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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Torfs, K.M.; Van Grieken, R.E.; Buzek, F. |
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Title |
Use of stable isotope measurements to evaluate the origin of suphur in gypsum layers on limestone buildings |
Type |
A1 Journal article |
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Year |
1997 |
Publication |
Environmental science and technology |
Abbreviated Journal |
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Volume |
31 |
Issue |
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Pages |
2650-2655 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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ISSN |
0013-936x; 1520-5851 |
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no |
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Call Number |
UA @ admin @ c:irua:18784 |
Serial |
8724 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.; Braun, T.; Van Dyck, P.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Heterogeneity effects in direct XRF analysis of traces of heavy metals preconcentrated on polyurethane foam sorbents |
Type |
A1 Journal article |
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Year |
1986 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
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Volume |
15 |
Issue |
1 |
Pages |
7-11 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Trace amounts of heavy metals were preconcentrated on discs of polyurethane (PU) foam loaded with ammonium diethyldithiocarbamate (DDTC), to increase the sensitivity of XRF. Since the diameter of the cavities in the open-cell PU foams reaches 30300 μm, considerable heterogeneity effects might occur, which could reduce the accuracy of the method. The possible systematic error introduced by considering the sample to be homogeneous is calculated using the Berry et al. model. The calculations show that the underestimation of the absorption correction factor when considering the sample as being homogeneous is less than 2% for high-Z elements when the sample thickness is at least 2 mm. The detection limits are also around the minima for this thickness. |
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A1986AYN6000002 |
Publication Date |
2005-05-28 |
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ISSN |
0049-8246 |
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UA library record; WoS full record; WoS citing articles |
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no |
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Call Number |
UA @ admin @ c:irua:116488 |
Serial |
8030 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.; Labar, J.; Schmeling, M.; Van Grieken, R. |
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Title |
X-ray spectrometry |
Type |
A1 Journal article |
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Year |
1998 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
70 |
Issue |
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Pages |
495r-517r |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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000074161100020 |
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0003-2700; 5206-882x |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:20967 |
Serial |
8776 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.; Sandor, S.; Xhoffer, C.; Van Grieken, R.; Meszaros, E.; Molnar, A. |
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Title |
Single particle analysis of Hungarian background aerosol |
Type |
A3 Journal article |
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Year |
1992 |
Publication |
Idojaras: quarterly journal of the Hungarian Meteorological Service |
Abbreviated Journal |
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Volume |
96 |
Issue |
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Pages |
223-233 |
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Keywords |
A3 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:2847 |
Serial |
8532 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.; Szandor, S.; Xhoffer, C.; Van Grieken, R. |
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Title |
Source apportionment of individual aerosol particles at Hungarian background stations |
Type |
H3 Book chapter |
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Year |
1993 |
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Abbreviated Journal |
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Pages |
32-331
T2 - Photo-oxidants: precursors and product |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:6265 |
Serial |
8559 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.; Van Dyck, P.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Heterogeneity effects in direct X-ray fluorescence analysis of hair |
Type |
A1 Journal article |
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Year |
1984 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
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Volume |
13 |
Issue |
1 |
Pages |
27-32 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
The methodology of direct hair analysis by energy-dispersive x-ray fluorescence was studied. The effect on the XRF result of having a non-homogeneous radial distribution of the analyte in a single hair strand and the macroscopic effects in a bundle of hairs were calculated to evaluate possible systematic errors. The detection limits were mapped as a function of the target thickness and surface fraction. It appeared that a 10 mg cm−2 sample thickness, i. e. a target with about four layers of hair strands, is recommended. The standard deviation of this simple direct analytical method is 619% for some important elements. Discrepancies with neutron activation analysis had a mean value of around 15%. About twelve elements can be determined simultaneously on a routine basis. |
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Wos |
A1984SB70200004 |
Publication Date |
2005-05-28 |
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ISSN |
0049-8246 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:116485 |
Serial |
8029 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.B.; Labar, J.; Injuk, J.; Van Grieken, R.E. |
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Title |
X-ray spectrometry |
Type |
A1 Journal article |
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Year |
1996 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
R68 |
Issue |
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Pages |
