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Author Buczyńska, A.J.; Krata, A.; Van Grieken, R.; Brown, A.; Polezer, G.; De Wael, K.; Potgieter-Vermaak, S.
Title Composition of PM2.5 and PM1 on high and low pollution event days and its relation to indoor air quality in a home for the elderly Type A1 Journal article
Year 2014 Publication The science of the total environment Abbreviated Journal Sci Total Environ
Volume 490 Issue Pages 134-143
Keywords A1 Journal article; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
Abstract Many studies probing the link between air quality and health have pointed towards associations between particulate matter (PM) exposure and decreased lung function, aggravation of respiratory diseases like asthma, premature death and increased hospitalisation admissions for the elderly and individuals with cardiopulmonary diseases. Of recent, it is believed that the chemical composition and physical properties of PM may contribute significantly to these adverse health effects. As part of a Belgian Science Policy project (Health effects of particulate matter in relation to physicalchemical characteristics and meteorology), the chemical composition (elemental and ionic compositions) and physical properties (PM mass concentrations) of PM were investigated, indoors and outdoors of old age homes in Antwerp. The case reported here specifically relates to high versus normal/low pollution event periods. PM mass concentrations for PM1 and PM2.5 fractions were determined gravimetrically after collection via impaction. These same samples were hence analysed by EDXRF spectrometry and IC for their elemental and ionic compositions, respectively. During high pollution event days, PM mass concentrations inside the old age home reached 53 μg m− 3 and 32 μg m− 3 whilst outside concentrations were 101 μg m− 3 and 46 μg m− 3 for PM2.5 and PM1, respectively. The sum of nss-sulphate, nitrate and ammonium, dominate the composition of PM, and contribute the most towards an increase in the PM during the episode days constituting 64% of ambient PM2.5 (52 μg m− 3) compared to 39% on non-episode days (10 μg m− 3). Other PM components, such as mineral dust, sea salt or heavy metals were found to be considerably higher during PM episodes but relatively less important. Amongst heavy metals Zn and Pb were found at the highest concentrations in both PM2.5 and PM1. Acidbase ionic balance equations were calculated and point to acidic aerosols during event days and acidic to alkaline aerosols during non-event days. No significant sources of indoor pollutants could be identified inside the old-age home as high correlations were found between outdoor and indoor PM, confirming mainly the outdoor origin of indoor air.
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Language Wos 000347293800015 Publication Date 2014-05-21
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ISSN 0048-9697 ISBN Additional Links UA library record; WoS full record; WoS citing articles
Impact Factor 4.9 Times cited 27 Open Access
Notes ; The work reported in this paper was financed by the Belgian Science Policy under the Science for Sustainable Development programme (SD/HE/01), the Flemish Scientific Fund (FWO:G.0873.11). We thank the direction and staff of the elderly homes for their support. The authors are thankful to the partners of the project Lotte Jacobs, Tim Nawrot and Benoit Nemery for taking care of project organization, Andy Delcoo, Jo Dewulf and Hugo De Backer from Royal Meteorological Institute, Brussels, Belgium for supplying the meteorological data. We acknowledge Dr. Laszlo Bencs for assistance regarding backward trajectory analyses and two reviewers for their constructive comments. The authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (http://www.ready.noaa.gov) used in this publication. ; Approved Most recent IF: 4.9; 2014 IF: 4.099
Call Number (up) UA @ admin @ c:irua:117005 Serial 5544
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Author Van Grieken, R.
Title Ocean-atmosphere interactions and oil pollution Type P3 Proceeding
Year 1974 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117457 Serial 8325
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Author Van Grieken, R.
Title Aerosol composition studies using accelerator proton bombardment Type P3 Proceeding
Year 1974 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117458 Serial 7424
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Author Winchester, J.W.; Meinert, D.L.; Nelson, J.W.; Johansson, T.B.; Van Grieken, R.E.; Orsini, C.; Kaufmann, H.C.; Akselsson, R.
Title Trace metals in the St-Louis aerosol Type H3 Book chapter
Year 1975 Publication Abbreviated Journal
Volume Issue Pages 385-394 T2 - Nuclear techniques in environmental r
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117459 Serial 8694
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Author Johansson, T.B.; Van Grieken, R.E.; Winchester, J.W.
