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Buczyńska, A.J.; Krata, A.; Van Grieken, R.; Brown, A.; Polezer, G.; De Wael, K.; Potgieter-Vermaak, S. |
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Title |
Composition of PM2.5 and PM1 on high and low pollution event days and its relation to indoor air quality in a home for the elderly |
Type |
A1 Journal article |
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Year |
2014 |
Publication |
The science of the total environment |
Abbreviated Journal |
Sci Total Environ |
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Volume |
490 |
Issue |
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Pages |
134-143 |
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Keywords |
A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Abstract |
Many studies probing the link between air quality and health have pointed towards associations between particulate matter (PM) exposure and decreased lung function, aggravation of respiratory diseases like asthma, premature death and increased hospitalisation admissions for the elderly and individuals with cardiopulmonary diseases. Of recent, it is believed that the chemical composition and physical properties of PM may contribute significantly to these adverse health effects. As part of a Belgian Science Policy project (Health effects of particulate matter in relation to physicalchemical characteristics and meteorology), the chemical composition (elemental and ionic compositions) and physical properties (PM mass concentrations) of PM were investigated, indoors and outdoors of old age homes in Antwerp. The case reported here specifically relates to high versus normal/low pollution event periods. PM mass concentrations for PM1 and PM2.5 fractions were determined gravimetrically after collection via impaction. These same samples were hence analysed by EDXRF spectrometry and IC for their elemental and ionic compositions, respectively. During high pollution event days, PM mass concentrations inside the old age home reached 53 μg m− 3 and 32 μg m− 3 whilst outside concentrations were 101 μg m− 3 and 46 μg m− 3 for PM2.5 and PM1, respectively. The sum of nss-sulphate, nitrate and ammonium, dominate the composition of PM, and contribute the most towards an increase in the PM during the episode days constituting 64% of ambient PM2.5 (52 μg m− 3) compared to 39% on non-episode days (10 μg m− 3). Other PM components, such as mineral dust, sea salt or heavy metals were found to be considerably higher during PM episodes but relatively less important. Amongst heavy metals Zn and Pb were found at the highest concentrations in both PM2.5 and PM1. Acidbase ionic balance equations were calculated and point to acidic aerosols during event days and acidic to alkaline aerosols during non-event days. No significant sources of indoor pollutants could be identified inside the old-age home as high correlations were found between outdoor and indoor PM, confirming mainly the outdoor origin of indoor air. |
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000347293800015 |
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2014-05-21 |
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ISSN |
0048-9697 |
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Additional Links |
UA library record; WoS full record; WoS citing articles |
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Impact Factor |
4.9 |
Times cited |
27 |
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Notes |
; The work reported in this paper was financed by the Belgian Science Policy under the Science for Sustainable Development programme (SD/HE/01), the Flemish Scientific Fund (FWO:G.0873.11). We thank the direction and staff of the elderly homes for their support. The authors are thankful to the partners of the project Lotte Jacobs, Tim Nawrot and Benoit Nemery for taking care of project organization, Andy Delcoo, Jo Dewulf and Hugo De Backer from Royal Meteorological Institute, Brussels, Belgium for supplying the meteorological data. We acknowledge Dr. Laszlo Bencs for assistance regarding backward trajectory analyses and two reviewers for their constructive comments. The authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (http://www.ready.noaa.gov) used in this publication. ; |
Approved |
Most recent IF: 4.9; 2014 IF: 4.099 |
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Call Number  |
UA @ admin @ c:irua:117005 |
Serial |
5544 |
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Author |
Van Grieken, R. |
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Title |
Ocean-atmosphere interactions and oil pollution |
Type |
P3 Proceeding |
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Year |
1974 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117457 |
Serial |
8325 |
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Van Grieken, R. |
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Title |
Aerosol composition studies using accelerator proton bombardment |
Type |
P3 Proceeding |
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Year |
1974 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117458 |
Serial |
7424 |
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Winchester, J.W.; Meinert, D.L.; Nelson, J.W.; Johansson, T.B.; Van Grieken, R.E.; Orsini, C.; Kaufmann, H.C.; Akselsson, R. |
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Title |
Trace metals in the St-Louis aerosol |
Type |
H3 Book chapter |
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Year |
1975 |
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Volume |
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Issue |
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Pages |
385-394
T2 - Nuclear techniques in environmental r |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117459 |
Serial |
8694 |
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Author |
Johansson, T.B.; Van Grieken, R.E.; Winchester, J.W. |
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Title |
Interpretation of aerosol trace metal particle size distributions |
Type |
H3 Book chapter |
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Year |
1975 |
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Volume |
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Pages |
356-365
T2 - Nuclear techniques in environmental r |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117460 |
Serial |
8117 |
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Author |
Vanderborght, B.; Van Grieken, R. |
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Title |
Energy-dispersive X-ray fluorescence for trace metals analysis of water |
Type |
H3 Book chapter |
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1975 |
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Pages |
1-9
T2 - Nuclear techniques in environmental resea |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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Call Number |
UA @ admin @ c:irua:117461 |
Serial |
7905 |
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Author |
Van Grieken, R. |
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Title |
Martime influences on the atmospheric aerosol composition |
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H3 Book chapter |
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1977 |
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139-148
T2 - Studie en beheer van het mariene syst |
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H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117463 |
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8205 |
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Annegarn, H.J.; Van Grieken, R.E.; Winchester, J.W.; Sellschop, J.P.F.; von Blottnitz, F. |
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Title |
Background aerosol concentrations at the Namib-Atlantic interface |
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P3 Proceeding |
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1979 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA @ admin @ c:irua:117465 |
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7546 |
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Author |
Van Grieken, R.; Hoste, J. |
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Title |