467-485 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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ISSN |
0003-2700; 5206-882x |
ISBN |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:14650 |
Serial |
8777 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Török, S.B.; Van Grieken, R.E. |
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Title |
X-ray spectrometry |
Type |
A1 Journal article |
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Year |
1992 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
64r |
Issue |
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Pages |
180-196 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
A1992HZ51800011 |
Publication Date |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Issue |
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Edition |
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ISSN |
0003-2700; 5206-882x |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Open Access |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:2823 |
Serial |
8778 |
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Trashin, S.; De Jong, M.; Breugelmans, T.; Pilehvar, S.; De Wael, K. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Label-free impedance aptasensor for major peanut allergen Ara h 1 |
Type |
A1 Journal article |
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Year |
2015 |
Publication |
Electroanalysis |
Abbreviated Journal |
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Volume |
27 |
Issue |
1 |
Pages |
32-37 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Applied Electrochemistry & Catalysis (ELCAT) |
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Abstract |
The peanut allergen Ara h 1 belonging to the vicilin family of seed storage proteins is known to be a suitable marker for peanut detection in foods. In the present work, we suggest an electrochemical detection of Ara h 1 using a recently selected 80-base DNA aptamer. The detection strategy relies on insulation effect of a bulky protein captured by an immobilized aptamer. The electrodes were modified by the aptamer and characterized using electrochemical impedance spectroscopy (EIS). The aptamer surface density and analytical parameters of the calibration curves for Ara h 1 were compared with the system prepared with thrombin binding aptamer (TBA) and operated in the same conditions. |
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000347838300004 |
Publication Date |
2014-10-13 |
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UA library record; WoS full record; WoS citing articles |
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Times cited |
10 |
Open Access |
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Notes |
; ST greatly appreciates the Research Council University of Antwerp (IWS BOF UA) for funding the post-doctoral fellowship. ; |
Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:119442 |
Serial |
5686 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Treiger, B.; Bondarenko, I.; van Espen, P.; Van Grieken, R.; Adams, F. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Classification of mineral particles by nonlinear mapping of electron microprobe energy-dispersive X-ray spectra |
Type |
A1 Journal article |
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Year |
1994 |
Publication |
The analyst |
Abbreviated Journal |
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Volume |
119 |
Issue |
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Pages |
971-974 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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Wos |
A1994NR76500037 |
Publication Date |
2004-03-24 |
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UA library record; WoS full record; WoS citing articles |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:8918 |
Serial |
7669 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Treiger, B.; Bondarenko, I.; van Malderen, H.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Elucidating the composition of atmospheric aerosols through the combined hierarchical, non-hierarchical and fuzzy clustering of large electron probe microanalysis data sets |
Type |
A1 Journal article |
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Year |
1995 |
Publication |
Analytica chimica acta |
Abbreviated Journal |
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Volume |
317 |
Issue |
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Pages |
33-51 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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A1995TP42200003 |
Publication Date |
2003-04-23 |
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ISSN |
0003-2670; 1873-4324 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Open Access |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:12355 |
Serial |
7897 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Treiger, B.; Bondarenko, I.; van Malderen, H.; Van Grieken, R. |
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Title |
Studying the composition of atmospheric aerosols through the joint application of hierarchical, non-hierarchical and fuzzy clustering to EPXMA data sets |
Type |
P3 Proceeding |
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Year |
1996 |
Publication |
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Abbreviated Journal |
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Pages |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:14661 |
Serial |
8611 |
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Treiger, B.; Injuk, J.; Bondarenko, I.; van Espen, P.; Van Grieken, R.; Breitenbach, L.; Wätjen, U. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Non-linear mapping of microbeam proton-induced X-ray emission data for source identification of North Sea aerosols |
Type |
A1 Journal article |
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Year |
1994 |
Publication |
Spectrochimica acta: part B : atomic spectroscopy |
Abbreviated Journal |
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Volume |
49 |
Issue |
4 |
Pages |
345-353 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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A1994NM41200004 |
Publication Date |
2003-04-25 |
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Abbreviated Series Title |
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ISSN |
0584-8547; 1873-3565 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Open Access |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:9500 |
Serial |
8314 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Treiger, B.; van Malderen, H.; Bondarenko, I.; van Espen, P.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Studying aerosol samples by non-linear mapping of electron probe microanalysis data |