Title Interpretation of aerosol trace metal particle size distributions Type H3 Book chapter
Year 1975 Publication Abbreviated Journal
Volume Issue Pages 356-365 T2 - Nuclear techniques in environmental r
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117460 Serial 8117
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Author Vanderborght, B.; Van Grieken, R.
Title Energy-dispersive X-ray fluorescence for trace metals analysis of water Type H3 Book chapter
Year 1975 Publication Abbreviated Journal
Volume Issue Pages 1-9 T2 - Nuclear techniques in environmental resea
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117461 Serial 7905
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Author Van Grieken, R.
Title Martime influences on the atmospheric aerosol composition Type H3 Book chapter
Year 1977 Publication Abbreviated Journal
Volume Issue Pages 139-148 T2 - Studie en beheer van het mariene syst
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117463 Serial 8205
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Author Annegarn, H.J.; Van Grieken, R.E.; Winchester, J.W.; Sellschop, J.P.F.; von Blottnitz, F.
Title Background aerosol concentrations at the Namib-Atlantic interface Type P3 Proceeding
Year 1979 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Call Number (up) UA @ admin @ c:irua:117465 Serial 7546
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Author Van Grieken, R.; Hoste, J.
Title Annotated bibliography on 14 MeV neutron activation analysis Type MA3 Book as author
Year 1972 Publication Abbreviated Journal
Volume Issue Pages 293 p.
Keywords MA3 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117467 Serial 7461
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Author Camuffo, D.; Pagan, E.; Schellen, H.; Van Grieken, R.; Bencs, L.; et al.
Title Church heating and cultural heritage conservation : guide to the analysis of pros and cons of various heating systems Type MA2 Book as author
Year 2006 Publication Abbreviated Journal
Volume Issue Pages 240 p.
Keywords MA2 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Language Wos Publication Date
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ISSN ISBN 88-370-5034-8 Additional Links UA library record
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117468 Serial 7665
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Author Van Grieken, R.
Title Analyse van ferro-metalen door activering met 14 MeV neutronen Type MA3 Book as author
Year 1973 Publication Abbreviated Journal
Volume Issue Pages 128 p.
Keywords MA3 Book as author; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Call Number (up) UA @ admin @ c:irua:117470 Serial 7440
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Author Van Grieken, R.; Wollast, R.
Title Progress in Belgian oceanographic research : proceedings of symposium, Brussels, 3-5 March 1985 Type ME3 Book as editor
Year 1985 Publication Abbreviated Journal
Volume Issue Pages 479 p.
Keywords ME3 Book as editor; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Call Number (up) UA @ admin @ c:irua:117474 Serial 8422
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Author Maenhaut, W.; Selen, A.; van Espen, P.; Van Grieken, R.; Winchester, J.W.
Title Sulfur and heavy metals over the Atlantic Ocean : comparison with other marine data Type P3 Proceeding
Year 1980 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Chemometrics (Mitac 3)
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Call Number (up) UA @ admin @ c:irua:117480 Serial 8618
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Author Robberecht, H.; Van Grieken, R.
Title Selenium content and speciation in environmental waters determied by X-ray fluorescence spectroscopy Type H3 Book chapter
Year 1980 Publication Abbreviated Journal
Volume Issue Pages 362-366 T2 - Trace substances in environmental hea
Keywords H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117481 Serial 8505
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Author Robberecht, H.; Van Grieken, R.; Van der Sloot, H.A.
Title OPtimized selenite determination in environmental waters by X-ray fluorescence Type H3 Book chapter
Year 1980 Publication Abbreviated Journal
Volume Issue Pages 463-468 T2 - Analytical techniques in environmenta
Keywords H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117482 Serial 8343
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Author vanden Berghe, D.; Deelstra, H.; Robberecht, H.; Van Grieken, R.
Title Selenium content of soils and rye grass (Lolium multiflorum) in Belgium Type H3 Book chapter
Year 1981 Publication Abbreviated Journal
Volume Issue Pages 85-105 T2 - Mineral elements '80 : part 1
Keywords H3 Book chapter; Pharmacology. Therapy; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117483 Serial 8506
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Author Van Dyck, P.; Van Grieken, R.