Annotated bibliography on 14 MeV neutron activation analysis |
Type |
MA3 Book as author |
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1972 |
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293 p. |
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MA3 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117467 |
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7461 |
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Author |
Camuffo, D.; Pagan, E.; Schellen, H.; Van Grieken, R.; Bencs, L.; et al. |
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Title |
Church heating and cultural heritage conservation : guide to the analysis of pros and cons of various heating systems |
Type |
MA2 Book as author |
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2006 |
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240 p. |
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MA2 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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88-370-5034-8 |
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UA @ admin @ c:irua:117468 |
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7665 |
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Author |
Van Grieken, R. |
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Title |
Analyse van ferro-metalen door activering met 14 MeV neutronen |
Type |
MA3 Book as author |
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1973 |
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128 p. |
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MA3 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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UA @ admin @ c:irua:117470 |
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7440 |
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Van Grieken, R.; Wollast, R. |
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Title |
Progress in Belgian oceanographic research : proceedings of symposium, Brussels, 3-5 March 1985 |
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1985 |
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479 p. |
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ME3 Book as editor; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117474 |
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8422 |
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Maenhaut, W.; Selen, A.; van Espen, P.; Van Grieken, R.; Winchester, J.W. |
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Title |
Sulfur and heavy metals over the Atlantic Ocean : comparison with other marine data |
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P3 Proceeding |
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Year |
1980 |
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P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3) |
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Call Number |
UA @ admin @ c:irua:117480 |
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8618 |
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Author |
Robberecht, H.; Van Grieken, R. |
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Title |
Selenium content and speciation in environmental waters determied by X-ray fluorescence spectroscopy |
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1980 |
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362-366
T2 - Trace substances in environmental hea |
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H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Call Number |
UA @ admin @ c:irua:117481 |
Serial |
8505 |
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Author |
Robberecht, H.; Van Grieken, R.; Van der Sloot, H.A. |
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Title |
OPtimized selenite determination in environmental waters by X-ray fluorescence |
Type |
H3 Book chapter |
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Year |
1980 |
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463-468
T2 - Analytical techniques in environmenta |
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H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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| |
Call Number |
UA @ admin @ c:irua:117482 |
Serial |
8343 |
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| Permanent link to this record |
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| |
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Author |
vanden Berghe, D.; Deelstra, H.; Robberecht, H.; Van Grieken, R. |
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| |
Title |
Selenium content of soils and rye grass (Lolium multiflorum) in Belgium |
Type |
H3 Book chapter |
| |
Year |
1981 |
Publication |
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Abbreviated Journal |
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| |
Volume |
|
Issue |
|
Pages |
85-105
T2 - Mineral elements '80 : part 1 |
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| |
Keywords |
H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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no |
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| |
Call Number |
UA @ admin @ c:irua:117483 |
Serial |
8506 |
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| Permanent link to this record |
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| |
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Author |
Van Dyck, P.; Van Grieken, R. |
|
| |
Title |
Automated energy-dispersive X-ray fluorescence analysis for diverse environmental samples |
Type |
H3 Book chapter |
| |
Year |
1982 |
Publication |
|
Abbreviated Journal |
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| |
Volume |
|
Issue |
|
Pages |
315-324
T2 - Analytical techniques in environmenta |
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Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Notes |
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Approved |
no |
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| |
Call Number |
UA @ admin @ c:irua:117484 |
Serial |
7536 |
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| Permanent link to this record |
| |
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| |
|
Author |
Van Grieken, R.; Robberecht, H.; Shani, J.; Van Dyck, P.; Vos, L. |
|
| |
Title |
Energy-dispersive X-ray fluorescence for direct trace analysis of biomedical and environmental samples |
Type |
H3 Book chapter |
| |
Year |
1982 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
159-178
T2 - X-ray fluorescence (XRF and PIXE) in |
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| |
Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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Additional Links |
UA library record |
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Open Access |
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|
| |
Notes |
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Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117485 |
Serial |
7904 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Vos, L.; Van Grieken, R. |
|
| |
Title |
Spark source mass spectrometry for trace analysis of diverse biological matrices |
Type |
H3 Book chapter |
| |
Year |
1983 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
303-306
T2 - Mass spectrometry advances 1982 / Sch |
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| |
Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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| |
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|
Additional Links |
UA library record |
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| |
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Open Access |
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|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117486 |
Serial |
8564 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Verbueken, A.; Paulus, G.; Van de Vyver, F.; Verpooten, G.; de Broe, M.; Van Grieken, R. |
|
| |
Title |
LAMMA : calibration and application to nephrotoxicology studies |
Type |
P3 Proceeding |
| |
Year |
1983 |
Publication |
|
Abbreviated Journal |
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|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