Type |
A1 Journal article |
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Year |
1993 |
Publication |
Analytica chimica acta |
Abbreviated Journal |
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Volume |
284 |
Issue |
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Pages |
119-124 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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A1993MR27600014 |
Publication Date |
2002-07-25 |
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Abbreviated Series Title |
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Series Volume |
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Edition |
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ISSN |
0003-2670; 1873-4324 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Impact Factor |
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Times cited |
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Open Access |
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Notes |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:6224 |
Serial |
8610 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Trenchev, G. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Computational modelling of atmospheric DC discharges for CO2 conversion |
Type |
Doctoral thesis |
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Year |
2019 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
206 p. |
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Keywords |
Doctoral thesis; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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UA library record |
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Open Access |
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Notes |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:163986 |
Serial |
6290 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Trincavelli, J.; Montoro, S.; van Espen, P.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
M\alpha/L\alpha intensity ratios for Ta, W, Pt, Au, Pb and Bi for electron energies in the 11-40 keV range |
Type |
A1 Journal article |
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Year |
1993 |
Publication |
X-ray spectrometry |
Abbreviated Journal |
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Volume |
22 |
Issue |
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Pages |
372-376 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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Abstract |
Both energy- and wavelength-dispersive systems were used to obtain Malpha/Lalpha intensity ratios for Ta, W, Pt, Au, Pb and Bi at various overvoltages. A table of these ratios corrected for matrix absorption and detector efficiency is presented, in addition to an interpolatory function of Malpha/Lalpha generated ratios vs. overvoltage, for each element. In addition, three different ZAF correction models were used to predict both detected and generated ratios. Finally, experimental Mbeta/Malpha ratios measured at different overvoltages are presented for the six elements considered. |
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A1993MB01200008 |
Publication Date |
2005-05-28 |
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ISSN |
0049-8246 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Times cited |
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Open Access |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:6221 |
Serial |
8649 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Trincavelli, J.; Montoro, S.; Van Grieken, R.; van Espen, P. |
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Title |
Prediction of Mα/Lα intensity ratios and the use in the spectra evaluation |
Type |
P3 Proceeding |
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Year |
1992 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
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Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:2863 |
Serial |
8405 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Trincavelli, J.C.; Van Grieken, R. |
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Title |
Analisis cuantitativo sin estandares de particulas individuales mediante microsonda de electrones |
Type |
H3 Book chapter |
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Year |
1996 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
273-278
T2 - Avances en analisis por tecnicas en r |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:14678 |
Serial |
7439 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Truong, B.; Siegert, K.; Lin, A.; Miller, V.; Krebs, F.C. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Apical application of nanosecond-pulsed dielectric barrier discharge plasma causes the basolateral release of adenosine triphosphate as a damage-associated molecular pattern from polarized HaCaT cells |
Type |
A1 Journal article |
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Year |
2017 |
Publication |
Plasma medicine |
Abbreviated Journal |
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Volume |
7 |
Issue |
2 |
Pages |
117-131 |
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Keywords |
A1 Journal article; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
Promising biomedical uses for nonthermal plasma (NTP) in the fields of regenerative medicine, cancer therapy, and vaccine delivery involve the noninvasive application of uniform nonequilibrium plasma (including dielectric barrier discharge plasma) to living skin. Whereas most investigations have focused on achieving desired therapeutic outcomes, fewer studies have examined the mechanisms and pathways by which epithelial cells respond to NTP exposure. Using a transwell apical-basolateral-chambered system to culture the human keratinocyte HaCaT cell line, in vitro experiments were performed to demonstrate the effects of nanosecond-pulsed dielectric barrier discharge (nsDBD) plasma on polarized epithelial cell viability, monolayer permeability, intracellular oxidative stress, and the release of adenosine triphosphate (ATP). Application of nsDBD plasma at 60 Hz or below had minimal or no effect on HaCaT monolayer viability or permeability. nsDBD plasma exposure did, however, result in frequency-dependent reductions in intracellular glutathione (indicating direct induction of oxidative stress by nsDBD plasma) and increased extracellular ATP concentrations in the ba-solateral (subepithelial) media, which are indicators of cellular stress and an NTP-induced inflammatory response. These studies provide new insights into nsDBD plasma-induced inflammation and local innate immune responses initiated by polarized epithelial tissues. |
