceeding |
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Year |
1996 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:14662 |
Serial |
7515 |
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Author |
Bencs, L.; Horemans, B.; Van Grieken, R.; et al. |
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Title |
Atmospheric deposition fluxes to the Belgian marine waters originating from ship emissions : SHIPFLUX : final report |
Type |
Minutes and reports |
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Year |
2012 |
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Keywords |
Minutes and reports; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:107883 |
Serial |
7524 |
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Author |
Injuk, J.; Van Grieken, R. |
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Title |
Atmospheric inputs of heavy metals into the North Sea |
Type |
P3 Proceeding |
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Year |
1996 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:14669 |
Serial |
7526 |
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Author |
Kontozova-Deutsch, V.; Horemans, B.; Cardell, C.; Van Grieken, R. |
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Title |
Atmospheric pollution at the Alhambra monument, Granada, Spain: a preventive conservation study |
Type |
P3 Proceeding |
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Year |
2010 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:85522 |
Serial |
7530 |
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Author |
Van Grieken, R.; Artaxo, P.; Xhoffer, C. |
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Title |
Automated EPXMA of individual environmental particles |
Type |
P3 Proceeding |
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Year |
1992 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:2860 |
Serial |
7537 |
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Author |
Annegarn, H.J.; Van Grieken, R.E.; Winchester, J.W.; Sellschop, J.P.F.; von Blottnitz, F. |
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Title |
Background aerosol concentrations at the Namib-Atlantic interface |
Type |
P3 Proceeding |
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Year |
1979 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117465 |
Serial |
7546 |
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Author |
Caen, J.; Schalm, O.; Janssens, K. |
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Title |
Caractérisation historique et chimique des peintures en grisaille et du verre de vitrail dans l'oeuvre de J.-B. Capronnier (1814 – 1891) et J.-B. Bethune (1821 – 1894) |
Type |
P3 Proceeding |
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Year |
2000 |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; Art; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:112007 |
Serial |
7576 |
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Author |
Kontozova, V.; Deutsch, F.; Godoi, R.; Godoi, A.F.; Joos, P.; Van Grieken, R. |
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Title |
Characterisation of air pollutants in museum showcases |
Type |
P3 Proceeding |
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Year |
2002 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:39524 |
Serial |
7592 |
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Author |
Bernard, P.C.; Van Grieken, R.E.; Eisma, D. |
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Title |
Characterisation of individual suspension particles in the Ems estuary |
Type |
P3 Proceeding |
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Year |
1986 |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117514 |
Serial |
7599 |
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Author |
Oh, K.-Y.; Ro, C.-U.; Kim, H.K.; Van Grieken, R. |
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Title |
Characterization of aerosol particles at Seoul, Korea, using ultrathin window EPMA |
Type |
P3 Proceeding |
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Year |
2000 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Approved |
no |
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| |
Call Number |
UA @ admin @ c:irua:34106 |
Serial |
7612 |
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| Permanent link to this record |
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Author |
Oh, K.-Y.; Ro, C.-U.; Kim, H.K.; Kim, Y.-P.; Van Grieken, R. |
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| |
Title |
Characterization of aerosol particles collected at Kosan and 1100 Hill sites, Cheju Island, Korea, using ultrathin window EPMA |
Type |
P3 Proceeding |
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Year |
2000 |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Approved |
no |
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| |
Call Number |
UA @ admin @ c:irua:34105 |
Serial |
7613 |
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| Permanent link to this record |
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| |
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Author |
Ro, C.-U.; Oh, K.-Y.; Kim, H.K.; Chun, Y.; Van Grieken, R. |
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| |
Title |
Characterization of Asian dust using ultrathin window EPMA |
Type |
P3 Proceeding |
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Year |
1999 |
Publication |
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Abbreviated Journal |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Notes |
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Approved |
no |
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| |
Call Number |
UA @ admin @ c:irua:55576 |
Serial |
7617 |
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| Permanent link to this record |
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Author |
Roekens, E.; Leysen, L.; Van Grieken, R.; Komy, Z. |
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| |
Title |
Chemical characterisation of weathering crust and run-off water for a deteriorated limestone cathedral |
Type |
P3 Proceeding |
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Year |
1986 |
Publication |
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Abbreviated Journal |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117506 |
Serial |
7641 |
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| Permanent link to this record |
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Author |
Ravindra, K.; Stranger, M.; Van Grieken, R.; Sokhi, R.S. |
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| |
Title |
Chemical characterization and source apportionment of fine aerosols |
Type |
H3 Book chapter |
| |
Year |
2009 |
Publication |