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| |
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Additional Links |
UA library record |
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| |
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117491 |
Serial |
8149 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Verbueken, A.H.; Paulus, G.J.; Van de Vyver, F.L.; Verpooten, G.A.; Visser, W.J.; de Broe, M.E.; Van Grieken, R.E. |
|
| |
Title |
LAMMA in nephrotoxicity studies |
Type |
P3 Proceeding |
| |
Year |
1984 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
|
| |
Abstract |
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| |
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|
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|
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|
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| |
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|
ISBN |
|
Additional Links |
UA library record |
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| |
Impact Factor |
|
Times cited |
|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117492 |
Serial |
8150 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Verbueken, A.H.; Van de Vyver, F.L.; Paulus, G.J.; Visser, W.J.; Verpooten, G.A.; de Broe, M.E.; Van Grieken, R.E. |
|
| |
Title |
Laser microprobe mass analysis (LAMMA) in nephrological investigations |
Type |
H3 Book chapter |
| |
Year |
1984 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
375-382
T2 - Trace element analytical chemistry in |
|
| |
Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
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| |
Abstract |
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| |
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|
ISBN |
|
Additional Links |
UA library record |
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| |
Impact Factor |
|
Times cited |
|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117493 |
Serial |
8156 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Bruynseels, F.; Van Grieken, R. |
|
| |
Title |
Speciation and distribution of sulfur and nitrogen in individual aerosol particles measured by LAMMA |
Type |
P3 Proceeding |
| |
Year |
1984 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
|
| |
Abstract |
|
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| |
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|
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|
|
| |
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|
ISBN |
|
Additional Links |
UA library record |
|
| |
Impact Factor |
|
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117494 |
Serial |
8568 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Van Grieken, R.E.; LaBrecque, J.J. |
|
| |
Title |
Trace analysis of environmental samples by X-ray emission spectroscopy |
Type |
H3 Book chapter |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
101-183
T2 - Trace analysis : vol. 4 / Lawrence, J |
|
| |
Keywords |
H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
|
| |
Abstract |
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| |
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|
Additional Links |
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| |
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|
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117495 |
Serial |
8686 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Visser, W.J.; Van de Vyver, F.L.; Verbueken, A.H.; d'Haese, P.; Bekaert, A.B.; Van Grieken, R.E.; Duursma, S.A.; de Broe, M.E. |
|
| |
Title |
Evaluation of different techniques used to determine aluminium in patients with chronic renal failure |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; Pathophysiology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP) |
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| |
Abstract |
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Additional Links |
UA library record |
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| |
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|
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117496 |
Serial |
7938 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
|
| |
Title |
Chemical characterization of individual aerosol particles from remote and polluted marine air |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
|
| |
Abstract |
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|
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| |
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|
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|
Additional Links |
UA library record |
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| |
Impact Factor |
|
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117497 |
Serial |
7647 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Bernard, P.; Van Grieken, R.; Eisma, D. |
|
| |
Title |
Study of individual estuarine suspension particles by automated electron-probe X-ray microanalysis |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
|
| |
Abstract |
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Address |
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| |
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Series Issue |
|
Edition |
|
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| |
ISSN |
|
ISBN |
|
Additional Links |
UA library record |
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| |
Impact Factor |
|
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|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117498 |
Serial |
8598 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Keppens, E.; Roekens, E.; Van Grieken, R. |
|
| |
Title |
Effect of pollution on sandy limestones of a historical cathedral in Belgium |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
|
| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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| |
Abstract |
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| |
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Wos |
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|
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| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
|
ISBN |
|
Additional Links |
UA library record |
|
| |
Impact Factor |
|
Times cited |
|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117499 |
Serial |
7838 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Bruynseels, F.; Storms, H.; Van Grieken, R. |
|
| |
Title |
Chemical characterization of airborne particulate matter above the North Sea |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
|
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| |
Volume |
|
Issue |
|
Pages |
|
|
| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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| |
Abstract |
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| |
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|
Wos |
|
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| |
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|
Series Title |
|
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|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
|
ISBN |
|
Additional Links |
UA library record |
|
| |
Impact Factor |
|
Times cited |
|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117500 |
Serial |
7646 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Van Grieken, R. |
|
| |
Title |
Stof : begrippen, bronnen en analysmethoden |
Type |
P3 Proceeding |
| |
Year |
1985 |
Publication |
|
Abbreviated Journal |
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| |
Volume |
|
Issue |
|
Pages |
|
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| |
Keywords |
P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation) |
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| |
Abstract |
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| |
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|
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|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
|
ISBN |
|
Additional Links |
UA library record |
|
| |
Impact Factor |
|
Times cited |
|
Open Access |
|
|
| |
Notes |
|
Approved |
no |
|
| |
Call Number |
UA @ admin @ c:irua:117501 |
Serial |
8582 |
|
| Permanent link to this record |