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2017-02-24 |
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UA library record |
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no |
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Call Number |
UA @ admin @ c:irua:155656 |
Serial |
7465 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Truta, F.; Drăgan, A.-M.; Tertis, M.; Parrilla, M.; Slosse, A.; Van Durme, F.; De Wael, K.; Cristea, C. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Electrochemical rapid detection of methamphetamine from confiscated samples using a graphene-based printed platform |
Type |
A1 Journal article |
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Year |
2023 |
Publication |
Sensors |
Abbreviated Journal |
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Volume |
23 |
Issue |
13 |
Pages |
6193-18 |
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Keywords |
A1 Journal article; Antwerp Electrochemical and Analytical Sciences Lab (A-Sense Lab) |
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Abstract |
Methamphetamine (MAP) is a highly addictive and illegal stimulant drug that has a significant impact on the central nervous system. Its detection in biological and street samples is crucial for various organizations involved in forensic medicine, anti-drug efforts, and clinical diagnosis. In recent years, nanotechnology and nanomaterials have played a significant role in the development of analytical sensors for MAP detection. In this study, a fast, simple, and cost-effective electrochemical sensor is presented that is used for the sensitive detection of MAP in confiscated street samples with a complex matrix. The optimized screen-printed sensor based on a carbon working electrode modified with graphene demonstrated an excellent limit of detection, good sensitivity, and a wide dynamic range (1–500 μM) for the target illicit drug both for standard solutions and real samples (seized samples, tap water, and wastewater samples). It can detect MAP at concentrations as low as 300 nM in real samples. This limit of detection is suitable for the rapid preliminary screening of suspicious samples in customs, ports, airports, and on the street. Furthermore, the sensor exhibits a good recovery rate, indicating its reliability and repeatability. This quality is crucial for ensuring consistent and accurate results during screening processes. |
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Wos |
001033277900001 |
Publication Date |
2023-07-07 |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1424-8220 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Impact Factor |
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Times cited |
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Open Access |
OpenAccess |
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Notes |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:198181 |
Serial |
8857 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tschulkow, M. |
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Title |
A techno-environmental economic assessment of a lignin-first biorefinery : a dynamic and prospective framework for emerging technologies |
Type |
Doctoral thesis |
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Year |
2022 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
175 p. |
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Keywords |
Doctoral thesis; Engineering sciences. Technology; Engineering Management (ENM) |
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Abstract |
Novel emerging biorefinery technologies have gained interest and have the potential to tackle several sustainability challenges in our society. A lignin-first biorefinery process – reductive catalytic fractionation (RCF) – is currently under development with the aim to process wood into high-value end-products that replace highly polluting fossil oil-based products. However, such emerging technologies are not matured yet, holding a certain degree of technological, economic, and environmental uncertainty. Hence, an appropriate assessment method is required to assess techno-economic feasibility and environmental impacts of emerging uncertain technologies (e.g lignin-first RCF process). This dissertation aims to develop an integrated techno-environmental economic assessment framework to assess emerging technologies dynamically and prospectively from economic and environmental points of view. First, a techno-economic assessment (TEA) is performed to assess the economic feasibility and the most influential economic and technological parameters of the lignin-first RCF biorefinery taking the whole wood value chain into account. By making the relations across the wood value chain, the scale of the biorefinery, wood species, and output prices highly determine the economic feasibility. The economic feasibility can be reached by a sufficient capacity level which depends on wood species-specific conditions. Also, waste wood proves to be the most profitable feedstock in comparison to virgin wood. Second, an analytical real options analysis (ROA) is performed taking two correlated market uncertainties and the value of flexibility into account to identify the optimal investment decision in an RCF biorefinery. Two different investment options, separated and united investments in harvesting equipment and RCF biorefinery, are analyzed. In both scenarios, market uncertainty postpones the investment. When both investment decisions are united, the probability of investment increases in comparison to separated investments. The study reveals that RCF has the potential to stimulate investments within the wood value chain. Third, a consequential life cycle assessment (LCA) is performed to assess the carbon emissions and the environmental consequences of the lignin-first RCF process and its products. The study reveals that at the current stage RCF products have higher carbon emissions than their alternative counterparts. Several options to improve the environmental performance are discussed such as different RCF technology configurations, targeting different RCF products with the ability to replace higher polluting alternative counterparts on the markets. Other discussion points such as transportation type and the distance, (in-)direct land-use change, the use stage and disposal stages implications, and a more comprehensive environmental view of the RCF products, show the potential to improve the environmental performance of the RCF technology. Overall, the study shows that