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Abbreviated Journal |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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978-1-905313-64-8 |
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UA @ admin @ c:irua:97558 |
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7644 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
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Title |
Chemical characterization of airborne particulate matter above the North Sea |
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P3 Proceeding |
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1985 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA @ admin @ c:irua:117500 |
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7646 |
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Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
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Title |
Chemical characterization of individual aerosol particles from remote and polluted marine air |
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P3 Proceeding |
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1985 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117497 |
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7647 |
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Author |
Otten, P.; Rajsic, S.; Van Grieken, R. |
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Title |
Detection of ammomium compounds at the single particle level |
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P3 Proceeding |
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1987 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117520 |
Serial |
7773 |
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Author |
Schmeling, M.; Van Grieken, R. |
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Title |
Determination of light elements in marine aerosols by grazing-emission X-ray fluorescence |
Type |
P3 Proceeding |
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1999 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:27596 |
Serial |
7781 |
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Author |
Rutten, I.; Safdar, S.; Ven, K.; Daems, D.; Spasic, D.; Lammertyn, J. |
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Title |
A DNA nanotechnology toolbox for mix-and-match biosensor design |
Type |
P3 Proceeding |
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Year |
2019 |
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P3 Proceeding; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA @ admin @ c:irua:166107 |
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7819 |
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Author |
Janssen, E.; Kontozova-Deutsch, V.; Krupińska, B.; Moris, H.; Peckstadt, A.; van Bos, M.; Watteeuw, L.; Van Grieken, R. |
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Title |
Do gaseous pollutants and particulate matter endanger our world heritage? A study in the Museum Plantin-Moretus, Antwerp |
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P3 Proceeding |
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2010 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:85520 |
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7820 |
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Geerts, R.; Vandermoere, F.; Halet, D.; Joos, P.; Van Den Steen, K.; Van Meenen, E.; Blust, R.; Van Winckel, T.; Vlaeminck, S. |
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Title |
Drinking waste? An exploration of public support for wastewater reuse in Flanders |
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P3 Proceeding |
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Year |
2020 |
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P3 Proceeding; Sociology; Engineering sciences. Technology; Sustainable Energy, Air and Water Technology (DuEL); Centre for Research on Environmental and Social Change |
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Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:186706 |
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7825 |
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Author |
Keppens, E.; Roekens, E.; Van Grieken, R. |
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Title |
Effect of pollution on sandy limestones of a historical cathedral in Belgium |
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P3 Proceeding |
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1985 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117499 |
Serial |
7838 |
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Author |
Leysen, L.; Roekens, E.; Van Grieken, R. |
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Title |
Effecten van luchtverontreiniging op historische gebouwen |
Type |
P3 Proceeding |
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Year |
1987 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117518 |
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7839 |
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Author |
Xhoffer, C.; Jacob, W.; Van Grieken, R.; Broekaert, J.A.C.; Buseck, P. |
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Title |
Electron energy-loss spectroscopy and its application to individual particle analysis |
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P3 Proceeding |
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1992 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:2862 |
Serial |
7868 |
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Van Grieken, R.; Bresseleers, K.; Smits, J.; Vanderborght, B.; Vanderstappen, M. |
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Title |
Enrichment procedures for water analysis by X-ray energy spectrometry |
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P3 Proceeding |
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1976 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:113634 |
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7924 |
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Visser, W.J.; Van de Vyver, F.L.; Verbueken, A.H.; d'Haese, P.; Bekaert, A.B.; Van Grieken, R.E.; Duursma, S.A.; de Broe, M.E. |
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Title |
Evaluation of different techniques used to determine aluminium in patients with chronic renal failure |
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P3 Proceeding |
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1985 |
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P3 Proceeding; Pathophysiology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
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Call Number |
UA @ admin @ c:irua:117496 |
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7938 |
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Author |
