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Author (down) Chin, C.–M.; Battle, P.D.; Hunter, E.C.; Avdeev, M.; Hendrickx, M.; Hadermann, J.
  Title Magnetic properties of La3Ni2Sb Ta Nb1––O9; from relaxor to spin glass Type A1 Journal article
  Year 2019 Publication Journal of solid state chemistry (Print) Abbreviated Journal Journal of Solid State Chemistry
  Volume 273 Issue Pages 175-185
  Keywords A1 Journal article; Electron microscopy for materials research (EMAT)
  Abstract Neutron diffraction experiments conducted at 5 K in a magnetic field 0 < H/kOe < 50 have shown that the monoclinic perovskite La3Ni2TaO9 behaves as a relaxor ferromagnet. Compositions in the series La3Ni2SbxTayNb1–x–yO9 have been synthesized in polycrystalline form. Electron microscopy, X–ray diffraction and neutron diffraction have shown that the solid solutions are largely homogeneous and monophasic. Magnetometry and neutron diffraction have shown that the relaxor magnetisation persists in low fields when x + y = 1 but is rapidly diminished by the introduction of niobium. This change in magnetic behaviour is ascribed to the differences in the d–orbital energies of Sb5+, Nb5+ and Ta5+.
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  Corporate Author Thesis
  Publisher Place of Publication Editor
  Language Wos 000466261100026 Publication Date 2019-03-02
  Series Editor Series Title Abbreviated Series Title
  Series Volume Series Issue Edition
  ISSN 0022-4596 ISBN Additional Links UA library record; WoS full record; WoS citing articles
  Impact Factor Times cited Open Access
  Notes We thank EPSRC for funding through grant EP/M0189541. CMC thanks the Croucher Foundation and the University of Oxford for the award of a graduate scholarship. Approved no
  Call Number EMAT @ emat @c:irua:166445 Serial 6346
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