Title Automated energy-dispersive X-ray fluorescence analysis for diverse environmental samples Type H3 Book chapter
Year 1982 Publication Abbreviated Journal
Volume Issue Pages 315-324 T2 - Analytical techniques in environmenta
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117484 Serial 7536
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Author Van Grieken, R.; Robberecht, H.; Shani, J.; Van Dyck, P.; Vos, L.
Title Energy-dispersive X-ray fluorescence for direct trace analysis of biomedical and environmental samples Type H3 Book chapter
Year 1982 Publication Abbreviated Journal
Volume Issue Pages 159-178 T2 - X-ray fluorescence (XRF and PIXE) in
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117485 Serial 7904
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Author Vos, L.; Van Grieken, R.
Title Spark source mass spectrometry for trace analysis of diverse biological matrices Type H3 Book chapter
Year 1983 Publication Abbreviated Journal
Volume Issue Pages 303-306 T2 - Mass spectrometry advances 1982 / Sch
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117486 Serial 8564
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Author Verbueken, A.; Paulus, G.; Van de Vyver, F.; Verpooten, G.; de Broe, M.; Van Grieken, R.
Title LAMMA : calibration and application to nephrotoxicology studies Type P3 Proceeding
Year 1983 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117491 Serial 8149
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Author Verbueken, A.H.; Paulus, G.J.; Van de Vyver, F.L.; Verpooten, G.A.; Visser, W.J.; de Broe, M.E.; Van Grieken, R.E.
Title LAMMA in nephrotoxicity studies Type P3 Proceeding
Year 1984 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP)
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Call Number (up) UA @ admin @ c:irua:117492 Serial 8150
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Author Verbueken, A.H.; Van de Vyver, F.L.; Paulus, G.J.; Visser, W.J.; Verpooten, G.A.; de Broe, M.E.; Van Grieken, R.E.
Title Laser microprobe mass analysis (LAMMA) in nephrological investigations Type H3 Book chapter
Year 1984 Publication Abbreviated Journal
Volume Issue Pages 375-382 T2 - Trace element analytical chemistry in
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117493 Serial 8156
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Author Bruynseels, F.; Van Grieken, R.
Title Speciation and distribution of sulfur and nitrogen in individual aerosol particles measured by LAMMA Type P3 Proceeding
Year 1984 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117494 Serial 8568
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Author Van Grieken, R.E.; LaBrecque, J.J.
Title Trace analysis of environmental samples by X-ray emission spectroscopy Type H3 Book chapter
Year 1985 Publication Abbreviated Journal
Volume Issue Pages 101-183 T2 - Trace analysis : vol. 4 / Lawrence, J
Keywords H3 Book chapter; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117495 Serial 8686
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Author Visser, W.J.; Van de Vyver, F.L.; Verbueken, A.H.; d'Haese, P.; Bekaert, A.B.; Van Grieken, R.E.; Duursma, S.A.; de Broe, M.E.
Title Evaluation of different techniques used to determine aluminium in patients with chronic renal failure Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; Pathophysiology; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation); Laboratory Experimental Medicine and Pediatrics (LEMP)
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ISSN ISBN Additional Links UA library record
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117496 Serial 7938
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Author Bruynseels, F.; Storms, H.; Van Grieken, R.
Title Chemical characterization of individual aerosol particles from remote and polluted marine air Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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ISSN ISBN Additional Links UA library record
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117497 Serial 7647
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Author Bernard, P.; Van Grieken, R.; Eisma, D.
Title Study of individual estuarine suspension particles by automated electron-probe X-ray microanalysis Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117498 Serial 8598
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Author Keppens, E.; Roekens, E.; Van Grieken, R.
Title Effect of pollution on sandy limestones of a historical cathedral in Belgium Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117499 Serial 7838
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Author Bruynseels, F.; Storms, H.; Van Grieken, R.
Title Chemical characterization of airborne particulate matter above the North Sea Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117500 Serial 7646
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Author Van Grieken, R.
Title Stof : begrippen, bronnen en analysmethoden Type P3 Proceeding
Year 1985 Publication Abbreviated Journal
Volume Issue Pages
Keywords P3 Proceeding; AXES (Antwerp X-ray Analysis, Electrochemistry and Speciation)
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Notes Approved no
Call Number (up) UA @ admin @ c:irua:117501 Serial 8582
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