the RCF process can be environmentally desirable if the appropriate RCF configuration and products are chosen. Finally, the above-mentioned methods – techno-economic assessment, analytical real options analysis, and consequential life cycle assessment – are uniquely integrated within the newly developed integrated assessment framework. The framework has the aim to complement the shortcomings and combine the advantages of all three methods. The framework assesses emerging technologies to give predictive insights about the time-specific economic and environmental performance under the newly developed three threshold conditions: technological readiness, economic feasibility, and environmental desirability. The developed integrated assessment framework assesses dynamically and prospectively the RCF biorefinery implementation under Belgian conditions. It reveals that the economic feasibility increases and carbon emissions decrease over time. The RCF biorefinery fulfills all three threshold conditions – technological readiness, economic feasibility, and environmental desirability – consecutively. The newly developed integrated assessment framework offers decision support to several stakeholders of emerging technologies starting from low technology readiness level (TRL). Practitioners such as the technology developers, researchers, and policymakers can use the framework to evaluate emerging technologies that deal with high levels of technological, economic, and environmental uncertainties. The framework assesses emerging technologies on a detailed level to give decision-makers in-depth insights into the intertwined nature of the technological, economic, and environmental dimensions. It offers insights into the expected time-specific economic and environmental performances, potential, and challenges of the emerging technology to further improve the technology and direct R&Ds along the right path. |
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UA library record |
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Notes |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:188968 |
Serial |
7369 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsonev, I.; Ahmadi Eshtehardi, H.; Delplancke, M.-P.; Bogaerts, A. |
![goto web page (via DOI) doi](http://nano.uantwerpen.be/nanorefs/img/doi.gif)
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Title |
Importance of geometric effects in scaling up energy-efficient plasma-based nitrogen fixation |
Type |
A1 Journal article |
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Year |
2024 |
Publication |
Sustainable energy & fuels |
Abbreviated Journal |
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Volume |
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Issue |
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Pages |
1-19 |
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Keywords |
A1 Journal article; Engineering sciences. Technology; Plasma Lab for Applications in Sustainability and Medicine – Antwerp (PLASMANT) |
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Abstract |
Despite the recent promising potential of plasma-based nitrogen fixation, the technology faces significant challenges in efficient upscaling. To tackle this challenge, we investigate two reactors, i.e., a small one, operating in a flow rate range of 5-20 ln min-1 and current range of 200-500 mA, and a larger one, operating at higher flow rate (100-300 ln min-1) and current (400-1000 mA). Both reactors operate in a pin-to-pin configuration and are powered by direct current (DC) from the same power supply unit, to allow easy comparison and evaluate the effect of upscaling. In the small reactor, we achieve the lowest energy cost (EC) of 2.8 MJ mol-1, for a NOx concentration of 1.72%, at a flow rate of 20 ln min-1, yielding a production rate (PR) of 33 g h-1. These values are obtained in air; in oxygen-enriched air, the results are typically better, at the cost of producing oxygen-enriched air. In the large reactor, the higher flow rates reduce the NOx concentration due to lower SEI, while maintaining a similar EC. This stresses the important effect of the geometrical configuration of the arc, which is typically concentrated in the center of the reactor, resulting in limited coverage of the reacting gas flow, and this is identified as the limiting factor for upscaling. However, our experiments reveal that by changing the reactor configuration, and thus the plasma geometry and power deposition mechanisms, the amount of gas treated by the plasma can be enhanced, leading to successful upscaling. To obtain more insights in our experiments, we performed thermodynamic equilibrium calculations. First of all, they show that our measured lowest EC closely aligns with the calculated minimum thermodynamic equilibrium at atmospheric pressure. In addition, they reveal that the limited NOx production in the large reactor results from the contracted nature of the plasma. To solve this limitation, we let the large reactor operate in so-called torch configuration. Indeed, the latter enhances the NOx concentrations compared to the pin-to-pin configuration, yielding a PR of 80 g h-1 at an EC of 2.9 MJ mol-1 and NOx concentration of 0.31%. This illustrates the importance of reactor design in upscaling. With the focus on feasibility evaluation of scaling-up plasma-based nitrogen fixation by combined experiments and thermodynamic modelling, we aim to tackle the challenge of design and development of an energy-efficient and scaled-up plasma reactor. |
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Wos |
001203657700001 |
Publication Date |
2024-04-11 |
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UA library record; WoS full record |
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Approved |
Most recent IF: NA |
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Call Number |
UA @ admin @ c:irua:205435 |
Serial |
9155 |
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Permanent link to this record |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Huisman, M.; Spolnik, Z.; Wagatsuma, K.; Mori, Y.; Van Grieken, R.E.; Vis, R.D. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Comparison of grazing-exit particle-induced X-ray emission with other related methods |
Type |
A1 Journal article |
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Year |
2000 |
Publication |
Spectrochimica acta: part B : atomic spectroscopy |
Abbreviated Journal |
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Volume |
55 |
Issue |
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Pages |
1009-1016 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