Cui, Z. |
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Title |
Experimental and theoretical study on SF6 degradation by packed-bed DBD plasma |
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Doctoral thesis |
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Year |
2021 |
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Doctoral thesis; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
Sulfur hexafluoride (SF6), as a man-made gas, is widely used in power industry, semiconductor industry and metal-processing industry. However, SF6 is a greenhouse gas and its global warming potential is 23500 times that of CO2. Besides, SF6 is very stable, with a lifetime in the atmosphere for more than one thousand years. Under natural conditions, only the ultraviolet light can make it slowly decomposed. Thus, the emission of SF6 has a great threat to the environment. In recent years, with the development of our national economy, the use of SF6 increased dramatically. And 90% of the SF6 emissions come from the power industry. In the meantime, the emission of SF6 exists a ‘hysteresis effect’, as many of the SF6-gas insulation equipment will retire in next decades, the emission of SF6 may increase sharply, and this may put great pressure on the environment. Therefore, it’s necessary to make efforts in controlling and treating the SF6 emission. Among the SF6 abatement technologies, the non-thermal plasma(NTP) represented by the dielectric barrier discharge(DBD) can effectively degrade SF6 and is suitable for large-scale industry applications. However, its energy efficiency still gets room for improvement and this kind of method has a defect that it’s hard to regulate the degradation by-products. Therefore, this paper proposed the combination of the packed bed reactor and the DBD technology to form a packed DBD discharge system for SF6 degradation, so that to further improve the energy efficiency and regulate the selectivity of by-products. By experiment and simulation research, the following innovations have been achieved: (1) Based on the packed bed DBD platform, the power parameter and gas-phase parameters of SF6 degradation were studied. It was found that the discharge process was significantly enhanced with the addition of packing particles, and the discharge energy efficiency was improved. The increase of input voltage can obviously increase the degradation rate, but reduces the energy efficiency. The increase of SF6 initial concentration and gas flow rate can improve the energy efficiency, but reduce the degradation rate. Therefore, both degradation rate and energy efficiency should be considered in deciding basic experimental conditions. (2) Active gases, such as O2, H2O and NH3, could effectively promote the degradation rate of SF6, and changed the product selectivity. In our packed bed DBD system, O2 and H2O have the optimal concentration conditions, which are 2% and 1%, respectively. The addition of O2 can promote the generation of S-O-F products, and inhibit the selectivity of SO2, while the addition of H2O had the opposite effects. In addition, the synergistic degradation of NH3 and SF6 will produce solid products, such as NH3HF, NH4HF2 and elemental S. For gaseous products, the increase of NH3 will lead to the generation of SO2 in the final degradation products and inhibit the generation of S-O-F products. (3) Different kinds of packing materials have great impacts on the degradation system in the discharge parameters, degradation rate and energy efficiency, as well as the products distribution. In the experiment, we compared the degradation results in three systems: glass beads packing, γ-Al2O3 packing and no-packing system. The packing of glass beads effectively improved the discharge voltage amplitude and discharge power, while had a limited effect on the equivalent capacitance of the dielectric. Besides, γ-Al2O3 packing had little effect on voltage amplitude, but obviously increased the equivalent capacitance of the dielectric. Furthermore, the degradation rate and energy efficiency in γ-Al2O3 system was higher than that of glass bead system. For products selectivity, γ-Al2O3 system was more desirable, where S-O-F type of product selectivity was suppressed and the SO2 selectivity increased significantly. By contrast, the glass beads system hardly affected the product selectivity. This results are presumably due to the relatively high dielectric constant of γ-Al2O3 particles and γ-Al2O3 itself may act as a reactant or a catalyst participating in the degradation reactions. (4) The size and status of the packing particles also have significant effects on the degradation process. The systems packed with 1, 2 and 4mm γ-Al2O3 particles for SF6 degradation were compared, and the 2mm system had the best performance, which may because the 2mm system had a good balance between the active contact area and the gas residence time. In addition, the packing pellets suffered from a hydration process slightly reduced the discharge parameters in the γ-Al2O3 packing system and significantly reduced the degradation rate was, which may because the H2O molecules pre-occupied the active sites on the γ-Al2O3 surface and reduced the discharge process. (5) Based on density functional theory (DFT), the degradation process of SF6 in the packed bed DBD system was studied at atomic scale. It was found that the SF6 can occur a physical adsorption at AlⅢ active sites on γ-Al2O3 surface. The activation barrier for the first degradation step of SF6 on γ-Al2O3 surface is much lower than in gas phase, which proved that the SF6 molecule is activated on the γ-Al2O3 surface. In addition, the plasma may affect the γ-Al2O3 surface to generate excess electrons or external electric fields. This two effects can change the adsorbed SF6 molecules from physical adsorption to chemisorption, together with an obvious stretching of S-F bonds, indicating that the plasma surface effects prmote the activation and decomposition of SF6 molecules. Furthermore, the stepwise degradation process of SF6 on γ-Al2O3 surface were investigated. The influence of radicals produced by plasma on the degradation process was analyzed. It was found that via Eley–Rideal (ER) reactions, high-energy radicals could effectively reduce the activation barriers and promote the surface reactions. Finally, the degradation mechanism of SF6 molecules in the packed bed plasma system was summarized, which may provide a theoretical basis for the study of harmless degradation of SF6. Keywords: SF6; Packed Bed DBD; Discharge Parameters; Products Analysis; Degradation Mechanism |
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Notes |
|
Approved |
Most recent IF: NA |
|
| |
Call Number |
UA @ admin @ c:irua:180819 |
Serial |
7946 |
|
| Permanent link to this record |