000088353100030 |
Publication Date |
2002-07-25 |
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ISSN |
0584-8547; 1873-3565 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:31671 |
Serial |
7692 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Injuk, J.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
X-ray spectrometry: recent technological advances |
Type |
ME1 Book as editor or co-editor |
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Year |
2004 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
616 p. |
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Keywords |
ME1 Book as editor or co-editor; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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0-471-48640-x |
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UA library record |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:43876 |
Serial |
8786 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Nullens, R.; Wagatsuma, K.; Van Grieken, R.E. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Elemental x-ray images obtained by grazing-exit electron probe microanalysis (GE-EPMA) |
Type |
A1 Journal article |
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Year |
1999 |
Publication |
Journal of analytical atomic spectrometry |
Abbreviated Journal |
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Volume |
14 |
Issue |
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Pages |
1711-1713 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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000083208000009 |
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2002-07-26 |
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0267-9477 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Approved |
no |
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Call Number |
UA @ admin @ c:irua:34103 |
Serial |
7896 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Sato, T.; Wagatsuma, K.; Claes, M.; Van Grieken, R. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Preliminary experiment of total reflection x-ray fluorescence using two glancing x-ray beams excitation |
Type |
A1 Journal article |
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Year |
1999 |
Publication |
The review of scientific instruments |
Abbreviated Journal |
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Volume |
70 |
Issue |
3 |
Pages |
1621-1623 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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000079012100006 |
Publication Date |
2002-07-26 |
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0034-6748 |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:23184 |
Serial |
8407 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Spolnik, Z.; Wagatsuma, K.; Nullens, R.; Van Grieken, R.E. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Detection limits of grazing-exit EPMA for particle analysis |
Type |
A1 Journal article |
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Year |
2000 |
Publication |
Microchimica acta |
Abbreviated Journal |
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Volume |
132 |
Issue |
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Pages |
357-360 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
000086810800030 |
Publication Date |
2003-02-12 |
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ISSN |
0026-3672; 1436-5073 |
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UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:27593 |
Serial |
7771 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Spolnik, Z.; Wagatsuma, K.; Nullens, R.; Van Grieken, R.E. |
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Title |
Preliminary experiments on grazing-exit electron probe microanalysis (GE-EPMA) |
Type |
P1 Proceeding |
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Year |
1999 |
Publication |
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Abbreviated Journal |
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Volume |
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Issue |
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Pages |
119-122
T2 - Electron Microscopy and Analysis 1999 |
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Keywords |
P1 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
000088782800027 |
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UA library record; WoS full record |
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Call Number |
UA @ admin @ c:irua:27602 |
Serial |
8408 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Spolnik, Z.; Wagatsuma, K.; Van Grieken, R.E.; Vis, R.D. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Grazing-exit particle-induced X-ray emission analysis with extremely low background |
Type |
A1 Journal article |
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Year |
1999 |
Publication |
Analytical chemistry |
Abbreviated Journal |
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Volume |
71 |
Issue |
22 |
Pages |
5033-5036 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Wos |
000083647100004 |
Publication Date |
2002-07-26 |
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ISSN |
0003-2700; 5206-882x |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Call Number |
UA @ admin @ c:irua:27588 |
Serial |
8010 |
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Author ![sorted by Author field, ascending order (up)](img/sort_asc.gif) |
Tsuji, K.; Spolnik, Z.; Wagatsuma, K.; Zhang, J.; Van Grieken, R.E. |
![find record details (via OpenURL) openurl](img/xref.gif)
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Title |
Enhancement of electron-induced X-ray intensity for single particles under grazing-exit conditions |
Type |
A1 Journal article |
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Year |
1999 |
Publication |
Spectrochimica acta: part B : atomic spectroscopy |
Abbreviated Journal |
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Volume |
54 |
Issue |
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Pages |
1243-1251 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
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Place of Publication |
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Wos |
000082048700010 |
Publication Date |
2002-07-26 |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0584-8547; 1873-3565 |
ISBN |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Open Access |
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Call Number |
UA @ admin @ c:irua:27583 |
Serial |
7917 |
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Permanent link to this record |